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学者姓名:汪宏

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Ultrahigh discharge efficiency and energy density achieved at low electric fields in sandwich-structured polymer films containing dielectric elastomers SCIE
期刊论文 | 2019 , 7 (8) , 3729-3736 | JOURNAL OF MATERIALS CHEMISTRY A
WoS CC Cited Count: 1
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Abstract :

Dielectric polymer capacitors, especially those capable of operating efficiently at relatively low operating voltages, are urgently needed to meet the growing demands for miniaturization and reliability in advanced electronics and electrical power systems in automobiles and aerospace. However, high-performance energy storage properties are normally obtained in dielectric capacitors under the application of high electric fields. Herein, a series of all-polymer sandwich-structured films comprised of acrylic rubber dielectric elastomers (DE) dispersed in ferroelectric poly(vinylidene fluoride-cohexafluoropropene) as the outer layer and poly(methyl methacrylate) as the middle layer have been fabricated. The maximum electrical displacement, energy density, and discharge efficiency of the sandwiched films have been improved significantly by optimizing the DE content. Notably, a high energy density of 11.8 J cm(-3) along with a very high efficiency of 89% has been achieved in the sandwiched film with 30 wt% DE at an applied field of 300 MV m(-1), which is the best overall property set ever achieved in the representative polymer dielectrics. Excellent power density and great stability of energy storage performance over the bending cycles have been demonstrated in the layered films. All these features offer new opportunities for designing a new class of hierarchically structured dielectric polymers with excellent energy storage capability that can be achieved at relatively low electric fields.

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GB/T 7714 Chen, Jie , Wang, Yifei , Xu, Xinwei et al. Ultrahigh discharge efficiency and energy density achieved at low electric fields in sandwich-structured polymer films containing dielectric elastomers [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2019 , 7 (8) : 3729-3736 .
MLA Chen, Jie et al. "Ultrahigh discharge efficiency and energy density achieved at low electric fields in sandwich-structured polymer films containing dielectric elastomers" . | JOURNAL OF MATERIALS CHEMISTRY A 7 . 8 (2019) : 3729-3736 .
APA Chen, Jie , Wang, Yifei , Xu, Xinwei , Yuan, Qibin , Niu, Yujuan , Wang, Qing et al. Ultrahigh discharge efficiency and energy density achieved at low electric fields in sandwich-structured polymer films containing dielectric elastomers . | JOURNAL OF MATERIALS CHEMISTRY A , 2019 , 7 (8) , 3729-3736 .
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Enhanced permittivity and permeability of (1-y)(Mg0.95Zn0.05)(2)TiO4-yMg(0.95) Zn0.05Fe2O4 ceramics EI SCIE Scopus
期刊论文 | 2018 , 38 (16) , 5367-5374 | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
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Abstract :

We report the preparation of the solid-solutions (1-y)(Mg0.95Zn0.05)(2)TiO4-yMg(0.95)Zn(0.05)Fe(2)O(4) (y = 0, 0.1, 0.3, 0.5, 0.7, 0.9, 1) by traditional solid-state reaction and systematically study their phases, morphologies, and magnetodielectric properties. The giant dielectric constants are observed at low frequency in the ceramics, with y > 0.5 when the sintering temperature exceeds 1200 degrees C. The highest relative permittivity epsilon' of 9.98 x 10(3) at 30 kHz and the largest squareness ratio of 0.89 for the magnetic hysteresis loop are achieved in 0.1MZT-0.9MZF. In addition, the enhanced initial permeability mu(i) of similar to 70 is obtained in 0.3MZT-0.7MZF due to its large grain size and probably the smaller magnetostriction and internal stress caused by lower relative density. All the results indicate that our solid-solutions with y > 0.5 can considerably improve the dielectric and magnetic properties, providing more advantages than the simple bi-phasic compounds in the applications for novel electronic devices.

Keyword :

Solid-solutions Ferrite Permeability Spinel Giant dielectric constant

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GB/T 7714 Me, Rong , Cheng, Yatong , Liu, Wenlong et al. Enhanced permittivity and permeability of (1-y)(Mg0.95Zn0.05)(2)TiO4-yMg(0.95) Zn0.05Fe2O4 ceramics [J]. | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY , 2018 , 38 (16) : 5367-5374 .
MLA Me, Rong et al. "Enhanced permittivity and permeability of (1-y)(Mg0.95Zn0.05)(2)TiO4-yMg(0.95) Zn0.05Fe2O4 ceramics" . | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY 38 . 16 (2018) : 5367-5374 .
APA Me, Rong , Cheng, Yatong , Liu, Wenlong , Wu, Liangliang , Yuan, Qibin , Zhang, Huachen et al. Enhanced permittivity and permeability of (1-y)(Mg0.95Zn0.05)(2)TiO4-yMg(0.95) Zn0.05Fe2O4 ceramics . | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY , 2018 , 38 (16) , 5367-5374 .
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Enhancement of light extraction by ZnO nanostructures on vertical GaN light emitting diodes EI CPCI-S
会议论文 | 2018 , 10823 | Conference on Nanophotonics and Micro/Nano Optics IV
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Abstract :

Controllable growth of ZnO nanostructures were realized on the surface patterned vertical-type GaN light emitting diodes (LEDs) by chemical solution method at low temperature. Aqueous ammonia has been added to manipulate the pH values of the growth solution to optimize the morphology of the ZnO nanostructures and light extraction efficiency from GaN LED surface. It is revealed that ZnO nanostructures were mainly grown on the tips of the GaN surface pyramids at pH value of 8.5. With decreasing pH value, ZnO nanostructures were observed grown both on tip and bottom of the GaN pyramids. On the contrary, the growth of ZnO nanostructures was greatly inhibited by increasing pH value above 10. The electroluminescence (EL) spectra intensity was enhanced by 40% for GaN LEDs topped with ZnO nanostructures at pH value of 8.5. This enhancement is attributed to the ZnO nanostructures tip-grown on vertical GaN LEDs effectively reducing the total internal reflection and minimizing Fresnel loss.

Keyword :

nanostructures Solid-state lighting GaN extraction efficiency surface texturing light emitting diodes

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GB/T 7714 Li, Yuanjie , Sun, Wenci , Wang, Hong et al. Enhancement of light extraction by ZnO nanostructures on vertical GaN light emitting diodes [C] . 2018 .
MLA Li, Yuanjie et al. "Enhancement of light extraction by ZnO nanostructures on vertical GaN light emitting diodes" . (2018) .
APA Li, Yuanjie , Sun, Wenci , Wang, Hong , Zhang, Minyan , Yun, Feng . Enhancement of light extraction by ZnO nanostructures on vertical GaN light emitting diodes . (2018) .
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Atomic-scale evidence for displacive disorder in bismuth zinc niobate pyrochlore EI SCIE PubMed Scopus
期刊论文 | 2018 , 192 , 57-68 | ULTRAMICROSCOPY
WoS CC Cited Count: 1 SCOPUS Cited Count: 1
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Abstract :

Pyrochlores characterized by the chemical formula A(2)B(2)O(7) form an extended class of materials with interesting physical and chemical properties. The compound Bi(1.5)ZnNb(1.5)O(7 )is prototypical. Its excellent dielectric properties make it attractive, e.g. for capacitors, tunable microwave devices and electric-energy storage equipment. Bi1.5ZnNb1.5O7 shows an intriguing frequency-dispersive dielectric relaxation at 50 K <= T <= 250 K, which has been studied intensively but is still not fully understood. In this first study on a pyrochlore by atomic-resolution transmission electron microscopy we observe the Bi atoms on A sites since, due to their low nuclear charge, the contribution of Zn atoms to the contrast of these sites is negligible. We find in our [(1) over bar 00]and [112] oriented images that the position of the atomic intensity maxima do not coincide with the projected Wyckoff positions of the basic pyrochlore lattice. This supplies atomic-scale evidence for displacive disorder on split A-type sites. The Bi atoms are sessile, only occasionally we observe in time sequences of images jumps between individual split-site positions. The apertaining jump rate of the order of 0.1-1 Hz is by ten orders of magnitude lower than the values derived in the literature from Arrhenius plots of the low-temperature dielectric relaxation data. It is argued that these jumps are radiation induced. Therefore our observations are ruling out a contribution of Bi-atom jumps to low-temperature dielectric A sites-related relaxation. It is suggested that this relaxation is mediated by jumps of Zn atoms.

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GB/T 7714 Jia, Chun-Lin , Jin, Lei , Chen, Yue-Hua et al. Atomic-scale evidence for displacive disorder in bismuth zinc niobate pyrochlore [J]. | ULTRAMICROSCOPY , 2018 , 192 : 57-68 .
MLA Jia, Chun-Lin et al. "Atomic-scale evidence for displacive disorder in bismuth zinc niobate pyrochlore" . | ULTRAMICROSCOPY 192 (2018) : 57-68 .
APA Jia, Chun-Lin , Jin, Lei , Chen, Yue-Hua , Urban, Knut W. , Wang, Hong . Atomic-scale evidence for displacive disorder in bismuth zinc niobate pyrochlore . | ULTRAMICROSCOPY , 2018 , 192 , 57-68 .
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Heteroepitaxial growth and interface structure of pyrochlore (Ca,Ti)(2)(Nb,Ti)(2)O-7 thin films on (110) NdGaO3 substrates EI SCIE Scopus
期刊论文 | 2018 , 484 , 64-69 | JOURNAL OF CRYSTAL GROWTH
WoS CC Cited Count: 2 SCOPUS Cited Count: 2
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Abstract :

Epitaxial thin films of (Ca, Ti)(2)(Nb, Ti)(2)O-7 with pyrochlore structure have been successfully fabricated on orthorhombic (1 1 0) NdGaO3 substrates by a magnetron sputtering system. By analysis of selected-area electron diffraction patterns, the film-substrate orientation relationship is determined to be < 0 0 1 >[1 0 0](film)//(0 0 1)(1 1 0)(substrate). Atomic-scale structure investigations of the heterointerface by means of advanced electron microscopy reveal that a perovskite-type Ca(Ti, Nb)O-3 layer with a thickness of several unit cells forms between the (Ca, Ti)(2)(Nb, Ti)(2)O-7 films and the NdGaO3 substrates. The formation of the Ca(Ti, Nb) O3 layer results from the demand for accommodation of the crystal structure mismatching between the pyrochlore film and the perovskite-type substrate, which favors the epitaxial growth of the (Ca, Ti)(2)(Nb, Ti)(2)O-7 films on the NdGaO3 substrates. (C) 2017 Elsevier B.V. All rights reserved.

Keyword :

Advanced electron microscopy Interface Pyrochlore structure Thin films

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GB/T 7714 Jin, Xiao-Wei , Chen, Yue-Hua , Lu, Lu et al. Heteroepitaxial growth and interface structure of pyrochlore (Ca,Ti)(2)(Nb,Ti)(2)O-7 thin films on (110) NdGaO3 substrates [J]. | JOURNAL OF CRYSTAL GROWTH , 2018 , 484 : 64-69 .
MLA Jin, Xiao-Wei et al. "Heteroepitaxial growth and interface structure of pyrochlore (Ca,Ti)(2)(Nb,Ti)(2)O-7 thin films on (110) NdGaO3 substrates" . | JOURNAL OF CRYSTAL GROWTH 484 (2018) : 64-69 .
APA Jin, Xiao-Wei , Chen, Yue-Hua , Lu, Lu , Mi, Shao-Bo , Jin, Lei , Jing, Hong-Mei et al. Heteroepitaxial growth and interface structure of pyrochlore (Ca,Ti)(2)(Nb,Ti)(2)O-7 thin films on (110) NdGaO3 substrates . | JOURNAL OF CRYSTAL GROWTH , 2018 , 484 , 64-69 .
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Interface thickness optimization of lead-free oxide multilayer capacitors for high-performance energy storage EI SCIE Scopus
期刊论文 | 2018 , 6 (4) , 1858-1864 | JOURNAL OF MATERIALS CHEMISTRY A
WoS CC Cited Count: 8 SCOPUS Cited Count: 8
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Abstract :

The effects of interface density and total multilayer film thickness on the dielectric properties and breakdown behavior have been revealed in this work by investigating the environment-friendly energy storage multilayer films of Ba0.7Ca0.3TiO3 (BCT) and BaZr0.2Ti0.8O3 (BZT) dielectrics. Numerical simulations based on a finite element method have given the breakdown process vividly, which agreed well with the experimental results. Moreover, not only the ultrahigh energy storage density of 51.8 J cm(-3) with a great efficiency of 81.2% at room temperature but also robust thermal stability has been obtained by optimizing the interface density and total thickness. High energy density above 25.1 J cm(-3) and excellent efficiency over 63.6% from room temperature to 200 degrees C provide a solid basis for potential applications of the multilayer systems in harsh environments.

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GB/T 7714 Sun, Zixiong , Wang, Linxi , Liu, Ming et al. Interface thickness optimization of lead-free oxide multilayer capacitors for high-performance energy storage [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2018 , 6 (4) : 1858-1864 .
MLA Sun, Zixiong et al. "Interface thickness optimization of lead-free oxide multilayer capacitors for high-performance energy storage" . | JOURNAL OF MATERIALS CHEMISTRY A 6 . 4 (2018) : 1858-1864 .
APA Sun, Zixiong , Wang, Linxi , Liu, Ming , Ma, Chunrui , Liang, Zhongshuai , Fan, Qiaolan et al. Interface thickness optimization of lead-free oxide multilayer capacitors for high-performance energy storage . | JOURNAL OF MATERIALS CHEMISTRY A , 2018 , 6 (4) , 1858-1864 .
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Ultra-low temperature sintering and microwave dielectric properties of a novel temperature stable Na2Mo2O7-Na0.5Bi0.5MoO4 ceramic EI SCIE Scopus
期刊论文 | 2018 , 38 (2) , 813-816 | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
WoS CC Cited Count: 12 SCOPUS Cited Count: 11
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Abstract :

The novel ultra-low temperature sintering (1-x)Na(2)Mo(2)O(7-)xNa(0.5)Bi(0.5)MoO(4) ceramics have been obtained via solid-state reaction method for passive integration use. The Na2Mo2O7 and Na0.5Bi0.5MoO4 crystal phases are found to be compatible with each other from the results of XRD and SEM-EDS. With the x value changing from 0.36 to 1.00, the epsilon(r) increases from 16.0 to 32.0 and the tau(f) value varies from -58 to 47 ppm/degrees C. At x = 0.75, the 0.25Na(2)Mo(2)O(7)-0.75Na(0.5)Bi(0.5)MoO(4) ceramic sintered at an ultra-low sintering temperature of 580 degrees C can be densified ( > 96%) and possesses good microwave dielectric properties of an epsilon(r) of 24.0, a Q x f value of 13,000 GHz (at 6.2 GHz), and a tau(f) value of 3 ppm/degrees C. The theoretical epsilon(r) and tau(f) of the (1-x)Na2Mo2O7-xNa(0.5)Bi(0.5)MoO(4) composites were calculated using the mixing law and in accordance with the measured values.

Keyword :

Ultra-low temperature sintering Microwave dielectric properties Dielectrics Temperature stable material Ceramics

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GB/T 7714 Zhang, Gaoqun , Guo, Jing , Yuan, Xiaofeng et al. Ultra-low temperature sintering and microwave dielectric properties of a novel temperature stable Na2Mo2O7-Na0.5Bi0.5MoO4 ceramic [J]. | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY , 2018 , 38 (2) : 813-816 .
MLA Zhang, Gaoqun et al. "Ultra-low temperature sintering and microwave dielectric properties of a novel temperature stable Na2Mo2O7-Na0.5Bi0.5MoO4 ceramic" . | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY 38 . 2 (2018) : 813-816 .
APA Zhang, Gaoqun , Guo, Jing , Yuan, Xiaofeng , Wang, Hong . Ultra-low temperature sintering and microwave dielectric properties of a novel temperature stable Na2Mo2O7-Na0.5Bi0.5MoO4 ceramic . | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY , 2018 , 38 (2) , 813-816 .
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Simultaneously achieved temperature-insensitive high energy density and efficiency in domain engineered BaTiO3-Bi(Mg0.5Zr0.5)O-3 lead-free relaxor ferroelectrics EI SCIE Scopus
期刊论文 | 2018 , 52 , 203-210 | NANO ENERGY
WoS CC Cited Count: 29 SCOPUS Cited Count: 35
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Abstract :

The development of lead-free ceramics for electrostatic energy storage has attracted great interest because of the growing environmental concerns. Despite the extensive exploration, the unsuccess in synergistically optimizing both energy density and efficiency of polycrystalline materials is the major hurdle for their practical applications. Herein, Bi(Mg0.5Zr0.5)O-3-modified BaTiO3 lead-free relaxor ferroelectric ceramics are demonstrated to be viable candidates for energy storage. The materials can simultaneously deliver a high recoverable energy density of 2.9 J cm(-3) and a high energy efficiency of 86.8%, which are enhanced by 625% and 156% over those of unmodified BaTiO3, while keeping insensitive to thermal stimulus over 30-150 degrees C. It is unveiled that the incorporation of Bi(Mg0.5Zr0.5)O-3 favors the formation of polar nanoregions (PNRs), as evidenced by transmission electron microscope and piezoresponse force microscopy, which increases the threshold field to induce long range order and decreases the stability thereof, contributing to the more linear-towards polarization behavior. The dynamic PNRs along with the decreased grain size, increased bulk density, and consequently enhanced dielectric breakdown strength (301.4 kV cm(-1)) are responsible for the superior energy storage performance of Bi (Mg0.5Zr0.5)O-3-modified BaTiO3 ceramics. This work opens up a new avenue to tailor lead-free dielectrics toward high energy storage performance for electrical energy storage.

Keyword :

BaTiO3-Bi(Mg0.5Zr0.5)O-3 Energy storage Lead-free Relaxor ferroelectrics Thermal stability

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GB/T 7714 Yuan, Qibin , Li, Geng , Yao, Fang-Zhou et al. Simultaneously achieved temperature-insensitive high energy density and efficiency in domain engineered BaTiO3-Bi(Mg0.5Zr0.5)O-3 lead-free relaxor ferroelectrics [J]. | NANO ENERGY , 2018 , 52 : 203-210 .
MLA Yuan, Qibin et al. "Simultaneously achieved temperature-insensitive high energy density and efficiency in domain engineered BaTiO3-Bi(Mg0.5Zr0.5)O-3 lead-free relaxor ferroelectrics" . | NANO ENERGY 52 (2018) : 203-210 .
APA Yuan, Qibin , Li, Geng , Yao, Fang-Zhou , Cheng, Shao-Dong , Wang, Yifei , Ma, Rong et al. Simultaneously achieved temperature-insensitive high energy density and efficiency in domain engineered BaTiO3-Bi(Mg0.5Zr0.5)O-3 lead-free relaxor ferroelectrics . | NANO ENERGY , 2018 , 52 , 203-210 .
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Ultrahigh energy density and greatly enhanced discharged efficiency of sandwich-structured polymer nanocomposites with optimized spatial organization EI SCIE Scopus
期刊论文 | 2018 , 44 , 364-370 | NANO ENERGY
WoS CC Cited Count: 34 SCOPUS Cited Count: 44
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Abstract :

Sandwich-structured polymer nanocomposites that provide a pathway to overcome the paradox between permittivity and breakdown strength ever existing in dielectric materials are receiving increasing attentions for their superior energy storage performance. Despite certain advances obtained in previous effort, further enhancement of the energy density by structure optimizing is still a challenge. Herein, we present a newly designed sandwich-structured barium titanate/poly(vinylidene fluoride-co-hexafluoropropylene) (BaTiO3/P(VDF-HFP)) nanocomposite via layer-by-layer tape casting process, where high contents of BaTiO3 nanoparticles are dispersed in the middle layer to offer high permittivity, while two outer layers containing small amounts of BaTiO3 provide favorable breakdown strength. The solution-processed nanocomposites with an optimal composition exhibits an ultrahigh discharged energy density of 26.4 J cm(-3) and a superior discharged efficiency of 72%, which are by far the highest values ever achieved in sandwich-structured dielectric polymer composites. It is revealed that the designed structure can enhance the breakdown strength and discharged efficiency by preventing the charge injection from electrodes and impeding the development of electrical tress during breakdown process, as confirmed by the leakage current and thermally stimulated depolarization current measurements, as well as the finite element simulations. This work represents a new design paradigm to exploit advanced dielectric materials for electrical energy storage applications.

Keyword :

Dielectric breakdown Sandwich structure Electrical energy storage Capacitor Polymer nanocomposites

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GB/T 7714 Wang, Yifei , Wang, Linxi , Yuan, Qibin et al. Ultrahigh energy density and greatly enhanced discharged efficiency of sandwich-structured polymer nanocomposites with optimized spatial organization [J]. | NANO ENERGY , 2018 , 44 : 364-370 .
MLA Wang, Yifei et al. "Ultrahigh energy density and greatly enhanced discharged efficiency of sandwich-structured polymer nanocomposites with optimized spatial organization" . | NANO ENERGY 44 (2018) : 364-370 .
APA Wang, Yifei , Wang, Linxi , Yuan, Qibin , Chen, Jie , Niu, Yujuan , Xu, Xinwei et al. Ultrahigh energy density and greatly enhanced discharged efficiency of sandwich-structured polymer nanocomposites with optimized spatial organization . | NANO ENERGY , 2018 , 44 , 364-370 .
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Multilayered ferroelectric polymer films incorporating low-dielectric-constant components for concurrent enhancement of energy density and charge?discharge efficiency EI Scopus SCIE
期刊论文 | 2018 , 54 , 288-296 | Nano Energy
WoS CC Cited Count: 7 SCOPUS Cited Count: 8
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Abstract :

Ferroelectric polymers are the materials of choice for capacitive energy storage owing to their highest dielectric constants (K) and the best energy densities among the current dielectric polymers. Herein, different from the conventional approaches based on the incorporation of high-K fillers into the single-layer films to enhance the capacitive performance, a low-K polymer, i.e. PMMA with a K value of 3–4, is selected as an example and introduced into the layered configurations of the ferroelectric polymer. Both improvements in the energy density (Ue) and charge–discharge efficiency (η) over those of the pristine polymer have been achieved via the establishment of multiple interlaminar interfaces and modulation of component ratios. The influence of film configuration on the capacitive performance has been systematically studied. The trilayered all-polymer film with optimized component ratio is capable of operating with a charge–discharge efficiency as high as 84% and concurrently delivering an energy density up to 20.3 J cm−3, surpassing the capacitive performance of the currently available polymer dielectrics that present the upper limits of Ue of ~20 J cm−3 and η of ~80%. Along with excellent stability of dielectric and mechanical properties of the polymer films, this work suggests great potential of the multicomponent ferroelectric polymers with layered architecture for electrical energy storage applications. © 2018 Elsevier Ltd

Keyword :

Capacitive energy storage Capacitive performance Dielectric constants (k) Electrical energy storages Ferroelectric polymer films Ferroelectric polymers Low dielectric constants Power densities

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GB/T 7714 Chen, Jie , Wang, Yifei , Yuan, Qibin et al. Multilayered ferroelectric polymer films incorporating low-dielectric-constant components for concurrent enhancement of energy density and charge?discharge efficiency [J]. | Nano Energy , 2018 , 54 : 288-296 .
MLA Chen, Jie et al. "Multilayered ferroelectric polymer films incorporating low-dielectric-constant components for concurrent enhancement of energy density and charge?discharge efficiency" . | Nano Energy 54 (2018) : 288-296 .
APA Chen, Jie , Wang, Yifei , Yuan, Qibin , Xu, Xinwei , Niu, Yujuan , Wang, Qing et al. Multilayered ferroelectric polymer films incorporating low-dielectric-constant components for concurrent enhancement of energy density and charge?discharge efficiency . | Nano Energy , 2018 , 54 , 288-296 .
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