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Low temperature solution-derived TiO2-SnO2 bilayered electron transport layer for high performance perovskite solar cells EI Scopus
期刊论文 | 2019 , 464 , 700-707 | Applied Surface Science
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Abstract :

Planar lead halide perovskite solar cells have shown a promising application in the field of printable solar cells. However, high-performance planar perovskite solar cells typically need a high-temperature process to achieve crystallized titanium oxide films as the electron transport layers, which hinders their application in flexible plastic substrates. Here, we demonstrate a bilayered TiO2-SnO2 film as an excellent substitute for electron transport layer using a low temperature liquid phase method. The bilayered TiO2-SnO2 film exhibits efficient electron extraction and hole blocking ability even at a low processing temperature of 150 °C. The as-obtained solar cells exhibit a champion power conversion efficiency of 18.85% (Voc = 1.100 V, Jsc = 22.52 mA cm−2 and FF = 0.761) under one sun illumination, which is much higher than the devices based on individual SnO2 or TiO2 electron transport layers. The higher electron extraction driving force at the SnO2/perovskite interface and the stronger hole blocking ability due to the defect-free physical contact at the TiO2/FTO interface are suggested to be the main reasons for the improved device performance. © 2018 Elsevier B.V.

Keyword :

Electron transport layers Flexible plastic substrates High temperature process Low processing temperature Low temperature solutions Low temperatures Power conversion efficiencies TiO2-SnO2

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GB/T 7714 Xie, Haixia , Yin, Xingtian , Liu, Jie et al. Low temperature solution-derived TiO2-SnO2 bilayered electron transport layer for high performance perovskite solar cells [J]. | Applied Surface Science , 2019 , 464 : 700-707 .
MLA Xie, Haixia et al. "Low temperature solution-derived TiO2-SnO2 bilayered electron transport layer for high performance perovskite solar cells" . | Applied Surface Science 464 (2019) : 700-707 .
APA Xie, Haixia , Yin, Xingtian , Liu, Jie , Guo, Yuxiao , Chen, Peng , Que, Wenxiu et al. Low temperature solution-derived TiO2-SnO2 bilayered electron transport layer for high performance perovskite solar cells . | Applied Surface Science , 2019 , 464 , 700-707 .
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Heavy metal waste treatment product as semiconductor: Efficient visible light photocatalytic activity of the Bismuth(III) chelates EI Scopus
期刊论文 | 2019 , 774 , 75-81 | Journal of Alloys and Compounds
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Abstract :

Trithiocyanuric acid trisodium salt hydrate (Na3TMT) has been proved an excellent heavy metal chelating agent and widely applied for heavy metal ions elimination in industrial wastewater. In this work, the chelating products of Bismuth(III) ion with this effective agent were prepared by solid state and liquid phase reactions, and proved as a new kind of n-type semiconductor. For full utilization of resource, the green and low-cost massive Bismuth chelate with good crystallinity, distinctive morphology, appropriate band structure and high stability was applied for photoelectrochemical application and photocatalytic organic pollutants degradation upon visible light. Results indicated that [rad]OH radicals were the main reactive specie in the photodegradation process. The combination of heavy metals and organic contaminants removal was achieved by a waste-to-wealth route. © 2018 Elsevier B.V.

Keyword :

Heavy metal chelating agents Heavy metal removal Industrial wastewaters Liquid-phase reaction Photoelectrochemical applications Trithiocyanuric acid Utilization of resources Visible light photocatalytic activity

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GB/T 7714 Guo, Yuxiao , Yang, Yawei , Yin, Xingtian et al. Heavy metal waste treatment product as semiconductor: Efficient visible light photocatalytic activity of the Bismuth(III) chelates [J]. | Journal of Alloys and Compounds , 2019 , 774 : 75-81 .
MLA Guo, Yuxiao et al. "Heavy metal waste treatment product as semiconductor: Efficient visible light photocatalytic activity of the Bismuth(III) chelates" . | Journal of Alloys and Compounds 774 (2019) : 75-81 .
APA Guo, Yuxiao , Yang, Yawei , Yin, Xingtian , Zhao, Jianqiu , Han, Yan , Liu, Jie et al. Heavy metal waste treatment product as semiconductor: Efficient visible light photocatalytic activity of the Bismuth(III) chelates . | Journal of Alloys and Compounds , 2019 , 774 , 75-81 .
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Polar domain structural evolution under electric field and temperature in the (Bi0.5Na0.5)TiO3-0.06BaTiO3 piezoceramics EI Scopus
期刊论文 | 2019 , 102 (1) , 437-447 | Journal of the American Ceramic Society
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Abstract :

Lead-free bismuth sodium titanate and related compounds are of great interest as promising candidates for piezoelectric applications. However, the full understanding of this family of materials is still a challenge partly because of their structural complexity and different behaviors with or without the application of an external electric field. Here, piezoresponse force microscopy is used to gain insight into the mesoscopic-scale domain structure of the morphotropic phase boundary (MPB) composition of (1-x)Bi0.5Na0.5TiO3-xBaTiO3 solid solution at x = 0.06 (abbreviated as BNT-6BT). The evolution of the domains with the changes of the electric field and temperature has been thoroughly examined in conjunction with the crystal structure analysis and dielectric studies. It is found that ferroelectric domains with size of hundreds of nanometers are embedded in a relaxor state without visible domains on a mesoscopic scale, which are considered to contribute to the tetragonal and cubic phases in the material, respectively. Temperature-independent domain configuration is observed in the unpoled sample from room temperature to 200°C. While, temperature-dependent domain configuration is observed in the poled sample. The homogenously poled state breaks into the mixed domain configuration containing polydomain structure and invisible state around the so-called depoling temperature. The structural changes on different length scales are also discussed. This work provides an in-depth understanding of the structural and domain changes under an electric field and the temperature-dependent domain evolution in both unpoled and poled states in the BNT-BT solid solution of the MPB composition. © 2018 The American Ceramic Society

Keyword :

Bismuth sodium titanate Crystal structure analysis Electric field and temperatures External electric field Lead free ceramics Morphotropic phase boundaries Piezoresponse force microscopy Temperature independents

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GB/T 7714 Zhao, Jinyan , Zhang, Nan , Ren, Wei et al. Polar domain structural evolution under electric field and temperature in the (Bi0.5Na0.5)TiO3-0.06BaTiO3 piezoceramics [J]. | Journal of the American Ceramic Society , 2019 , 102 (1) : 437-447 .
MLA Zhao, Jinyan et al. "Polar domain structural evolution under electric field and temperature in the (Bi0.5Na0.5)TiO3-0.06BaTiO3 piezoceramics" . | Journal of the American Ceramic Society 102 . 1 (2019) : 437-447 .
APA Zhao, Jinyan , Zhang, Nan , Ren, Wei , Niu, Gang , Walker, David , Thomas, Pamela A. et al. Polar domain structural evolution under electric field and temperature in the (Bi0.5Na0.5)TiO3-0.06BaTiO3 piezoceramics . | Journal of the American Ceramic Society , 2019 , 102 (1) , 437-447 .
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High electric field-induced strain with ultra-low hysteresis and giant electrostrictive coefficient in barium strontium titanate lead-free ferroelectrics EI Scopus
期刊论文 | 2019 , 39 (2-3) , 295-304 | Journal of the European Ceramic Society
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Abstract :

Ferroelectrics with high electrostrictive properties are of great interest in fundamental researches and industrial applications. In this work, the phase structural evolution, dielectric properties as well as electrostrictive properties in barium strontium titanate [(Ba1-xSrx)TiO3, BST] lead-free ferroelectrics with x from 0.05 to 0.4 were investigated in details. High electric field-induced strain (∼0.2%) at 60 kV/cm are obtained in x = 0.05 and 0.1 compositions. More importantly, almost purely positive strains with ultra-low hysteresis (<8%) determined from bipolar strain-electric field curves are observed in compositions with x from 0.05 to 0.3, suggesting the dominating role of electrostrictive effect. Temperature-insensitive and composition-insensitive longitudinal electrostrictive coefficient Q33 for BST ceramics with giant values from 0.0409 m4/C2 to 0.0479 m4/C2 is identified. These features suggest that BST ceramics not only possess high electric field-induced strain with ultra-low hysteresis and giant Q33, but also are good candidates for potential application in high-precision actuator devices. © 2018 Elsevier Ltd

Keyword :

Electric field curves Electric-field-induced strain Electrostrictive coefficients Electrostrictive effects Fundamental research Lead-Free Lead-free ferroelectrics Temperature-insensitive

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GB/T 7714 Jin, Li , Luo, Wenting , Hou, Lei et al. High electric field-induced strain with ultra-low hysteresis and giant electrostrictive coefficient in barium strontium titanate lead-free ferroelectrics [J]. | Journal of the European Ceramic Society , 2019 , 39 (2-3) : 295-304 .
MLA Jin, Li et al. "High electric field-induced strain with ultra-low hysteresis and giant electrostrictive coefficient in barium strontium titanate lead-free ferroelectrics" . | Journal of the European Ceramic Society 39 . 2-3 (2019) : 295-304 .
APA Jin, Li , Luo, Wenting , Hou, Lei , Tian, Ye , Hu, Qingyuan , Wang, Liang et al. High electric field-induced strain with ultra-low hysteresis and giant electrostrictive coefficient in barium strontium titanate lead-free ferroelectrics . | Journal of the European Ceramic Society , 2019 , 39 (2-3) , 295-304 .
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High thermal stability of electric field-induced strain in (1?x)(Bi0.5Na0.5)TiO3-xBa0.85Ca0.15Ti0.9Zr0.1O3 lead-free ferroelectrics EI Scopus
期刊论文 | 2019 , 39 (2-3) , 277-286 | Journal of the European Ceramic Society
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Abstract :

In ferroelectric materials high electric field-induced strain (EFIS) with good thermal stability is of much interest from both fundamental research and potential applications. Here we propose a strategy to achieve high thermally stable EFIS based on electrostrictive effect and thermal stability of polarization. According to this strategy, we synthesized (1−x)(Bi0.5Na0.5)TiO3-xBa0.85Ca0.15Ti0.9Zr0.1O3 (BNT-xBCZT) ferroelectric ceramics in order to tailor the thermal stability of dielectric permittivity, polarization and EFIS. A dielectric platform with a wide temperature region is induced by increasing x from 0.24 to 0.36 gradually. From 30 °C to 150 °C, a variation of 20% polarization results in a change of 36% EFIS, suggesting a good thermal stability as expect. Temperature-insensitive electrostrictive coefficient Q33 ranges from 0.0264 m4/C2 to 0.0314 m4/C2. These results not only prove the effectiveness of this strategy, but also suggest that this strategy can be applied to other ferroelectric materials to improve the thermal stability. © 2018 Elsevier Ltd

Keyword :

BCZT Dielectric permittivities Electric-field-induced strain Electrostrictive coefficients Electrostrictive effects High thermal stability Lead-free ferroelectrics Temperature-insensitive

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GB/T 7714 Jin, Li , Luo, Wenting , Wang, Liang et al. High thermal stability of electric field-induced strain in (1?x)(Bi0.5Na0.5)TiO3-xBa0.85Ca0.15Ti0.9Zr0.1O3 lead-free ferroelectrics [J]. | Journal of the European Ceramic Society , 2019 , 39 (2-3) : 277-286 .
MLA Jin, Li et al. "High thermal stability of electric field-induced strain in (1?x)(Bi0.5Na0.5)TiO3-xBa0.85Ca0.15Ti0.9Zr0.1O3 lead-free ferroelectrics" . | Journal of the European Ceramic Society 39 . 2-3 (2019) : 277-286 .
APA Jin, Li , Luo, Wenting , Wang, Liang , Tian, Ye , Hu, Qingyuan , Hou, Lei et al. High thermal stability of electric field-induced strain in (1?x)(Bi0.5Na0.5)TiO3-xBa0.85Ca0.15Ti0.9Zr0.1O3 lead-free ferroelectrics . | Journal of the European Ceramic Society , 2019 , 39 (2-3) , 277-286 .
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Reduced graphene oxide supporting Ag meso-flowers and phenyl-modified graphitic carbon nitride as self-cleaning flexible SERS membrane for molecular trace-detection EI Scopus
期刊论文 | 2019 , 560 , 9-19 | Colloids and Surfaces A: Physicochemical and Engineering Aspects
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Abstract :

There is an imperious demand on developing of self-cleaning surface enhanced Raman scattering (SERS) substrates, for eliminating traditional single-use substrates. Herein, ternary flexible membranes of reduced graphene oxide (r-GO) supporting Ag meso-flowers (Ag-MFs) and phenyl-modified graphitic carbon nitride nanosheets (PCNs) were fabricated for photocatalysis-driven self-cleaning SERS detection. In-situ growth of Ag-MFs with tunable morphology (such as coral-like, urchin-like, highly-branched, etc.) on r-GO surfaces provide abundant options for optimizing SERS detection limit, and thus, these PCNs/Ag-MFs@r-GO membranes exhibited strong SERS activity attributed to high density of intraparticle “hotspot” in Ag-MFs and preconcentration ability to probe molecules via π-π stacking. Among these membranes, the optimum PCNs/Ag-MFs@r-GO membrane shown a detection limit of 10−15 M for rhodamine 6G (R6G) molecules, and this membrane could effectively remove probe molecules due to the excellent photocatalytic activity. We used R6G or methylene blue (MB) molecules for investigating the self-cleaning repeatability and stability of this PCNs/Ag-MFs@r-GO membrane, and the signal intensity for SERS detection maintained a high degree of 95% after five cycle-runs. Besides, this PCNs/Ag-MFs@r-GO membrane can be used as a high-efficiency filter membrane for simultaneous detection and purification in wastewater treatment (10 mg/mL imidacloprid solution as the example). © 2018 Elsevier B.V.

Keyword :

Excellent photocatalytic activities Graphitic carbon nitrides High efficiency filter Molecular detection Reduced graphene oxides Self cleaning SERS Simultaneous detection

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GB/T 7714 Qiu, Hengwei , Guo, Jun , Wang, Minqiang et al. Reduced graphene oxide supporting Ag meso-flowers and phenyl-modified graphitic carbon nitride as self-cleaning flexible SERS membrane for molecular trace-detection [J]. | Colloids and Surfaces A: Physicochemical and Engineering Aspects , 2019 , 560 : 9-19 .
MLA Qiu, Hengwei et al. "Reduced graphene oxide supporting Ag meso-flowers and phenyl-modified graphitic carbon nitride as self-cleaning flexible SERS membrane for molecular trace-detection" . | Colloids and Surfaces A: Physicochemical and Engineering Aspects 560 (2019) : 9-19 .
APA Qiu, Hengwei , Guo, Jun , Wang, Minqiang , Ji, Shangdong , Cao, Minghui , Padhiar, Muhammad Amin et al. Reduced graphene oxide supporting Ag meso-flowers and phenyl-modified graphitic carbon nitride as self-cleaning flexible SERS membrane for molecular trace-detection . | Colloids and Surfaces A: Physicochemical and Engineering Aspects , 2019 , 560 , 9-19 .
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Giant resistive switching in mixed phase BiFeO3via phase population control. EI PubMed Scopus
期刊论文 | 2018 , 10 (37) , 17629-17637 | Nanoscale
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Abstract :

Highly-strained coherent interfaces, between rhombohedral-like (R) and tetragonal-like (T) phases in BiFeO3 thin films, often show enhanced electrical conductivity in comparison to non-interfacial regions. In principle, changing the population and distribution of these interfaces should therefore allow different resistance states to be created. However, doing this controllably has been challenging to date. Here, we show that local thin film phase microstructures (and hence R-T interface densities) can be changed in a thermodynamically predictable way (predictions made using atomistic simulations) by applying different combinations of mechanical stress and electric field. We use both pressure and electric field to reversibly generate metastable changes in microstructure that result in very large changes of resistance of up to 108%, comparable to those seen in Tunnelling Electro-Resistance (TER) devices.

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GB/T 7714 Edwards David , Browne Niall , Holsgrove Kristina M et al. Giant resistive switching in mixed phase BiFeO3via phase population control. [J]. | Nanoscale , 2018 , 10 (37) : 17629-17637 .
MLA Edwards David et al. "Giant resistive switching in mixed phase BiFeO3via phase population control." . | Nanoscale 10 . 37 (2018) : 17629-17637 .
APA Edwards David , Browne Niall , Holsgrove Kristina M , Naden Aaron B , Sayedghaee Sayed O , Xu Bin et al. Giant resistive switching in mixed phase BiFeO3via phase population control. . | Nanoscale , 2018 , 10 (37) , 17629-17637 .
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Novel Competitive Chemiluminescence DNA Assay Based on Fe3O4@SiO2@Au-Functionalized Magnetic Nanoparticles for Sensitive Detection of p53 Tumor Suppressor Gene. EI PubMed Scopus
期刊论文 | 2018 | Applied biochemistry and biotechnology
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Abstract :

A simple, rapid response time and ultrahigh sensitive chemiluminescence (CL) DNA assay based on Fe3O4@SiO2@Au-functionalized magnetic nanoparticles (Au-MNPs) was developed for detection of p53 tumor suppressor gene. In this study, 2',6'-dimethylcarbonylphenyl-10-sulfopropyl acridinium-9-carboxylate 4'-NHS ester (NSP-DMAE-NHS), as a new kind of highly efficient luminescence reagent, was immobilized on the complementary sequence of the wild-type p53 (ssDNA) to improve the detection sensitivity. The optimal concentration of ssDNA-(NSP-DMAE-NHS) conjugates mixed with the wild-type p53 (wtp53) samples respectively. Then, the wtp53-Au-MNPs conjugates were added to continue the competitive reaction in the above solution. Subsequently, the Au-MNPs separated under magnetic field, measured by a homemade luminescent measurement system. Under optimal conditions, the method exhibited ultrasensitive sensitivity with a detection limit of 0.001 ng mL<sup>-1</sup> (0.16 pM), a wide range of liner response from 0.001 ng mL<sup>-1</sup>~6.6 μg mL<sup>-1</sup>. Therefore, the immunomagnetic nanocomposites-based detection strategy was rapid, low-cost, and highly sensitive that can be easily extended to the early diagnosis of cancer development and monitoring of patient therapy.

Keyword :

Fe3O4@SiO2@Au magnetic nanoparticles (Au-MNPs) Chemiluminescence DNA assay Wild-type p53·NSP-DMAE-NHS

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GB/T 7714 Wang Linyu , Yao Manwen , Fang Xiangyi et al. Novel Competitive Chemiluminescence DNA Assay Based on Fe3O4@SiO2@Au-Functionalized Magnetic Nanoparticles for Sensitive Detection of p53 Tumor Suppressor Gene. [J]. | Applied biochemistry and biotechnology , 2018 .
MLA Wang Linyu et al. "Novel Competitive Chemiluminescence DNA Assay Based on Fe3O4@SiO2@Au-Functionalized Magnetic Nanoparticles for Sensitive Detection of p53 Tumor Suppressor Gene." . | Applied biochemistry and biotechnology (2018) .
APA Wang Linyu , Yao Manwen , Fang Xiangyi , Yao Xi . Novel Competitive Chemiluminescence DNA Assay Based on Fe3O4@SiO2@Au-Functionalized Magnetic Nanoparticles for Sensitive Detection of p53 Tumor Suppressor Gene. . | Applied biochemistry and biotechnology , 2018 .
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Fabrication and Characterization of High-Frequency Ultrasound Transducers Based on Lead-Free BNT-BT Tape-Casting Thick Film. EI PubMed Scopus
期刊论文 | 2018 , 18 (9) | Sensors
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Abstract :

A lead-free 0.94(Na0.5Bi0.5) TiO₃-0.06 BaTiO₃ (BNT-BT) thick film, with a thickness of 60 μm, has been fabricated using a tape-casting method. The longitudinal piezoelectric constant, clamped dielectric permittivity constant, remnant polarization and coercive field of the BNT-BT thick film were measured to be 150 pC/N, 1928, 13.6 μC/cm², and 33.6 kV/cm, respectively. The electromechanical coupling coefficient <i>kt</i> was calculated to be 0.55 according to the measured electrical impedance spectrum. A high-frequency plane ultrasound transducer was successfully fabricated using a BNT-BT thick film. The performance of the transducer was characterized and evaluated by the pulse-echo testing and wire phantom imaging operations. The BNT-BT thick film transducer exhibits a center frequency of 34 MHz, a -6 dB bandwidth of 26%, an axial resolution of 77 μm and a lateral resolution of 484 μm. The results suggest that lead-free BNT-BT thick film fabricated by tape-casting method is a promising lead-free candidate for high-frequency ultrasonic transducer applications.

Keyword :

lead-free BNT-BT thick film tape-casting method high-frequency ultrasound transducer pulse-echo method

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GB/T 7714 Zhang Junshan , Ren Wei , Liu Yantao et al. Fabrication and Characterization of High-Frequency Ultrasound Transducers Based on Lead-Free BNT-BT Tape-Casting Thick Film. [J]. | Sensors , 2018 , 18 (9) .
MLA Zhang Junshan et al. "Fabrication and Characterization of High-Frequency Ultrasound Transducers Based on Lead-Free BNT-BT Tape-Casting Thick Film." . | Sensors 18 . 9 (2018) .
APA Zhang Junshan , Ren Wei , Liu Yantao , Wu Xiaoqing , Fei Chunlong , Quan Yi et al. Fabrication and Characterization of High-Frequency Ultrasound Transducers Based on Lead-Free BNT-BT Tape-Casting Thick Film. . | Sensors , 2018 , 18 (9) .
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Synthesis, Structure, and Properties of the PbZrO3-PbTiO3-Bi(Zn2/3Nb1/3)O3 Ternary Solid Solution System Around the Morphotropic Phase Boundary EI Scopus
期刊论文 | 2018 , 215 (20) | Physica Status Solidi (A) Applications and Materials Science
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PbZrO3-PbTiO3-Bi(Zn2/3Nb1/3)O3 ternary solid solution system with various compositions is synthesized in the form of ceramics by solid-state reaction method. Their crystal structure and electric properties are investigated by X-ray diffraction, dielectric spectroscopy, ferroelectric and piezoelectric measurements. Studies are mainly focused on two series of compounds 0.95[(1−x)PbZrO3-xPbTiO3]-0.05Bi(Zn2/3Nb1/3)O3 and 0.90[(1−x)PbZrO3-xPbTiO3]-0.10Bi(Zn2/3Nb1/3)O3, which have their compositions across the morphotropic phase boundary (MPB). It is found that the addition of Bi(Zn2/3Nb1/3)O3 broadens the MPB region of the well-known lead zirconate titanate (PZT) binary system and leads to a gradually curved MPB line in the pseudobinary phase diagram and a gradually decreased Curie temperature in these two systems. Enhanced remnant polarization, coercive field, and electromechanical properties are found in the ternary solid solution system compared with pure PZT ceramics. © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim

Keyword :

Complex perovskites Electromechanical property Morphotropic phase boundaries Piezoelectric measurements Pseudo-binaries Remnant polarizations Solid state reaction method Ternary solid solutions

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GB/T 7714 Liu, Zenghui , Gao, Pan , Wu, Hua et al. Synthesis, Structure, and Properties of the PbZrO3-PbTiO3-Bi(Zn2/3Nb1/3)O3 Ternary Solid Solution System Around the Morphotropic Phase Boundary [J]. | Physica Status Solidi (A) Applications and Materials Science , 2018 , 215 (20) .
MLA Liu, Zenghui et al. "Synthesis, Structure, and Properties of the PbZrO3-PbTiO3-Bi(Zn2/3Nb1/3)O3 Ternary Solid Solution System Around the Morphotropic Phase Boundary" . | Physica Status Solidi (A) Applications and Materials Science 215 . 20 (2018) .
APA Liu, Zenghui , Gao, Pan , Wu, Hua , Ren, Wei , Ye, Zuo-Guang . Synthesis, Structure, and Properties of the PbZrO3-PbTiO3-Bi(Zn2/3Nb1/3)O3 Ternary Solid Solution System Around the Morphotropic Phase Boundary . | Physica Status Solidi (A) Applications and Materials Science , 2018 , 215 (20) .
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