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The impact of surface plasma on the total emission charge from PZST cathode induced by nanosecond electric pulse SCIE
期刊论文 | 2019 , 92 (4) | PRAMANA-JOURNAL OF PHYSICS
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Abstract :

Electron emission from antiferroelectric ( cathode has been investigated. The PZST cathode can maintain a metastable ferroelectric phase by the application of a high-enough field, thus implying three possibly pulse-loading configurations for electron emission measurements. The fact that emission charge is larger than the non-compensated charge indicates that the surface plasma contributes to the total emission charge. Furthermore, , characterising the contribution of surface plasma to the total emission charge, was defined. It was found that the emission charge increases almost linearly with . Our results are of great importance for a better understanding of electron emission in antiferroelectric / ferroelectric cathodes.

Keyword :

metastable ferroelectric Electron emission emission charge surface plasma

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GB/T 7714 Liu, Yang , Xu, Xuezhong , Xu, Zhuo et al. The impact of surface plasma on the total emission charge from PZST cathode induced by nanosecond electric pulse [J]. | PRAMANA-JOURNAL OF PHYSICS , 2019 , 92 (4) .
MLA Liu, Yang et al. "The impact of surface plasma on the total emission charge from PZST cathode induced by nanosecond electric pulse" . | PRAMANA-JOURNAL OF PHYSICS 92 . 4 (2019) .
APA Liu, Yang , Xu, Xuezhong , Xu, Zhuo , Feng, Yujun , Lou, Xiaojie . The impact of surface plasma on the total emission charge from PZST cathode induced by nanosecond electric pulse . | PRAMANA-JOURNAL OF PHYSICS , 2019 , 92 (4) .
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Lead-free A(2)Bi(4)Ti(5)O(18) thin film capacitors (A = Ba and Sr) with large energy storage density, high efficiency, and excellent thermal stability SCIE
期刊论文 | 2019 , 7 (7) , 1888-1895 | JOURNAL OF MATERIALS CHEMISTRY C
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Lead-free thin film capacitors, simultaneously possessing a large energy storage density, ultrahigh efficiency and an extra wide working temperature range, are desirable in applications. In this work, A(2)Bi(4)Ti(5)O(18) (A = Ba and Sr) thin films were successfully deposited onto Pt/Ti/SiO2/Si by chemical solution deposition. A large energy storage density (Ure) of 37.1 and 17.2 J cm(-3) and a high efficiency (Z) of 91.5% and 80.8% were achieved in Ba2Bi4Ti5O18 and Sr2Bi4Ti5O18 thin films, respectively. Moreover, these two thin films show excellent thermal abilities under an extra wide working temperature range from -100 degrees C to 180 degrees C. Additionally, high cycling fatigue endurance with a variation of the energy storage density of less than 3.7% and efficiency less than 2.1% after 2 x 10(8) charge-discharge cycles is obtained for these two thin films. These results indicate that A(2)Bi(4)Ti(5)O(18) thin film capacitors have strong potential applications in equipment in harsh working environments.

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GB/T 7714 Yang, Bingbing , Guo, Mengyao , Tang, Xianwu et al. Lead-free A(2)Bi(4)Ti(5)O(18) thin film capacitors (A = Ba and Sr) with large energy storage density, high efficiency, and excellent thermal stability [J]. | JOURNAL OF MATERIALS CHEMISTRY C , 2019 , 7 (7) : 1888-1895 .
MLA Yang, Bingbing et al. "Lead-free A(2)Bi(4)Ti(5)O(18) thin film capacitors (A = Ba and Sr) with large energy storage density, high efficiency, and excellent thermal stability" . | JOURNAL OF MATERIALS CHEMISTRY C 7 . 7 (2019) : 1888-1895 .
APA Yang, Bingbing , Guo, Mengyao , Tang, Xianwu , Wei, Renhuai , Hu, Ling , Yang, Jie et al. Lead-free A(2)Bi(4)Ti(5)O(18) thin film capacitors (A = Ba and Sr) with large energy storage density, high efficiency, and excellent thermal stability . | JOURNAL OF MATERIALS CHEMISTRY C , 2019 , 7 (7) , 1888-1895 .
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Flexible lead-free oxide film capacitors with ultrahigh energy storage performances in extremely wide operating temperature EI SCIE
期刊论文 | 2019 , 57 , 519-527 | Nano Energy
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Here, large-scaled flexible Ba(Zr0.35Ti0.65)O3 ferroelectric film capacitors not only exhibit ultrahigh energy storage performances but also have excellent mechanical flexibility and ferroelectric fatigue endurance. In ultra-wide temperature range from −100 °C to 200 °C, the flexible Ba(Zr0.35Ti0.65)O3 film capacitors show excellent thermal stability with recoverable energy density (Wrec) of over 65.1 J/cm3 and efficiency (η) of over 72.9%, which presents the highest Wrec obtained up to now not only in flexible polymer film dielectric capacitors but also in the ceramic film capacitors including lead-free and lead-based film capacitors on rigid substrates in this measuring temperature range. All these results demonstrate that the flexible Ba(Zr0.35Ti0.65)O3 film capacitors have huge potential in the applications of flexible electronics operated in cold polar regions, extreme altitudes and outer space, as well as high temperature regions. © 2018 Elsevier Ltd

Keyword :

Ceramic film capacitors Dielectric capacitors Flexible device High temperature Lead-free ferroelectrics Measuring temperature Mechanical flexibility Operating temperature

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GB/T 7714 Liang, Zhongshuai , Ma, Chunrui , Shen, Lvkang et al. Flexible lead-free oxide film capacitors with ultrahigh energy storage performances in extremely wide operating temperature [J]. | Nano Energy , 2019 , 57 : 519-527 .
MLA Liang, Zhongshuai et al. "Flexible lead-free oxide film capacitors with ultrahigh energy storage performances in extremely wide operating temperature" . | Nano Energy 57 (2019) : 519-527 .
APA Liang, Zhongshuai , Ma, Chunrui , Shen, Lvkang , Lu, Lu , Lu, Xiaoli , Lou, Xiaojie et al. Flexible lead-free oxide film capacitors with ultrahigh energy storage performances in extremely wide operating temperature . | Nano Energy , 2019 , 57 , 519-527 .
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Giant negative electrocaloric effect in antiferroelectric PbZrO3 thin films in an ultra-low temperature range SCIE
期刊论文 | 2019 , 7 (3) , 617-621 | JOURNAL OF MATERIALS CHEMISTRY C
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Antiferroelectric thin films have demonstrated an excellent negative electrocaloric effect, and are potential candidates for future refrigeration applications. In this study, the electrocaloric effect of polycrystalline PbZrO3 antiferroelectric thin films, deposited on Pt/Ti/SiO2/Si substrates by a sol-gel method, were studied by an indirect method based on the Maxwell relations. It was found that the PbZrO3 thin film undergoes a phase transition from the antiferroelectric to ferroelectric phase driven by the coupling of electric field and temperature. The antiferroelectric to ferroelectric transition leads to a giant negative electrocaloric effect in the PbZrO3 thin film. It is also found that the phase transition temperature decreases with the increase in the applied electric field. As a result, the giant negative electrocaloric effect of the PbZrO3 thin film could be tuned to room temperature, liquid nitrogen temperature and even down to liquid helium temperature range by applying different magnitudes of external fields. For instance, the maximum electrocaloric temperature change is -6.8 K at 292 K under 500 kV cm(-1), -6.7 K at 229 K under 600 kV cm(-1) and -3.8 K at 138 K under 700 kV cm(-1). Our results expand the working temperature of the electrocaloric materials into the ultra-low temperature range, and open up a new landscape for achieving low temperature cooling using ECE devices.

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GB/T 7714 Guo, Mengyao , Wu, Ming , Gao, Weiwei et al. Giant negative electrocaloric effect in antiferroelectric PbZrO3 thin films in an ultra-low temperature range [J]. | JOURNAL OF MATERIALS CHEMISTRY C , 2019 , 7 (3) : 617-621 .
MLA Guo, Mengyao et al. "Giant negative electrocaloric effect in antiferroelectric PbZrO3 thin films in an ultra-low temperature range" . | JOURNAL OF MATERIALS CHEMISTRY C 7 . 3 (2019) : 617-621 .
APA Guo, Mengyao , Wu, Ming , Gao, Weiwei , Sun, Buwei , Lou, Xiaojie . Giant negative electrocaloric effect in antiferroelectric PbZrO3 thin films in an ultra-low temperature range . | JOURNAL OF MATERIALS CHEMISTRY C , 2019 , 7 (3) , 617-621 .
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Large energy storage properties of lead-free (1-x)(0.72Bi(0.5)Na(0.5)TiO(3)-0.28SrTiO(3))-xBiAlO(3) ceramics at broad temperature range SCIE
期刊论文 | 2019 , 784 , 788-793 | JOURNAL OF ALLOYS AND COMPOUNDS
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(1-x)(0.72Bi(0.5)Na(0.5)TiO(3)-0.28SrTiO(3))-xBiAlO(3) (BNT-ST-xBA) lead-free ceramics were prepared through solid-state sintering methods. The structural, dielectric and energy storage properties of the ceramics were studied in this work. A large energy storage density of BNT-ST-0.01BA ceramics exceeding 1.746J/cm(3) has been obtained. The ceramics exhibit a good thermal stability at the temperature ranging from 20 degrees C to 120 degrees C. In addition, energy storage properties are relatively stable after completing 10000 electrical cycles, which shows promising potential for energy storage devices at a high temperature region. (C) 2019 Published by Elsevier B.V.

Keyword :

Energy storage Ferroelectric Lead-free ceramics

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GB/T 7714 Shi, Peng , Zhu, Linguang , Gao, Weiwei et al. Large energy storage properties of lead-free (1-x)(0.72Bi(0.5)Na(0.5)TiO(3)-0.28SrTiO(3))-xBiAlO(3) ceramics at broad temperature range [J]. | JOURNAL OF ALLOYS AND COMPOUNDS , 2019 , 784 : 788-793 .
MLA Shi, Peng et al. "Large energy storage properties of lead-free (1-x)(0.72Bi(0.5)Na(0.5)TiO(3)-0.28SrTiO(3))-xBiAlO(3) ceramics at broad temperature range" . | JOURNAL OF ALLOYS AND COMPOUNDS 784 (2019) : 788-793 .
APA Shi, Peng , Zhu, Linguang , Gao, Weiwei , Yu, Zhonghai , Lou, Xiaojie , Wang, Xiangjian et al. Large energy storage properties of lead-free (1-x)(0.72Bi(0.5)Na(0.5)TiO(3)-0.28SrTiO(3))-xBiAlO(3) ceramics at broad temperature range . | JOURNAL OF ALLOYS AND COMPOUNDS , 2019 , 784 , 788-793 .
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All-Inorganic Flexible Embedded Thin-Film Capacitors for Dielectric Energy Storage with High Performance. PubMed SCIE
期刊论文 | 2019 , 11 (5) , 5247-5255 | ACS applied materials & interfaces
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As passive components in flexible electronics, the dielectric capacitors for energy storage are facing the challenges of flexibility and capability for integration and miniaturization. In this work, the all-inorganic flexible dielectric film capacitors have been obtained. The flexible capacitors show a desirable recoverable energy density ( Wrec) of 40.6 J/cm<sup>3</sup> and a good energy efficiency (η) of 68.9%. Moreover, they have no obvious deterioration on both the Wrec and η after 10<sup>4</sup> times of mechanical bending cycles or under the bending state with a curvature radius of 4 mm. Besides, the outstanding stability of the capacitors against cycle fatigue over fast 10<sup>6</sup> charge-discharge cycles is demonstrated. Most importantly, they work properly at a wide temperature range from -120 to 150 °C with Wrec > 15 J/cm<sup>3</sup> and η > 70%. These fascinating performances endow the flexible capacitors with huge potential application in the future "microenergy storage" system in flexible electronics.

Keyword :

energy storage wide temperature range flexible all-inorganic embedded capacitors fatigue stability

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GB/T 7714 Liang Zhongshuai , Liu Ming , Shen Lvkang et al. All-Inorganic Flexible Embedded Thin-Film Capacitors for Dielectric Energy Storage with High Performance. [J]. | ACS applied materials & interfaces , 2019 , 11 (5) : 5247-5255 .
MLA Liang Zhongshuai et al. "All-Inorganic Flexible Embedded Thin-Film Capacitors for Dielectric Energy Storage with High Performance." . | ACS applied materials & interfaces 11 . 5 (2019) : 5247-5255 .
APA Liang Zhongshuai , Liu Ming , Shen Lvkang , Lu Lu , Ma Chunrui , Lu Xiaoli et al. All-Inorganic Flexible Embedded Thin-Film Capacitors for Dielectric Energy Storage with High Performance. . | ACS applied materials & interfaces , 2019 , 11 (5) , 5247-5255 .
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Enhanced piezoelectric, electrocaloric and energy storage properties at high temperature in lead-free Bi0.5(Na1-xKx)0.5TiO3 ceramics EI SCIE
期刊论文 | 2019 , 45 (4) , 4274-4282 | Ceramics International
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The piezoelectric, electrocaloric and energy storage properties were systemically investigated in lead-free Bi0.5(Na1-xKx)0.5TiO3 ceramics from room temperature to high temperature region. These ceramics can be poled completely to obtain large piezoelectric coefficient (104–153 pC/N) at low electric field of ~30 kV/cm. The piezoelectric property shows good thermal stability due to high depolarization temperature (Td). For BNKT20, a large low electric field-induced strain of 0.36% is obtained at 120 °C under 50 kV/cm, the corresponding normalized strain coefficient is up to 720 pm/V, which is larger than other BNT-based ceramics at high temperature region. The electrocaloric properties of these ceramics are studied via indirect and direct methods. Large EC value (~1.08 K) in BNKT20 ceramic is obtained at 50 kV/cm using indirect calculation. Above 100 °C, the dielectric energy storage density and efficiency of BNKT20 is still up to ~0.85 J/cm3 and 0.75, respectively. The BNKTx ceramics may become promising candidates in the fields of actuators, electrocaloric cooling and energy storage at high temperature region. © 2018 Elsevier Ltd and Techna Group S.r.l.

Keyword :

Depolarization temperature Electric-field-induced strain Electrocaloric Energy storage properties Lead-Free Piezoelectric Piezoelectric coefficient Piezoelectric property

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GB/T 7714 Wang, Xiangjian , Gao, Hongcheng , Hao, Xihong et al. Enhanced piezoelectric, electrocaloric and energy storage properties at high temperature in lead-free Bi0.5(Na1-xKx)0.5TiO3 ceramics [J]. | Ceramics International , 2019 , 45 (4) : 4274-4282 .
MLA Wang, Xiangjian et al. "Enhanced piezoelectric, electrocaloric and energy storage properties at high temperature in lead-free Bi0.5(Na1-xKx)0.5TiO3 ceramics" . | Ceramics International 45 . 4 (2019) : 4274-4282 .
APA Wang, Xiangjian , Gao, Hongcheng , Hao, Xihong , Lou, Xiaojie . Enhanced piezoelectric, electrocaloric and energy storage properties at high temperature in lead-free Bi0.5(Na1-xKx)0.5TiO3 ceramics . | Ceramics International , 2019 , 45 (4) , 4274-4282 .
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Electroresistance of Pt/BaTiO3/LaNiO3 ferroelectric tunnel junctions and its dependence on BaTiO3 thickness SCIE
期刊论文 | 2019 , 6 (4) | MATERIALS RESEARCH EXPRESS
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Recently, ferroelectric tunnel junctions (FTJs) have attracted considerable attention due to their great potential in next generation non-volatile memories. In this work, we report on thickness-dependent tunneling electroresistance (TER) and corresponding evolution of transport behavior in Pt/BaTiO3/LaNiO3 FTJs with various BaTiO3 thicknesses of 2.0, 3.2, and 4.8 nm. The TER effect is observed in the 3.2 nm-thick Pt/BaTiO3/LaNiO3 tunnel junction and an ON/OFF current ratio of similar to 170 is achieved due to the modulation of barrier height by polarization reversal. When the BaTiO3 is increased to 4.8 nm in thickness, the ferroelectric-modulation of the barrier profile becomes more pronounced and the dominant transport mechanism changes from electron tunneling to thermally-activated thermionic injection. As a result, the OFF state current is significantly reduced due to the suppression of the Fowler-Nordheim tunneling with increased width and height of the BaTiO3 barrier. A greatly improved ON/OFF current ratio of similar to 12 500 is thus achieved in the 4.8 nm-thick Pt/BaTiO3/LaNiO3 FTJ device. These results facilitate deeper understanding of the TER effects from the viewpoint of not only the barrier profile but also the transport mechanism.

Keyword :

ferroelectric memory pulsed laser deposition ferroelectric tunnel junctions resistive switching

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GB/T 7714 Wang, Xi , Wu, Ming , Wei, Fansen et al. Electroresistance of Pt/BaTiO3/LaNiO3 ferroelectric tunnel junctions and its dependence on BaTiO3 thickness [J]. | MATERIALS RESEARCH EXPRESS , 2019 , 6 (4) .
MLA Wang, Xi et al. "Electroresistance of Pt/BaTiO3/LaNiO3 ferroelectric tunnel junctions and its dependence on BaTiO3 thickness" . | MATERIALS RESEARCH EXPRESS 6 . 4 (2019) .
APA Wang, Xi , Wu, Ming , Wei, Fansen , Zhang, Yiteng , Zheng, Chunyan , Lou, Xiaojie et al. Electroresistance of Pt/BaTiO3/LaNiO3 ferroelectric tunnel junctions and its dependence on BaTiO3 thickness . | MATERIALS RESEARCH EXPRESS , 2019 , 6 (4) .
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Tuning the microstructure of BaTiO3@SiO2 core-shell nanoparticles for high energy storage composite ceramics SCIE
期刊论文 | 2019 , 784 , 173-181 | JOURNAL OF ALLOYS AND COMPOUNDS
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Core-shell nanoparticles used as blocks to construct composite ceramics can exhibit high energy storage density, but the effects of original tunable shell thickness on the microstructures and energy storage property of finally sintered bulk ceramics has not been clarified, thus how to achieve the full potential of this technology to improve the energy storage density of ferroelectric-based ceramics remains to be solved. In this study, as precursors to fabricate bulk ceramics, BaTiO3@SiO2 core-shell nanoparticles were successfully synthesized by a wet-chemical method and they were used as models to investigate the effect of the core-shell nanostructured precursors on the energy storage property of the bulk composite ceramics. The original BaTiO3 nanoparticles coated with various homogenous SiO2 shells were acquired by controlling the concentration of tetraethyl orthosilicate (TEOS). The surface microstructure of the bulk composite ceramics observed by scanning electron microscope (SEM) revealed that the SiO2 outer shell of BaTiO3@SiO2 nanoparticles plays an important role in constructing the microstructure of the ceramics. The remodeled microstructure has a great impact on leakage current density and dielectric property, and it makes a leading contribution to the energy storage performance of ceramics. As a result, the optimum SiO2 loading range was confirmed and the maximum energy storage density obtained from BaTiO3@20 wt%SiO2 was similar to 4.799 J/cm(3) at 370 kV/cm, demonstrating that nanoscale core-shell architecture is an effective strategy to improve the energy storage performance of ferroelectric-based composite ceramics. (C) 2019 Elsevier B.V. All rights reserved.

Keyword :

Energy storage Composite ceramics Core-shell structure BaTiO3

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GB/T 7714 Xu, Congcong , Su, Ran , Wang, Zhipeng et al. Tuning the microstructure of BaTiO3@SiO2 core-shell nanoparticles for high energy storage composite ceramics [J]. | JOURNAL OF ALLOYS AND COMPOUNDS , 2019 , 784 : 173-181 .
MLA Xu, Congcong et al. "Tuning the microstructure of BaTiO3@SiO2 core-shell nanoparticles for high energy storage composite ceramics" . | JOURNAL OF ALLOYS AND COMPOUNDS 784 (2019) : 173-181 .
APA Xu, Congcong , Su, Ran , Wang, Zhipeng , Wang, Yuting , Zhang, Dawei , Wang, Jinkai et al. Tuning the microstructure of BaTiO3@SiO2 core-shell nanoparticles for high energy storage composite ceramics . | JOURNAL OF ALLOYS AND COMPOUNDS , 2019 , 784 , 173-181 .
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Thermal strain induced large electrocaloric effect of relaxor thin film on LaNiO3/Pt composite electrode with the coexistence of nanoscale antiferroelectric and ferroelectric phases in a broad temperature range EI SCIE Scopus
期刊论文 | 2018 , 47 , 285-293 | NANO ENERGY
WoS CC Cited Count: 7 SCOPUS Cited Count: 9
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Ferroelectric/antiferroelectric thin/thick films with large electrocaloric (EC) effect in a broad operational temperature range are very attractive in solid-state cooling devices. We demonstrated that a large positive electrocaloric (EC) effect (maximum Delta T similar to 20.7 K) in a broad temperature range (similar to 110 K) was realized in Pb0.97La0.02(Zr0.65Sn0.3Ti0.05)O-3 (PLZST) relaxor antiferroelectric (AFE) thin film prepared using a sol-gel method. The large positive EC effect may be ascribed to the in-plane residual thermal tensile stress during the layer-by-layer annealing process, and the high-quality film structure owing to the utilization of the LaNiO3/Pt composite bottom electrode. The broad EC temperature range may be ascribed to the great dielectric relaxor dispersion around the dielectric peak because of the coexistence of nanoscale multiple FE and AFE phases. Moreover, a large pyroelectric energy density (6.10 Jcm(-3)) was harvested by using an Olsen cycle, which is much larger than those (usually less than 10(-) Jcm(-3)) obtained by using direct thermal-electrical, Stirling and Carnot cycles, etc. These breakthroughs enable the PLZST thin film an attractive multifunctional material for applications in modern solid-state cooling and energy harvesting.

Keyword :

Electrocaloric Antiferroelectric Thin film Sol-gel Relaxor

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GB/T 7714 Peng, Biaolin , Zhang, Qi , Lyu, Yinong et al. Thermal strain induced large electrocaloric effect of relaxor thin film on LaNiO3/Pt composite electrode with the coexistence of nanoscale antiferroelectric and ferroelectric phases in a broad temperature range [J]. | NANO ENERGY , 2018 , 47 : 285-293 .
MLA Peng, Biaolin et al. "Thermal strain induced large electrocaloric effect of relaxor thin film on LaNiO3/Pt composite electrode with the coexistence of nanoscale antiferroelectric and ferroelectric phases in a broad temperature range" . | NANO ENERGY 47 (2018) : 285-293 .
APA Peng, Biaolin , Zhang, Qi , Lyu, Yinong , Liu, Laijun , Lou, Xiaojie , Shaw, Christopher et al. Thermal strain induced large electrocaloric effect of relaxor thin film on LaNiO3/Pt composite electrode with the coexistence of nanoscale antiferroelectric and ferroelectric phases in a broad temperature range . | NANO ENERGY , 2018 , 47 , 285-293 .
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