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Efficient inactivation of the contamination with pathogenic microorganisms by a combination of water spray and plasma-activated air EI SCIE Scopus
期刊论文 | 2023 , 446 | JOURNAL OF HAZARDOUS MATERIALS
SCOPUS Cited Count: 2
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Abstract :

The global pandemic caused by SARS-CoV-2 has lasted two and a half years and the infections caused by the viral contamination are still occurring. Developing efficient disinfection technology is crucial for the current epidemic or infectious diseases caused by other pathogenic microorganisms. Gas plasma can efficiently inactivate different microorganisms, therefore, in this study, a combination of water spray and plasma-activated air was established for the disinfection of pathogenic microorganisms. The combined treatment efficiently inactivated the Omicron-pseudovirus through caused the nitration modification of the spike proteins and also the pathogenic bacteria. The combined treatment was improved with a funnel-shaped nozzle to form a temporary relatively sealed environ-ment for the treatment of the contaminated area. The improved device could efficiently inactivate the Omicron-pseudovirus and bacteria on the surface of different materials including quartz, metal, leather, plastic, and cardboard and the particle size of the water spray did not affect the inactivation effects. This study supplied a disinfection strategy based on plasma-activated air for the inactivation of contaminated pathogenic microorganisms.

Keyword :

Bactericidal effects Nitration modification Plasma-activated air (PAA) Reactive species SARS-CoV-2 Omicron variant

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GB/T 7714 Guo, Li , Zhao, Pengyu , Jia, Yikang et al. Efficient inactivation of the contamination with pathogenic microorganisms by a combination of water spray and plasma-activated air [J]. | JOURNAL OF HAZARDOUS MATERIALS , 2023 , 446 .
MLA Guo, Li et al. "Efficient inactivation of the contamination with pathogenic microorganisms by a combination of water spray and plasma-activated air" . | JOURNAL OF HAZARDOUS MATERIALS 446 (2023) .
APA Guo, Li , Zhao, Pengyu , Jia, Yikang , Li, Tianhui , Huang, Lingling , Wang, Zifeng et al. Efficient inactivation of the contamination with pathogenic microorganisms by a combination of water spray and plasma-activated air . | JOURNAL OF HAZARDOUS MATERIALS , 2023 , 446 .
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N2O5 in air discharge plasma: energy-efficient production, maintenance factors and sterilization effects SCIE Scopus
期刊论文 | 2023 , 56 (7) | JOURNAL OF PHYSICS D-APPLIED PHYSICS
SCOPUS Cited Count: 7
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Abstract :

N2O5, a reactive species produced by air discharge plasma, has recently attracted much attention. Due to its high reactivity and solubility, N2O5 is a key molecule in nitrogen fixation processes and exhibits promising prospects in plasma biomedicine. However, thus far, it is not well known how to produce N2O5 efficiently and then maintain its concentration under the action of fast removal reactions. In view of this, N2O5 production by dielectric barrier discharge (DBD) alone and by the combination of DBD and gliding arc discharge is compared in this paper. It is found that the combination method can yield over three times the concentration of N2O5 compared to the single DBD method with the optimum discharge power. Moreover, the concentration of N2O5 in the effluent gas can be maintained once O-3 also exists because O-3 can continually produce N2O5 to compensate for its reduction. Finally, the sterilization effects of both the plasma effluent gas and plasma-activated water have trends similar to the trend of the gaseous N2O5 concentration, implying that N2O5 plays an important role in sterilization. This paper enhances the understanding of N2O5 chemistry in air discharge plasma and provides an effective way to produce and maintain N2O5 for subsequent applications.

Keyword :

energy efficiency N2O5 plasma-activated water plasma effluent gas sterilization effect

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GB/T 7714 Wang, Zifeng , Zhu, Mengying , Liu, Dingxin et al. N2O5 in air discharge plasma: energy-efficient production, maintenance factors and sterilization effects [J]. | JOURNAL OF PHYSICS D-APPLIED PHYSICS , 2023 , 56 (7) .
MLA Wang, Zifeng et al. "N2O5 in air discharge plasma: energy-efficient production, maintenance factors and sterilization effects" . | JOURNAL OF PHYSICS D-APPLIED PHYSICS 56 . 7 (2023) .
APA Wang, Zifeng , Zhu, Mengying , Liu, Dingxin , Liu, Linbo , Wang, Xiangyu , Chen, Jinkun et al. N2O5 in air discharge plasma: energy-efficient production, maintenance factors and sterilization effects . | JOURNAL OF PHYSICS D-APPLIED PHYSICS , 2023 , 56 (7) .
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Gliding arc discharge used for water activation: the production mechanism of aqueous NO and its role in sterilization SCIE Scopus
期刊论文 | 2023 , 56 (3) | JOURNAL OF PHYSICS D-APPLIED PHYSICS
SCOPUS Cited Count: 2
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Abstract :

Gliding arc is a promising plasma technology for water activation due to its high energy efficiency for producing reactive nitrogen species (RNS), which is believed as the key agent for the sustained bactericidal effect of plasma-activated water (PAW). Nitric oxide (NO) is the major product of gliding arc and also widely exists in PAW, but the production mechanism of aqueous NO and its role in sterilization have been little investigated before. In this paper, NO-rich plasma effluent gas is produced by gliding arc discharge and introduced into water to produce PAW. The concentrations of gaseous and aqueous reactive species are detected, which decrease with the increasing air flowrate of the gliding arc. To clarify the contribution of plasma-induced RNS on water activation, the NO + air mixed gas is used to simulate the plasma effluent gas, and the results show that the two gases have similar gaseous composition and aqueous NO yield. Compared with the NO + Ar mixed gas with the same NO proportion, the NO + air mixed gas produces much more aqueous NO, implying that the presence of O-2 significantly enhances the production of aqueous NO. The sterilization experiments demonstrate the key role of aqueous NO in sterilization, but an acidic environment is necessary for aqueous NO to achieve a potent bactericidal effect.

Keyword :

gliding arc discharge nitric oxide plasma-activated water reactive species sterilization

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GB/T 7714 Zhu, Mengying , Wang, Zifeng , Chen, Jinkun et al. Gliding arc discharge used for water activation: the production mechanism of aqueous NO and its role in sterilization [J]. | JOURNAL OF PHYSICS D-APPLIED PHYSICS , 2023 , 56 (3) .
MLA Zhu, Mengying et al. "Gliding arc discharge used for water activation: the production mechanism of aqueous NO and its role in sterilization" . | JOURNAL OF PHYSICS D-APPLIED PHYSICS 56 . 3 (2023) .
APA Zhu, Mengying , Wang, Zifeng , Chen, Jinkun , Liu, Linbo , Xi, Wang , Zhang, Fugao et al. Gliding arc discharge used for water activation: the production mechanism of aqueous NO and its role in sterilization . | JOURNAL OF PHYSICS D-APPLIED PHYSICS , 2023 , 56 (3) .
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Inactivation effects of the mist nebulized with plasma-activated air on Pseudomonas aeruginosa through the simulated respiratory tract SCIE Scopus
期刊论文 | 2023 | PLASMA PROCESSES AND POLYMERS
SCOPUS Cited Count: 4
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Abstract :

Plasma-based technology has been widely applied in the biomedicine, agriculture, and environmental fields. In this study, a new application mode, namely plasma-activated nebulized mist (PANM) was proposed. The saline was nebulized by the plasma-activated air to form a mist, and the inactivation effects on Pseudomonas aeruginosa were analyzed based on the simulated respiratory tract. The PANM through the simulated trachea with different lengths or diameters, and the branched once or twice simulated respiratory tract exhibited effective inactivation effects. The PANM through the combined simulated trachea and pig trachea could also inactivate the bacteria on the inner wall of the pig trachea. This study supplied a potent alternative to antibiotics for the treatment of respiratory tract infections.

Keyword :

arc discharge inactivation plasma-activated nebulized mist (PANM) reactive species

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GB/T 7714 Guo, Li , Niyazi, Gulimire , Huang, Lingling et al. Inactivation effects of the mist nebulized with plasma-activated air on Pseudomonas aeruginosa through the simulated respiratory tract [J]. | PLASMA PROCESSES AND POLYMERS , 2023 .
MLA Guo, Li et al. "Inactivation effects of the mist nebulized with plasma-activated air on Pseudomonas aeruginosa through the simulated respiratory tract" . | PLASMA PROCESSES AND POLYMERS (2023) .
APA Guo, Li , Niyazi, Gulimire , Huang, Lingling , Zhao, Pengyu , Wang, Zifeng , Lin, Jiao et al. Inactivation effects of the mist nebulized with plasma-activated air on Pseudomonas aeruginosa through the simulated respiratory tract . | PLASMA PROCESSES AND POLYMERS , 2023 .
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Theoretical Study on the Degradation Pathways of Unsymmetrical Dimethylhydrazine by Aqueous O-3 SCIE Scopus
期刊论文 | 2023 , 43 (1) , 81-97 | PLASMA CHEMISTRY AND PLASMA PROCESSING
SCOPUS Cited Count: 2
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Abstract :

Air discharge plasma is a potential method for the removal of the toxic rocket propellant unsymmetrical dimethylhydrazine ((CH3)(2)NNH2, UDMH for abbreviation). Combining density functional theory calculation and transition state theory, this paper presents theoretical investigation of the degradation pathways of UDMH under the influence of O-3 in aqueous environment, which is the main reactive species generated by air plasma. The neutral, protonated and deprotonated forms of UDMH are included in our study considering the effect of pH. The results show that the UDMH degradation by O-3 usually initials with the oxygen addition to the N atom, and the reaction positions would change with the pH variation. The main reaction position of neutral and protonated forms of UDMH are the N atom of primary ammonia of UDMH, where UDMH will be converted into N-nitrosodimethylamine and NH2OH through multi-step reactions. For deprotonated UDMH, its main reaction position changes to the N atom of secondary ammonia of UDMH, and it finally decomposes to (CH3)(2)NN and OH with the rate constant of 8.26 x 10(3) M-1 s(-1). The pH value also largely influences the degradation processes, where the rate constants of corresponding reactions would vary by up to 12 orders of magnitude for different forms of UDMH. Based on our calculation, the main byproducts of UDMH degradation and their subsequent degradation pathways are summarized. This work is helpful to lay the theoretical basis of UDMH degradation by plasma ozonation.

Keyword :

Air plasma Chemical kinetics DFT calculation O-3 UDMH

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GB/T 7714 Luo, Santu , Fu, Yuwei , Zhang, Mingyan et al. Theoretical Study on the Degradation Pathways of Unsymmetrical Dimethylhydrazine by Aqueous O-3 [J]. | PLASMA CHEMISTRY AND PLASMA PROCESSING , 2023 , 43 (1) : 81-97 .
MLA Luo, Santu et al. "Theoretical Study on the Degradation Pathways of Unsymmetrical Dimethylhydrazine by Aqueous O-3" . | PLASMA CHEMISTRY AND PLASMA PROCESSING 43 . 1 (2023) : 81-97 .
APA Luo, Santu , Fu, Yuwei , Zhang, Mingyan , Liu, Yifan , Wang, Diankai , Zhang, Jiawei et al. Theoretical Study on the Degradation Pathways of Unsymmetrical Dimethylhydrazine by Aqueous O-3 . | PLASMA CHEMISTRY AND PLASMA PROCESSING , 2023 , 43 (1) , 81-97 .
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Study on the Anticancer Effects of Plasma-Activated Saline Perfusion Based on a Microfluidic System SCIE Scopus
期刊论文 | 2022 , 43 (1) , 99-110 | PLASMA CHEMISTRY AND PLASMA PROCESSING
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Abstract :

As a means of applying cold atmospheric plasma (CAP), plasma-activated solutions have received extensive attention for their excellent anticancer effects. However, previous studies have focused mainly on the local injection of plasma-activated solutions for cancer treatment while ignoring the anticancer effects of intraluminal plasma-activated solution perfusion. In this paper, the anticancer effects of flowing plasma-activated saline (PAS) on human bladder cancer cell lines (J82) were studied in vitro in a microfluidic system. It is noteworthy that flowing PAS can kill cancer cells more efficiently than PAS immersion. Further experimental results show that the anticancer effects of PAS on J82 cells in the microcavity are affected by plasma irradiation time, perfusion time and liquid flow rate. Our research suggests that PAS perfusion therapy can become a controllable alternative therapy pathway in the future clinical treatment of intracavitary tumors.

Keyword :

Cold atmospheric plasma Microfluidic system Perfusion therapy Plasma-activated saline Reactive oxygen species

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GB/T 7714 Zhang, Jishen , Xu, Shengduo , Jing, Xixi et al. Study on the Anticancer Effects of Plasma-Activated Saline Perfusion Based on a Microfluidic System [J]. | PLASMA CHEMISTRY AND PLASMA PROCESSING , 2022 , 43 (1) : 99-110 .
MLA Zhang, Jishen et al. "Study on the Anticancer Effects of Plasma-Activated Saline Perfusion Based on a Microfluidic System" . | PLASMA CHEMISTRY AND PLASMA PROCESSING 43 . 1 (2022) : 99-110 .
APA Zhang, Jishen , Xu, Shengduo , Jing, Xixi , Liu, Dingxin , Zhang, Hao , Wang, Zifeng et al. Study on the Anticancer Effects of Plasma-Activated Saline Perfusion Based on a Microfluidic System . | PLASMA CHEMISTRY AND PLASMA PROCESSING , 2022 , 43 (1) , 99-110 .
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Discharge characteristics of a microsecond pulse power supply driven air plasma jet and its anticancer cell effect EI SCIE Scopus
期刊论文 | 2022 , 29 (1) | PHYSICS OF PLASMAS
SCOPUS Cited Count: 5
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Abstract :

In plasma cancer therapy, atmospheric pressure plasma jets have attracted increasing attention in recent years. In this study, from the point of view of economic costs and portability, we have employed atmospheric air as the working gas in order to investigate the effects of the rate of flow, applied voltage, frequency, and pulse width on the characteristics of discharge. The concentrations of reactive oxygen and nitrogen species (RONS) in a plasma-activated medium (PAM) were characterized in order to explore their chemical activity. In addition, the inactivating effect of tumor cells induced by an air plasma jet was investigated and the corresponding inactivation mechanism is also discussed. The results showed that the discharge intensity was positively correlated with frequency and voltage, and negatively correlated with pulse width. Regarding the gas flow rate, when the air flow rate was 1 standard liter per minute (SLM), the discharge intensity was strongest according to the length of the plume. By summarizing the discharge characteristics and emission spectra under different experimental parameters, the stable treatment conditions producing rich active substances were as follows: a frequency of 6 kHz, a voltage of 14 kV, a gas flow rate of 1 SLM, and a pulse width of 1 mu s. Furthermore, under these stabilized conditions, the air plasma jet produced rich aqueous RONS in a PAM effectively, which killed cells in significant numbers and reduced the cell survival rate. Therefore, this study demonstrates the potential application of an atmospheric PAM for the treatment of tumor cells and promotes a deeper understanding of plasma liquid chemistry.

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GB/T 7714 Peng, Sansan , Qi, Miao , Zhang, Huaiyan et al. Discharge characteristics of a microsecond pulse power supply driven air plasma jet and its anticancer cell effect [J]. | PHYSICS OF PLASMAS , 2022 , 29 (1) .
MLA Peng, Sansan et al. "Discharge characteristics of a microsecond pulse power supply driven air plasma jet and its anticancer cell effect" . | PHYSICS OF PLASMAS 29 . 1 (2022) .
APA Peng, Sansan , Qi, Miao , Zhang, Huaiyan , Zhang, Jin , Liu, Rong , Pang, Bolun et al. Discharge characteristics of a microsecond pulse power supply driven air plasma jet and its anticancer cell effect . | PHYSICS OF PLASMAS , 2022 , 29 (1) .
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Enhancement by Spark Discharge in LIBS Detection of Copper Particle Contamination in Oil-Immersed Transformer EI SCIE Scopus
期刊论文 | 2022 , 29 (5) , 2034-2041 | IEEE TRANSACTIONS ON DIELECTRICS AND ELECTRICAL INSULATION
SCOPUS Cited Count: 2
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Abstract :

The detection of copper particles in transformer oil based on laser-induced breakdown spectroscopy (LIBS) technology has been preliminarily studied, but its limit of detection (LOD) needs to be further strengthened. Therefore, spark-discharge assistant method was used to solve the problem, and its enhancement mechanism has been studied in the research. The study of the correlation between spark-discharge-assisted LIBS (SD-LIBS) spectral intensity and Cu concentration shows that spark discharge has a significant increase in plasma size and spectral intensity; for Cu atomic lines at 324.75 and 327.39 nm, the determination coefficient R-2 between their internal standard correction intensity and Cu concentration is promoted to 0.996 and 0.997, respectively; spark-discharge assistant method improves the LOD of LIBS from 0.775 to 0.112 mu g/g. Due to the great improvement in detection performance, the application prospect of LIBS as fine particles detection method in transformer oil has become practical.

Keyword :

Copper particle enhancement laser-induced breakdown spectroscopy (LIBS) spark discharge

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GB/T 7714 Ye, Zhe , Ke, Wei , Wang, Wanting et al. Enhancement by Spark Discharge in LIBS Detection of Copper Particle Contamination in Oil-Immersed Transformer [J]. | IEEE TRANSACTIONS ON DIELECTRICS AND ELECTRICAL INSULATION , 2022 , 29 (5) : 2034-2041 .
MLA Ye, Zhe et al. "Enhancement by Spark Discharge in LIBS Detection of Copper Particle Contamination in Oil-Immersed Transformer" . | IEEE TRANSACTIONS ON DIELECTRICS AND ELECTRICAL INSULATION 29 . 5 (2022) : 2034-2041 .
APA Ye, Zhe , Ke, Wei , Wang, Wanting , Yuan, Huan , Wang, Xiaonan , Wang, Xiaohua et al. Enhancement by Spark Discharge in LIBS Detection of Copper Particle Contamination in Oil-Immersed Transformer . | IEEE TRANSACTIONS ON DIELECTRICS AND ELECTRICAL INSULATION , 2022 , 29 (5) , 2034-2041 .
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Chemical Kinetics of C5F10O with Reactive center dot OH Radical Induced in AOP in Gaseous and Aqueous Phases SCIE Scopus
期刊论文 | 2022 , 42 (6) , 1265-1278 | PLASMA CHEMISTRY AND PLASMA PROCESSING
SCOPUS Cited Count: 2
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Abstract :

C5F10O-insulated environmental-friendly power equipment has great potential to be used in the near future to reduce greenhouse effect. During maintenance, C5F10O should be supplemented or replaced, and the released gas is promisingly to be removed by advanced oxidation processes, but chemical kinetics of C5F10O with the most reactive and dominant species center dot OH radical in air plasma is still not clear. Therefore, this paper studied the degradation pathways and rate constants of C5F10O + center dot OH in both gaseous and aqueous phases with M06-2X/6-31G* method and transition state theory. A continuum solvation model was also employed to study the influence of solvent on chemical kinetics of C5F10O + center dot OH. The results show that most reactions (except for R7 and R8) in both phases have a similar transition state vibration mode leading to same products but rate constants are different. The rate constants of reactions R5 and S5 are highest in corresponding states, respectively, playing a dominant role in the degradation of C5F10O + center dot OH, but the rate constant of reaction S5 is much lower indicating that AOP treatment for C5F10O in gas phase is more effective. This work lays a theoretical basis for plasma modeling and experimental investigation for C5F10O degradation by advanced oxidation process.

Keyword :

6-31G* C5F10O Chemical kinetics Degradation pathways M06-2X

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GB/T 7714 Fu, Yuwei , Luo, Santu , Li, Xingdi et al. Chemical Kinetics of C5F10O with Reactive center dot OH Radical Induced in AOP in Gaseous and Aqueous Phases [J]. | PLASMA CHEMISTRY AND PLASMA PROCESSING , 2022 , 42 (6) : 1265-1278 .
MLA Fu, Yuwei et al. "Chemical Kinetics of C5F10O with Reactive center dot OH Radical Induced in AOP in Gaseous and Aqueous Phases" . | PLASMA CHEMISTRY AND PLASMA PROCESSING 42 . 6 (2022) : 1265-1278 .
APA Fu, Yuwei , Luo, Santu , Li, Xingdi , Chen, Chi , Wang, Chuang , Zhang, Zaiqin et al. Chemical Kinetics of C5F10O with Reactive center dot OH Radical Induced in AOP in Gaseous and Aqueous Phases . | PLASMA CHEMISTRY AND PLASMA PROCESSING , 2022 , 42 (6) , 1265-1278 .
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Chemical Kinetics of Unsymmetrical Dimethylhydrazine (UDMH) Degradation in Wastewater by center dot OH Radical SCIE Scopus
期刊论文 | 2022 , 42 (2) , 363-375 | PLASMA CHEMISTRY AND PLASMA PROCESSING
SCOPUS Cited Count: 6
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Abstract :

Decontamination of organic pollutants by plasma is a novel advanced oxidation process, in which center dot OH is believed to play a crucial role, and it's potential to be applied in the degradation of wastewater containing unsymmetrical dimethylhydrazine (UDMH). However, the chemical kinetics of UDMH decompose still remain unclear which makes UDMH degradation by plasma a lack of theoretical basis, so the chemical kinetics of UDMH with center dot OH should be studied. In this paper, the decomposition mechanism of UDMH with center dot OH was investigated theoretically based on density functional theory (DFT). The calculation level adopted in this paper is M06-2X/6-31G* method in a solvation model based on solute electron density (SMD). Reaction of UDMH + center dot OH -> (CH3)(2)NNH (UDMHr) + H2O was first studied and compared in both aqueous solution and gaseous phase to reveal the necessity of considering solvent, and the results showed that solvent has non-negligible effect in aqueous reaction mechanism to improve the accuracy of rate constant. Then, six potential reactions were found in UDMH + center dot OH decomposition pathways in aqueous solution and a two-step calculation procedure was adopted to guarantee the accuracy of free energy. Based on the calculated rate constants, UDMHr, (CH3)CH2NNH2, dimethylamino and CH3NNH2 were selected as the precursors of subsequent byproducts of N-nitrosodimethylamine, methylhydrazine, nitromethane, formaldehyde hydrazone and dimethyldiazene. And methanol and hydroxylamine were sorted into critical byproducts of UDMH + center dot OH. The potential transformation pathways of main decomposition byproducts were also summarized. The work is a pilot study for subsequent theoretical plasma modeling and experiments.

Keyword :

Chemical kinetics Decomposition pathway OH Plasma decontamination UDMH

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GB/T 7714 Fu, Yuwei , Luo, Santu , Zhang, Mingyan et al. Chemical Kinetics of Unsymmetrical Dimethylhydrazine (UDMH) Degradation in Wastewater by center dot OH Radical [J]. | PLASMA CHEMISTRY AND PLASMA PROCESSING , 2022 , 42 (2) : 363-375 .
MLA Fu, Yuwei et al. "Chemical Kinetics of Unsymmetrical Dimethylhydrazine (UDMH) Degradation in Wastewater by center dot OH Radical" . | PLASMA CHEMISTRY AND PLASMA PROCESSING 42 . 2 (2022) : 363-375 .
APA Fu, Yuwei , Luo, Santu , Zhang, Mingyan , Liu, Dingxin , Sun, Bowen , Liu, Zhijie et al. Chemical Kinetics of Unsymmetrical Dimethylhydrazine (UDMH) Degradation in Wastewater by center dot OH Radical . | PLASMA CHEMISTRY AND PLASMA PROCESSING , 2022 , 42 (2) , 363-375 .
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