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Effect of particle aggregation on thermal conductivity of nanofluids: Enhancement of phonon MFP SCIE
期刊论文 | 2019 , 125 (1) | JOURNAL OF APPLIED PHYSICS
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Abstract :

Particle aggregation in nanofluids is a common phenomenon. Some studies indicated that aggregation can increase the thermal conductivity of nanofluids due to the formation of an "efficient heat channel," while the underlying mechanism is still unclear. In this study, an effective medium model considering phonon scattering is applied to explore the effect of particle aggregation on nanofluid thermal conductivity. The aggregation is simulated by a diffusion-limit-cluster-aggregation model, where the effects of nanoparticle size, concentration, and number in a cluster on the aggregation structure are studied. Results show that nanoparticle aggregation can dramatically increase the thermal conductivity of nanofluids, and aggregation puts up stronger effects for the case of smaller nanoparticles and lower concentrations. The main mechanism is that the aggregation raises the phonon MFP in the solid phase, which further results in the thermal conductivity enhancement of nanoparticles. Published under license by AIP Publishing.

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GB/T 7714 Song, Dongxing , Jing, Dengwei , Ma, Weigang et al. Effect of particle aggregation on thermal conductivity of nanofluids: Enhancement of phonon MFP [J]. | JOURNAL OF APPLIED PHYSICS , 2019 , 125 (1) .
MLA Song, Dongxing et al. "Effect of particle aggregation on thermal conductivity of nanofluids: Enhancement of phonon MFP" . | JOURNAL OF APPLIED PHYSICS 125 . 1 (2019) .
APA Song, Dongxing , Jing, Dengwei , Ma, Weigang , Zhang, Xing . Effect of particle aggregation on thermal conductivity of nanofluids: Enhancement of phonon MFP . | JOURNAL OF APPLIED PHYSICS , 2019 , 125 (1) .
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Unassisted solar water splitting with 9.8% efficiency and over 100 h stability based on Si solar cells and photoelectrodes catalyzed by bifunctional Ni-Mo/Ni SCIE
期刊论文 | 2019 , 7 (5) , 2200-2209 | JOURNAL OF MATERIALS CHEMISTRY A
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Designing a highly efficient and stable photoelectrochemical (PEC) tandem cell for unassisted solar water splitting is considered a promising approach for large-scale solar energy storage. To date, various tandem device configurations have been reported. However, the achievement of a solar-to-hydrogen conversion efficiency (eta(STH)) of 10% is still full of challenges, due to the incompatibility between the two photoelectrode materials. Here, we report a highly efficient and stable photovoltaic (PV)-PEC tandem device composed of a dual Si photoelectrode and two series-connected ordinary Si PV cells. The dual-photoelectrode device consists of an n(+)np(+)-Si photocathode and p(+)pn(+)-Si photoanode, which allow back illumination from the Si substrate, spatially and functionally decoupling the optical absorption and the catalytic activity. By further employing a Ni protective layer together with a bifunctional Ni-Mo catalyst for both the Si photocathode and photoanode, the PV-PEC tandem cell can perform spontaneous water splitting without any applied bias. A high eta(STH) of 9.8% with a stability of over 100 h was achieved in alkaline solution under parallel AM 1.5G 1 sun illumination. This work essentially allows a modular independent optimization of each component which can enhance the efficiency and stability of the PV-PEC cells.

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GB/T 7714 Fan, Ronglei , Cheng, Shaobo , Huang, Guanping et al. Unassisted solar water splitting with 9.8% efficiency and over 100 h stability based on Si solar cells and photoelectrodes catalyzed by bifunctional Ni-Mo/Ni [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2019 , 7 (5) : 2200-2209 .
MLA Fan, Ronglei et al. "Unassisted solar water splitting with 9.8% efficiency and over 100 h stability based on Si solar cells and photoelectrodes catalyzed by bifunctional Ni-Mo/Ni" . | JOURNAL OF MATERIALS CHEMISTRY A 7 . 5 (2019) : 2200-2209 .
APA Fan, Ronglei , Cheng, Shaobo , Huang, Guanping , Wang, Yongjie , Zhang, Yazhou , Vanka, Srinivas et al. Unassisted solar water splitting with 9.8% efficiency and over 100 h stability based on Si solar cells and photoelectrodes catalyzed by bifunctional Ni-Mo/Ni . | JOURNAL OF MATERIALS CHEMISTRY A , 2019 , 7 (5) , 2200-2209 .
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Strengthened spatial charge separation over Z-scheme heterojunction photocatalyst for efficient photocatalytic H-2 evolution SCIE
期刊论文 | 2019 , 475 , 453-461 | APPLIED SURFACE SCIENCE
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Abstract :

Graphitic carbon nitride (g-C3N4) is a very promising earth abundant and visible light response photocatalyst for H-2 production. Fabricating novel nanostructure or combining with other semiconductors have been attempted to further enhance its activity. alpha-FeOOH, due to its structures greatly facilitating electrolyte transport, has been widely used as an excellent OER cocatalyst assisting the PEC water splitting process. However, to the best of our knowledge, it has not been attempted in photocatalytic H-2 generation. Herein, g-C3N4 modified with beta-FeOOH was designed for the first time for photocatalytic H-2 production. It showed H-2 production rate as 2.02 mmol.h(-1).g(-1), which was almost 6 times of pure g-C3N4. The significantly promoted catalytic activity was ascribed to the greatly enhanced charge separation efficiency by forming spatial separated reservoirs of photo activated electrons and holes in the Z-scheme heterojunction, corresponding to the conduction band of g-C3N4 and the valence band of beta-FeOOH, respectively. Our work should be valuable for fabricating visible-light response heterojunction based photocatalysts with better photocatalytic performance.

Keyword :

beta-FeOOH Graphitic carbon nitride Hydrogen evolution Photocatalysis Heterojunction

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GB/T 7714 Lu, Bing , Song, Rui , Geng, Jiafeng et al. Strengthened spatial charge separation over Z-scheme heterojunction photocatalyst for efficient photocatalytic H-2 evolution [J]. | APPLIED SURFACE SCIENCE , 2019 , 475 : 453-461 .
MLA Lu, Bing et al. "Strengthened spatial charge separation over Z-scheme heterojunction photocatalyst for efficient photocatalytic H-2 evolution" . | APPLIED SURFACE SCIENCE 475 (2019) : 453-461 .
APA Lu, Bing , Song, Rui , Geng, Jiafeng , Jing, Dengwei , Huang, Zhenxiong . Strengthened spatial charge separation over Z-scheme heterojunction photocatalyst for efficient photocatalytic H-2 evolution . | APPLIED SURFACE SCIENCE , 2019 , 475 , 453-461 .
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Significantly enhanced photocatalytic hydrogen generation over graphitic carbon nitride with carefully modified intralayer structures EI SCIE Scopus
期刊论文 | 2018 , 332 , 499-507 | CHEMICAL ENGINEERING JOURNAL
WoS CC Cited Count: 7 SCOPUS Cited Count: 9
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Graphitic carbon nitride has been widely investigated as promising photocatalyst for solar-driven photocatalytic hydrogen production. In this study, the intralayer properties of graphitic carbon nitride was modified by a facile hydrothermal treatment with appropriate amount of ammonium hydroxide to promote its photocatalytic H-2 production performance. Transition from intralayer modification to bulk structural transformation occurred once the concentration of NH3 center dot H2O is over certain concentration. The destruction of heptazine units resulted in the partial oxidation of C atoms in g-C3N4 during the hydrothermal treatment process and the introduction of -OH and -C=O- can effectively enhance the interaction between g-C3N4 with reactants. Band structure measurement revealed that the thus obtained g-C3N4 possessed elevated conduction band bottom indicative of improved reduction capacities. The significantly enhanced redox ability on the surface reaction sites overcame the deceased light absorption and higher charge recombination efficiency of charge carriers, and finally induced a significantly improved photocatalytic H-2 evolution (707.58 mu mol.h(-1).g(-1)). The highest visible light photocatalytic H-2 evolution rate was 7.5 times higher than that of pristine graphitic carbon nitride (94.46 mu mol.h(-1).g(-1)), with an apparent quantum yield of 5.18% at 420 nm. This study demonstrates a facile and effective strategy to tune the electronic and photocatalytic properties of carbon nitride for improved solar energy conversion efficiency which are expected to be extended to the modifications of other photocatalytic materials.

Keyword :

Photocatalysis Carbon nitride Ammonium hydroxide Hydrothermal treatment

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GB/T 7714 Luo, Bing , Song, Rui , Jing, Dengwei . Significantly enhanced photocatalytic hydrogen generation over graphitic carbon nitride with carefully modified intralayer structures [J]. | CHEMICAL ENGINEERING JOURNAL , 2018 , 332 : 499-507 .
MLA Luo, Bing et al. "Significantly enhanced photocatalytic hydrogen generation over graphitic carbon nitride with carefully modified intralayer structures" . | CHEMICAL ENGINEERING JOURNAL 332 (2018) : 499-507 .
APA Luo, Bing , Song, Rui , Jing, Dengwei . Significantly enhanced photocatalytic hydrogen generation over graphitic carbon nitride with carefully modified intralayer structures . | CHEMICAL ENGINEERING JOURNAL , 2018 , 332 , 499-507 .
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Dynamic properties of polydisperse colloidal particles in the presence of thermal gradient studied by a modified Brownian dynamic model EI SCIE Scopus
期刊论文 | 2018 , 51 (10) | JOURNAL OF PHYSICS D-APPLIED PHYSICS
WoS CC Cited Count: 2 SCOPUS Cited Count: 2
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Abstract :

Aggregation and migration of colloidal particles under the thermal gradient widely exists in nature and many industrial processes. In this study, dynamic properties of polydisperse colloidal particles in the presence of thermal gradient were studied by a modified Brownian dynamic model. Other than the traditional forces on colloidal particles, including Brownian force, hydrodynamic force, and electrostatic force from other particles, the electrostatic force from the asymmetric ionic diffusion layer under a thermal gradient has been considered and introduced into the Brownian dynamic model. The aggregation ratio of particles (R-A), the balance time (t(B)) indicating the time threshold when RA becomes constant, the porosity (P-BA), fractal dimension (D-f) and distributions of concentration (DISC) and aggregation (DISA) for the aggregated particles were discussed based on this model. The aggregated structures formed by polydisperse particles are less dense and the particles therein are loosely bonded. Also it showed a quite large compressibility as the increases of concentration and interparticle potential can significantly increase the fractal dimension. The thermal gradient can induce two competitive factors leading to a two-stage migration of particles. When t < t(B), the unsynchronized aggregation is dominant and the particles slightly migrate along the thermal gradient. When t > t(B), the thermophoresis becomes dominant thus the migrations of particles are against the thermal gradient. The effect of thermophoresis on the aggregate structures was found to be similar to the effect of increasing particle concentration. This study demonstrates how the thermal gradient affects the aggregation of monodisperse and polydisperse particles and can be a guide for the biomimetics and precise control of colloid system under the thermal gradient. Moreover, our model can be easily extended to other more complex colloidal systems considering shear, temperature fluctuation, surfactant, etc.

Keyword :

polydisperse particles modified Brownian dynamic model aggregation thermal gradient

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GB/T 7714 Song, Dongxing , Jin, Hui , Jing, Dengwei et al. Dynamic properties of polydisperse colloidal particles in the presence of thermal gradient studied by a modified Brownian dynamic model [J]. | JOURNAL OF PHYSICS D-APPLIED PHYSICS , 2018 , 51 (10) .
MLA Song, Dongxing et al. "Dynamic properties of polydisperse colloidal particles in the presence of thermal gradient studied by a modified Brownian dynamic model" . | JOURNAL OF PHYSICS D-APPLIED PHYSICS 51 . 10 (2018) .
APA Song, Dongxing , Jin, Hui , Jing, Dengwei , Wang, Xin . Dynamic properties of polydisperse colloidal particles in the presence of thermal gradient studied by a modified Brownian dynamic model . | JOURNAL OF PHYSICS D-APPLIED PHYSICS , 2018 , 51 (10) .
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Synthesis of AgI/Bi2MoO6 nano-heterostructure with enhanced visible-light photocatalytic property SCIE Scopus CSCD
期刊论文 | 2018 , 28 (2) , 235-241 | PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL
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A novel nano-heterostructure of AgI/Bi2MoO6 photocatalyst was successfully synthesized via a facile depositionprecipitation method. The samples were systematically characterized by X-ray diffraction, scanning and transmission electron microscopy, X-ray photoemission spectroscopy, UV-Vis absorption spectroscopy, and photoluminescence spectra. While sole Bi2MoO6 or AgI showed poor activity toward photocatalytic rhodamine B degradation, the nano-heterostructure was found with superior performance. The AgI/Bi2MoO6 composite with an optimal content of 20 wt% AgI exhibited the highest photocatalytic degradation rate. Rhodamine B was totally degraded within 75 min visible-light irradiation. Moreover, the hybrid photocatalyst also showed a fairly good stability for several-cycle reuse. This study indicates that the AgI/Bi2MoO6 nano-heterostructure can be used as an effective candidate for photocatalytic degradation of organic pollutants.

Keyword :

RhB-degradation Heterostructure Photocatalyst

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GB/T 7714 Zhang, Li , Teng, Hongcheng , Zhou, Jiancheng et al. Synthesis of AgI/Bi2MoO6 nano-heterostructure with enhanced visible-light photocatalytic property [J]. | PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL , 2018 , 28 (2) : 235-241 .
MLA Zhang, Li et al. "Synthesis of AgI/Bi2MoO6 nano-heterostructure with enhanced visible-light photocatalytic property" . | PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL 28 . 2 (2018) : 235-241 .
APA Zhang, Li , Teng, Hongcheng , Zhou, Jiancheng , Sun, Yueming , Li, Naixu , Liu, Maochang et al. Synthesis of AgI/Bi2MoO6 nano-heterostructure with enhanced visible-light photocatalytic property . | PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL , 2018 , 28 (2) , 235-241 .
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Insights into the complex interaction between hydrophilic nanoparticles and ionic surfactants at the liquid/air interface SCIE PubMed Scopus
期刊论文 | 2018 , 20 (22) , 15223-15235 | PHYSICAL CHEMISTRY CHEMICAL PHYSICS
SCOPUS Cited Count: 1
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Combinations of nanoparticles and surfactants have been widely employed in many industrial processes, i.e., boiling and condensation in heat transfer and hydraulic fracturing in shale oil and gas production, etc. However, the underlying mechanism for various phenomena resulting from the addition of nanoparticles into the surfactant solutions is still unclear. For instance, there are contradictory conclusions from the literature regarding the variations of surface tension upon the addition of nanoparticles into surfactant solutions. In this work, the dominating factors determining if the surface activity of the surfactant solution will increase or conversely decrease when adding certain kinds of nanoparticles have been investigated. Two typical hydrophilic nanoparticles, SiO2 and TiO2 with anionic or cationic surfactants, respectively, have been considered. The surface tension has been measured in a wide range of nanoparticle and surfactant concentrations. It was found that the surface tension of the ionic surfactant solution can be further reduced only if nanoparticles of the same charge were added. For instance, a system containing 0.25 CMC SDS and 1 wt% SiO2 behaves similar to a 0.34 CMC SDS-only solution. Interestingly, the observed synergistic effect is found to be more significant if the surfactant concentration is much lower than its CMC for a given nanoparticle content. Moreover, the effect is perfectly reversible. When the nanoparticles were separated from the system, the surface tension values recovered fully to that of the pure surfactants. If nanoparticles of opposite charge were added, however, the surface tension of the surfactant solution increased. Zeta potential measurement and centrifugal treatment have been employed to reveal the interplay between nanoparticles and surfactants and the adsorption behavior of their assemblies at the liquid/air interface. Based on the experimental outcomes, a possible physical mechanism was proposed. It was concluded that the electrostatic repulsion between surfactant molecules and nanoparticles should be the dominant factor responsible for the observed reversible synergistic effect. Our study is expected to contribute to a better understanding of the interfacial phenomenon in nanoparticle-surfactant complex systems.

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GB/T 7714 Jin, Jingyu , Li, Xiaoyan , Geng, Jiafeng et al. Insights into the complex interaction between hydrophilic nanoparticles and ionic surfactants at the liquid/air interface [J]. | PHYSICAL CHEMISTRY CHEMICAL PHYSICS , 2018 , 20 (22) : 15223-15235 .
MLA Jin, Jingyu et al. "Insights into the complex interaction between hydrophilic nanoparticles and ionic surfactants at the liquid/air interface" . | PHYSICAL CHEMISTRY CHEMICAL PHYSICS 20 . 22 (2018) : 15223-15235 .
APA Jin, Jingyu , Li, Xiaoyan , Geng, Jiafeng , Jing, Dengwei . Insights into the complex interaction between hydrophilic nanoparticles and ionic surfactants at the liquid/air interface . | PHYSICAL CHEMISTRY CHEMICAL PHYSICS , 2018 , 20 (22) , 15223-15235 .
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Vacancy-doped homojunction structural TiO2 nanorod, photoelectrodes with greatly enhanced photoelectrochemical activity EI SCIE Scopus
期刊论文 | 2018 , 43 (4) , 2057-2063 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
WoS CC Cited Count: 3
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In this study, we report a simple, effective and universal approach to fabricate homojunction structural TiO2 nanorod array photoelectrodes through doping of gradient distributed oxygen vacancies introduced by annealing in high vacuum with controlled time. The homogeneous junction structure promotes the separation and transport of photoexcited charge carriers, and the photocurrent density of TiO2 nanorod arrays annealed in high vacuum for 2 h was 20 times higher than that of the pristine TiO2 nanorod arrays. The results indicate that annealing in high vacuum with controlled time could form a homojunction structure, which is an effective approach for further enhancing the performance of U-V visible light driven photocatalytic materials for water splitting. (C) 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

Keyword :

TiO2 nanorod arrays Homojunction structure Water splitting High vacuum annealing

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GB/T 7714 Liu, Yichao , Ren, Fen , Shen, Shaohua et al. Vacancy-doped homojunction structural TiO2 nanorod, photoelectrodes with greatly enhanced photoelectrochemical activity [J]. | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2018 , 43 (4) : 2057-2063 .
MLA Liu, Yichao et al. "Vacancy-doped homojunction structural TiO2 nanorod, photoelectrodes with greatly enhanced photoelectrochemical activity" . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 43 . 4 (2018) : 2057-2063 .
APA Liu, Yichao , Ren, Fen , Shen, Shaohua , Chen, Jianan , Fu, Yanming , Cai, Guangxu et al. Vacancy-doped homojunction structural TiO2 nanorod, photoelectrodes with greatly enhanced photoelectrochemical activity . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2018 , 43 (4) , 2057-2063 .
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Time-dependent scattering of incident light of various wavelengths in ferrofluids under external magnetic field EI SCIE Scopus
期刊论文 | 2018 , 447 , 124-133 | JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS
WoS CC Cited Count: 2 SCOPUS Cited Count: 2
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Ferrofluids can exhibit the anisotropic thermodynamic properties under magnetic fields. The dynamic optical properties of ferrofluids in the presence of magnetic fields are of particular interest due to their potential application as various optical devices. Although time-dependent light scattering by ferrofluids have been extensively studied, the effect of wavelength of incident light have been rarely considered. Here, for the first time, we investigated both the time-and wavelength-dependent light scattering in water based ferrofluids containing Fe3O4 nanoparticles under an external magnetic field. The field-induced response behavior of the prepared ferrofluid samples was determined and verified first by thermal conductivity measurement and numerical simulation. Double-beam UV-Vis spectrophotometer was employed to record the temporal evolution of transmitted intensity of incident light of various wavelengths passing through the ferrofluid sample and propagating parallel to the applied field. As expected, the light intensity decreases to a certain value right after the field is turned on due to the thermal fluctuation induced disorder inside the flexible particle chains. Then the light intensity further decreases with time until the appearance of a minimum at time tau(0) followed by an inversed increase before finally reaches equilibrium at a particular time. More importantly, the characteristic inversion time tau(0) was found to follow a power law increase with the wavelength of incident light (tau(0) similar to lambda(alpha), where alpha = 2.07). A quantitative explanation for the wavelength dependence of characteristic time was proposed based on the finite-difference time-domain (FDTD) method. The simulation results are in good agreement with our experimental observations. The time-dependent light scattering in ferrofluids under different incident wavelengths was rationalized by considering both the coarsening process of the particle chains and the occurrence of resonance within the magnetic scatterers. Our finding should be of value for the development of various light-tunable optical devices. (c) 2017 Elsevier B.V. All rights reserved.

Keyword :

Aggregation kinematics Light scattering FDTD simulation Incident wavelength Ferrofluids

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GB/T 7714 Jin, Jingyu , Song, Dongxing , Geng, Jiafeng et al. Time-dependent scattering of incident light of various wavelengths in ferrofluids under external magnetic field [J]. | JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS , 2018 , 447 : 124-133 .
MLA Jin, Jingyu et al. "Time-dependent scattering of incident light of various wavelengths in ferrofluids under external magnetic field" . | JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 447 (2018) : 124-133 .
APA Jin, Jingyu , Song, Dongxing , Geng, Jiafeng , Jing, Dengwei . Time-dependent scattering of incident light of various wavelengths in ferrofluids under external magnetic field . | JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS , 2018 , 447 , 124-133 .
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Photothermocatalytic Hydrogen Evolution over Ni2P/TiO2 for Full Spectrum Solar Energy Conversion EI SCIE Scopus
期刊论文 | 2018 , 57 (23) , 7846-7854 | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
WoS CC Cited Count: 1 SCOPUS Cited Count: 1
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For photocatalytic solar energy conversion, the critical challenge is to enhance the solar utilization efficiency. Many efforts have focused on the development of broad-band response nanomaterials. Here, we propose an alternative approach wherein, over Ni2P/TiO2 nanoparticles without noble metal, the UV-vis part of solar energy was absorbed and converted by a semiconductor and its infrared part was separately collected and converted into thermal energy to heat the photocatalytic reaction to a certain temperature. The photothermocatalytic hydrogen activity was 3.6 times that of the sum of the photocatalytic and thermocatalytic reactions. The in situ generated oxygen vacancies in Ni2P/TiO2 during the photothermocatalytic reaction were found to be responsible for the enhanced activity. Moreover, the photocurrent transient response results revealed the faster transfer of electrons from TiO2 to Ni2P at higher temperature which is vital for the significantly enhanced photothermocatalytic hydrogen production. The long-term test also shows the stability of the proposed reaction system.

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GB/T 7714 Song, Rui , Luo, Bing , Geng, Jiafeng et al. Photothermocatalytic Hydrogen Evolution over Ni2P/TiO2 for Full Spectrum Solar Energy Conversion [J]. | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH , 2018 , 57 (23) : 7846-7854 .
MLA Song, Rui et al. "Photothermocatalytic Hydrogen Evolution over Ni2P/TiO2 for Full Spectrum Solar Energy Conversion" . | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 57 . 23 (2018) : 7846-7854 .
APA Song, Rui , Luo, Bing , Geng, Jiafeng , Song, Dongxing , Jing, Dengwei . Photothermocatalytic Hydrogen Evolution over Ni2P/TiO2 for Full Spectrum Solar Energy Conversion . | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH , 2018 , 57 (23) , 7846-7854 .
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