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Mn-based layered oxide microspheres assembled by ultrathin nanosheets as cathode material for potassium-ion batteries EI Scopus SCIE
期刊论文 | 2019 , 293 , 299-306 | Electrochimica Acta
WoS CC Cited Count: 2 SCOPUS Cited Count: 1
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Abstract :

© 2018 Elsevier Ltd Potassium-ion batteries (KIBs) are regarded as potentially promising large-scale energy storage (EES) systems due to the close redox potential to lithium, the rich reserve and low cost of potassium resources. Nevertheless, the larger ionic radius of K-ion makes cathode materials for KIBs be a difficult issue. Herein, we construct Mn-based layered oxide (K0.32MnO2) microsphere, self-assembled by ultrathin nanosheets, as potential cathode electrode for nonaqueous KIBs, which delivers a reversible discharge capacity of 95.1 mAh·g−1 at 10 mA g−1. It is demonstrated that K0.32MnO2 undergoes a simple solid solution reaction mechanism for K-ions deintercalation/intercalation during the initial charge-discharge process, which is not like complex multiple processes accompanied by phase transition for Mn-based layered oxide particles. Ex situ measurements reveal that K0.32MnO2 nanosheets can provide outstanding morphology and structure stability, as well as fast electrochemical kinetics upon cycling, thus high rate capacity, improved cycling lifetime and voltage stability at low and high rates can be obtained. We also verify the practical feasibility of K-ion full cell with commercial super P carbon black anode. This novel work illuminates the electrochemical mechanism for K-ions storage in depth, which may push the study on layered oxide cathodes and accelerate the development of KIBs.

Keyword :

Cathode material Mn-based layered oxide Nonaqueous electrolyte Potassium-ion battery Solid solution process

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GB/T 7714 Chong, Shaokun , Wu, Yifang , Chen, Yuanzhen et al. Mn-based layered oxide microspheres assembled by ultrathin nanosheets as cathode material for potassium-ion batteries [J]. | Electrochimica Acta , 2019 , 293 : 299-306 .
MLA Chong, Shaokun et al. "Mn-based layered oxide microspheres assembled by ultrathin nanosheets as cathode material for potassium-ion batteries" . | Electrochimica Acta 293 (2019) : 299-306 .
APA Chong, Shaokun , Wu, Yifang , Chen, Yuanzhen , Guo, Shengwu , Tai, Zige , Shu, Chengyong et al. Mn-based layered oxide microspheres assembled by ultrathin nanosheets as cathode material for potassium-ion batteries . | Electrochimica Acta , 2019 , 293 , 299-306 .
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Ultrafine grained dual-phase martensite/ferrite steel strengthened and toughened by lamella structure EI SCIE Scopus
期刊论文 | 2018 , 734 , 311-317 | MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING
WoS CC Cited Count: 2 SCOPUS Cited Count: 2
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Abstract :

Grain refinement is one of the most effective methods for strengthening steels, but grain refinement to 1 pm or less deteriorates the ductility considerably. To evade the strength-ductility trade-off, a lamellar-structured (LS) ultrafine-grained (UFG) dual-phase (DP) ferrite/martensite (F/M) steel was produced by warm rolling an intercritical annealed low-carbon martensite and subsequent air cooling in this paper. The microstructure is similar to a short fiber reinforced composite, and the highest strength (1432 +/- 15 MPa) combined with a decent ductility (16.5 +/- 0.5% elongation) is achieved in DP steel. Compared with conventional equiaxed coarse grained (CG) and UFG DP counterparts, the LS martensite in UFG DP steel can produce extra strengthening effect and is also beneficial to ductility. And the short fiber theory can predict the strength very well.

Keyword :

Dual phases Lamella structure Mechanical properties Steel Ultrafine grained microstructure

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GB/T 7714 Sun, Junjie , Jiang, Tao , Wang, Yingjun et al. Ultrafine grained dual-phase martensite/ferrite steel strengthened and toughened by lamella structure [J]. | MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING , 2018 , 734 : 311-317 .
MLA Sun, Junjie et al. "Ultrafine grained dual-phase martensite/ferrite steel strengthened and toughened by lamella structure" . | MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING 734 (2018) : 311-317 .
APA Sun, Junjie , Jiang, Tao , Wang, Yingjun , Guo, Shengwu , Liu, Yongning . Ultrafine grained dual-phase martensite/ferrite steel strengthened and toughened by lamella structure . | MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING , 2018 , 734 , 311-317 .
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Effect of grain refinement on high-carbon martensite transformation and its mechanical properties EI SCIE Scopus
期刊论文 | 2018 , 726 , 342-349 | MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING
WoS CC Cited Count: 4 SCOPUS Cited Count: 4
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Abstract :

In this paper, the grain size effect on martensite transformation and its mechanical properties were investigated in two high-carbon steels. The results show that grain refinement can induce a phase transformation of high carbon martensite substructure from twin to dislocations. When grains are refined to smaller than 4 mu m, no twin could be observed, instead, full dislocation substructure is obtained. And the martensite substructure transition results in an enhancement in mechanical properties, an ultrahigh tensile strength of 2.28 GPa and a significant elongation of 6.8% are obtained in the 0.61 wt%C steel. A model based on the relationship between dislocation slip stress (tau(S)) and twin shear stress (tau(T)) with grain size (d) is developed to explain the above phase transformation phenomenon. The tau(T) is proportional to d(-1) and tau(S) is proportional to d(-1/2), both of which increase with reducing grain size, but tau(T) is more sensitive to grain size. Therefore, a critical grain size (d(c)) is obtained, at which the stresses for twining and for dislocation gliding are equal, lower than this value (i.e. grain is finer), the stress for twin is higher than that for dislocation gliding, so dislocation slip becomes main deformation process in martensite transformation. The theoretically calculated d(c) is about 2.7-7.6 mu m, which is in good agreement with the experimental results. These findings may provide a new way to design ultra-high strength and high ductility steels.

Keyword :

Martensitic phase transformation High-carbon steel Dislocation structure Twinning Mechanical property

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GB/T 7714 Sun, Junjie , Jiang, Tao , Wang, Yingjun et al. Effect of grain refinement on high-carbon martensite transformation and its mechanical properties [J]. | MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING , 2018 , 726 : 342-349 .
MLA Sun, Junjie et al. "Effect of grain refinement on high-carbon martensite transformation and its mechanical properties" . | MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING 726 (2018) : 342-349 .
APA Sun, Junjie , Jiang, Tao , Wang, Yingjun , Guo, Shengwu , Liu, Yongning . Effect of grain refinement on high-carbon martensite transformation and its mechanical properties . | MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING , 2018 , 726 , 342-349 .
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A low-alloy high-carbon martensite steel with 2.6 GPa tensile strength and good ductility EI SCIE Scopus
期刊论文 | 2018 , 158 , 247-256 | ACTA MATERIALIA
WoS CC Cited Count: 4 SCOPUS Cited Count: 6
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Abstract :

A low-alloy and high-carbon martensite steel (0.66% C) with ultrafine grains is produced by combination of Tempforming (tempering and deforming of a quenched steel) and reheating followed by water quenching and low temperature tempering. The size of prior-austenite grains of the steel is reduced to 2.4 mu m through this new technique, and its ultimate tensile strength of 2.6 GPa and elongation of 7% are obtained, which is the highest strength in low alloy high strength steels. The microstructure of the high carbon martensite consists of high density dislocations, undissolved spherical carbides, and dispersed nano-scale Fe3C and Fe5C2\ phases precipitated at interior of martensitic after tempering. The strengthening mechanisms of the ultrafine grain martensitic steel are mainly dislocation strengthening and precipitation strengthening and also fine grain strengthening. The tensile strength and ductility of the steel are superior to that of existing maraging steels, such as C350, the highest strength in commercialized level, in which more than 20% precious alloy elements such as Co, Mo, Ni, and Ti are contained, and the cost of our materials is only about 1/50 of the C350. All above advantages are desirable for broad industrial applications at an economic cost. (C) 2018 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.

Keyword :

Dislocation substructure Ductility High carbon martensite steel Ultrafine grain Ultrahigh strength

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GB/T 7714 Wang, Yingjun , Sun, Junjie , Jiang, Tao et al. A low-alloy high-carbon martensite steel with 2.6 GPa tensile strength and good ductility [J]. | ACTA MATERIALIA , 2018 , 158 : 247-256 .
MLA Wang, Yingjun et al. "A low-alloy high-carbon martensite steel with 2.6 GPa tensile strength and good ductility" . | ACTA MATERIALIA 158 (2018) : 247-256 .
APA Wang, Yingjun , Sun, Junjie , Jiang, Tao , Sun, Yu , Guo, Shengwu , Liu, Yongning . A low-alloy high-carbon martensite steel with 2.6 GPa tensile strength and good ductility . | ACTA MATERIALIA , 2018 , 158 , 247-256 .
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Cryptomelane-type MnO2/carbon nanotube hybrids as bifunctional electrode material for high capacity potassium-ion full batteries EI SCIE Scopus
期刊论文 | 2018 , 54 , 106-115 | Nano Energy
WoS CC Cited Count: 10 SCOPUS Cited Count: 8
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Abstract :

Potassium-ion batteries (PIBs) have been receiving a great deal of attention owing to abundant and cost-effective potassium resources. However, the key issue is to explore suitable electrode materials for accommodating the large size K-ions reversibly. In this report, K1.06Mn8O16/CNT hybrids are systematically studied for the first time as bifunctional PIBs-electrodes, in which Mn-ions play as the redox center. As the cathode, it exhibits excellent electrochemical kinetics and reversibility, as well as highly structure stability. The cathode displays an unprecedented capacity of 309.4 mA h g−1 at 20 mA g−1 with the energy density of 733.3 Wh kg−1 and outstanding rate performance (187.1 mA h g−1 at 500 mA g−1). In addition, the high capacity of 636.6 mA h g−1 at 20 mA g−1, ultra-long cycling lifespan over 500 cycles and remarkable rate capability can also be acquired when the material was tested as the anode. The extraordinary electrochemical properties are ascribed to the well-developed conductive network and robust microstructure stability. Meanwhile, the symmetrical K-ions full cell exhibits high discharge capacity of 241.0 mA h g−1 at 100 mA g−1. This work reveals the K-ions storage mechanism in cryptomelane bifunctional electrodes in depth and the fundamental understanding help us open up a new direction for PIBs. © 2018 Elsevier Ltd

Keyword :

Bifunctional electrodes Conductive networks Cryptomelane Discharge capacities Electrochemical kinetics High capacity Microstructure stability Potassium ions

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GB/T 7714 Chong, Shaokun , Wu, Yifang , Liu, Chaofeng et al. Cryptomelane-type MnO2/carbon nanotube hybrids as bifunctional electrode material for high capacity potassium-ion full batteries [J]. | Nano Energy , 2018 , 54 : 106-115 .
MLA Chong, Shaokun et al. "Cryptomelane-type MnO2/carbon nanotube hybrids as bifunctional electrode material for high capacity potassium-ion full batteries" . | Nano Energy 54 (2018) : 106-115 .
APA Chong, Shaokun , Wu, Yifang , Liu, Chaofeng , Chen, Yuanzhen , Guo, Shengwu , Liu, Yongning et al. Cryptomelane-type MnO2/carbon nanotube hybrids as bifunctional electrode material for high capacity potassium-ion full batteries . | Nano Energy , 2018 , 54 , 106-115 .
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高能量密度锂离子电池用富锂正极材料 CSCD PKU
期刊论文 | 2017 , (z2) , 27-38 | 化学进展 | IF: 0.82
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Keyword :

层-尖转变 富锂材料 表面包覆 锂离子电池

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GB/T 7714 严武渭 , 柳永宁 , 崇少坤 et al. 高能量密度锂离子电池用富锂正极材料 [J]. | 化学进展 , 2017 , (z2) : 27-38 .
MLA 严武渭 et al. "高能量密度锂离子电池用富锂正极材料" . | 化学进展 z2 (2017) : 27-38 .
APA 严武渭 , 柳永宁 , 崇少坤 , 周亚萍 , 刘建国 , 邹志刚 . 高能量密度锂离子电池用富锂正极材料 . | 化学进展 , 2017 , (z2) , 27-38 .
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A high performance martensitic stainless steel containing 1.5 wt% Si EI SCIE Scopus
期刊论文 | 2017 , 125 , 35-45 | MATERIALS & DESIGN | IF: 4.525
WoS CC Cited Count: 3 SCOPUS Cited Count: 4
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Abstract :

Usually, martensitic precipitation hardening stainless steels (MPHSSs) contain ultralow carbon concentration to ensure its high performance in corrosion resistance, weldability and toughness. Meanwhile, high content of alloy elements (such as Mo, Ni, Ti and Cu) is inevitably added in order to obtain superb strength by precipitation hardening. In this work, a new idea of alloying design in stainless steels has been proposed, in which carbon serves as the main strengthening element and high silicon concentration (1.5 wt%) is used to suppress carbide precipitation and coarsening during tempering. A steel with composition of Fe-0.2C-15Cr-3Ni-1.5Si-1.0Mn has been designed and prepared, and its excellent mechanical performance (ultimate tensile strength of 1680 MPa, total elongation of 16%), pitting corrosion resistance and weldability have been displayed. Moreover only low-cost alloying components and ordinary treatments are needed to obtain those outstanding properties which are comparable to commercialized MPHSSs (such as 17-4 PH, PH13-8 Mo). (C) 2017 Elsevier Ltd. All rights reserved.

Keyword :

Solution strengthening Stainless steel Mechanical property Alloying design

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GB/T 7714 Jiang, Tao , Sun, Junjie , Liu, Hongji et al. A high performance martensitic stainless steel containing 1.5 wt% Si [J]. | MATERIALS & DESIGN , 2017 , 125 : 35-45 .
MLA Jiang, Tao et al. "A high performance martensitic stainless steel containing 1.5 wt% Si" . | MATERIALS & DESIGN 125 (2017) : 35-45 .
APA Jiang, Tao , Sun, Junjie , Liu, Hongji , Wang, Yingjun , Guo, Shengwu , Sun, Yu et al. A high performance martensitic stainless steel containing 1.5 wt% Si . | MATERIALS & DESIGN , 2017 , 125 , 35-45 .
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Two 3D structured Co-Ni bimetallic oxides as cathode catalysts for high-performance alkaline direct methanol fuel cells EI SCIE Scopus
期刊论文 | 2017 , 361 , 160-169 | JOURNAL OF POWER SOURCES | IF: 6.945
WoS CC Cited Count: 6 SCOPUS Cited Count: 7
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Abstract :

Two NiCo2O4 bimetallic oxides were synthesized via a facile hydrothermal method. SEM and TEM observations show that these materials have three-dimensional (3D) dandelion-like (DL) and flower-like (FL) morphologies. Their large specific surface areas (90.68 and 19.8 m(2).g(-1)) and porous structures provide many active sites and effective transport pathways for the oxygen reduction reaction (ORR). Electrochemical measurements with a rotating ring-disc electrode (RRDE) indicate that the electron transfer numbers of the NiCo2O4-DL and NiCo2O4-FL catalysts for ORR in an alkaline solution are 3.97 and 3.91, respectively. Fuel cells were assembled with the bimetallic oxides, PtRu/C and a polymer fiber membrane (PFM) as cathode catalysts, anode catalyst and electrolyte film, respectively. For NiCo2O4-DL, the peak power density reaches up to 73.5 mW.cm(-2) at 26 degrees C, which is the highest room-temperature value reported to date. The high catalytic activity of NiCo2O4 is mainly attributed to the presence of many Co3+ cations that directly donate electrons to O-2 to reduce it via a more efficient and effective route. Furthermore, the catalytic performance of NiCo2O4-DL is superior to that of NiCo2O4-FL because it has a higher specific surface area and is less crystalline. (C) 2017 Elsevier B.V. All rights reserved.

Keyword :

Flower-like NiCo2O4 Hierarchical dandelion-like NiCO2O4 Direct methanol fuel cell Oxygen reduction reaction

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GB/T 7714 Liu, Yan , Shu, Chengyong , Fang, Yuan et al. Two 3D structured Co-Ni bimetallic oxides as cathode catalysts for high-performance alkaline direct methanol fuel cells [J]. | JOURNAL OF POWER SOURCES , 2017 , 361 : 160-169 .
MLA Liu, Yan et al. "Two 3D structured Co-Ni bimetallic oxides as cathode catalysts for high-performance alkaline direct methanol fuel cells" . | JOURNAL OF POWER SOURCES 361 (2017) : 160-169 .
APA Liu, Yan , Shu, Chengyong , Fang, Yuan , Chen, Yuanzhen , Liu, Yongning . Two 3D structured Co-Ni bimetallic oxides as cathode catalysts for high-performance alkaline direct methanol fuel cells . | JOURNAL OF POWER SOURCES , 2017 , 361 , 160-169 .
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Potassium ferrous ferricyanide nanoparticles as a high capacity and ultralong life cathode material for nonaqueous potassium-ion batteries EI SCIE Scopus
期刊论文 | 2017 , 5 (43) , 22465-22471 | JOURNAL OF MATERIALS CHEMISTRY A | IF: 9.931
WoS CC Cited Count: 26 SCOPUS Cited Count: 27
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Abstract :

We propose potassium ferrous ferricyanide (KFeII[Fe-III(CN)(6)]) nano particles with a 3D open framework structure as a cathode for nonaqueous K-ion batteries. Electrochemical reaction mechanism analyses identify that two redox-active sites based on C and N coordinated Fe-II/Fe-III redox couples play a role in K-ion storage, and no phase change occurs in the different states of the initial and second charge-discharge processes. Thus, the (KFeII[Fe-III(CN)(6)] electrode exhibits a high discharge capacity of 118.7 mA h g(-1) at an operating voltage of 3.34 V and extremely excellent cycling stability with a capacity value of 111.3 mA h g(-1) after 100 cycles at 10 mA g(-1). Moreover, an ultralong cycling lifespan of 1000 cycles with a high capacity retention of 80.49% and extraordinary voltage stability at 100 mA g(-1) can be acquired. Ex situ characterizations verify that the outstanding electrochemical performance of (KFeII[Fe-III(CN)(6)] is attributed to superior structural stability and electrochemical reversibility upon long-term cycling. Therefore, the (KFeII[Fe-III(CN)(6)] material can make KlBs competitive in EES applications.

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GB/T 7714 Chong, Shaokun , Chen, Yuanzhen , Zheng, Yang et al. Potassium ferrous ferricyanide nanoparticles as a high capacity and ultralong life cathode material for nonaqueous potassium-ion batteries [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2017 , 5 (43) : 22465-22471 .
MLA Chong, Shaokun et al. "Potassium ferrous ferricyanide nanoparticles as a high capacity and ultralong life cathode material for nonaqueous potassium-ion batteries" . | JOURNAL OF MATERIALS CHEMISTRY A 5 . 43 (2017) : 22465-22471 .
APA Chong, Shaokun , Chen, Yuanzhen , Zheng, Yang , Tan, Qiang , Shu, Chengyong , Liu, Yongning et al. Potassium ferrous ferricyanide nanoparticles as a high capacity and ultralong life cathode material for nonaqueous potassium-ion batteries . | JOURNAL OF MATERIALS CHEMISTRY A , 2017 , 5 (43) , 22465-22471 .
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A strategy of constructing spherical core-shell structure of Li1.2Ni0.2Mn0.O2@Li1.2Ni0.4Mn0.4O2 cathode material for high-performance lithium-ion batteries EI SCIE Scopus
期刊论文 | 2017 , 356 , 153-162 | JOURNAL OF POWER SOURCES | IF: 6.945
WoS CC Cited Count: 23 SCOPUS Cited Count: 24
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Abstract :

Serious decay of capacity and voltage for Li-rich layered cathode materials restrict their commercial application for Li-ion batteries. In this paper, a spherical core-shell structure, Li1.2Ni0.2Mn0.4O2@Li1.2Ni0.4Mn0.4O2 was in-situ prepared using hydrothermal method. SEM images as well as the analysis with XPS and EDS verified that the core-shell structure grows well. Electrochemical properties showed that the merits of the both materials have been preserved for high capacity of core material and high voltage as well as superior cycling stability of shell material. C/S-1/1 sample, whose mass proportion of core to shell is 1:1, exhibits the initial discharge capacity Of 218 mAh.g(-1) with the highest operating voltage of 3.763 Vat 0.1C between 2.0 and 4.8 V, splendid cycling stability with the capacity retention of 93.1% and high voltage retention value of 3.335 V after 100 cycles. The improvement of electrochemical performances are attributed to the stable Li1.2Ni0.4Mn0.4O2 protective shell, which is beneficial to improve the electrochemical kinetics, mitigate the morphology evolution and retard the layered-spinel phase transition by restraining the release of O-2 and weakening the electrode-electrolyte interfacial reaction. (C) 2017 Elsevier B.V. All rights reserved.

Keyword :

Capacity fading Lithium-ion battery Core-shell structure Cathode material Voltage decay

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GB/T 7714 Chong, Shaokun , Wu, Yifang , Chen, Yuanzhen et al. A strategy of constructing spherical core-shell structure of Li1.2Ni0.2Mn0.O2@Li1.2Ni0.4Mn0.4O2 cathode material for high-performance lithium-ion batteries [J]. | JOURNAL OF POWER SOURCES , 2017 , 356 : 153-162 .
MLA Chong, Shaokun et al. "A strategy of constructing spherical core-shell structure of Li1.2Ni0.2Mn0.O2@Li1.2Ni0.4Mn0.4O2 cathode material for high-performance lithium-ion batteries" . | JOURNAL OF POWER SOURCES 356 (2017) : 153-162 .
APA Chong, Shaokun , Wu, Yifang , Chen, Yuanzhen , Shu, Chengyong , Liu, Yongning . A strategy of constructing spherical core-shell structure of Li1.2Ni0.2Mn0.O2@Li1.2Ni0.4Mn0.4O2 cathode material for high-performance lithium-ion batteries . | JOURNAL OF POWER SOURCES , 2017 , 356 , 153-162 .
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