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Author:

Han, Y. M. (Han, Y. M..) | Han, Z. W. (Han, Z. W..) | Cao, J. J. (Cao, J. J..) | Chow, J. C. (Chow, J. C..) | Watson, J. G. (Watson, J. G..) | An, Z. S. (An, Z. S..) | Liu, S. X. (Liu, S. X..) | Zhang, R. J. (Zhang, R. J..)

Indexed by:

SCIE EI Scopus

Abstract:

PM2.5 and TSP samples were collected at Lake Daihai, a rural high-mountain area in China, in four seasons during 2005-2007. Organic carbon (OC), elemental carbon (EC), char-EC, and soot-EC were analyzed using the thermal/optical reflectance (TOR) method with different temperature plateaus and oxidation atmospheres. TC, OC, EC, and char-EC concentrations of TSP and PM2.5 showed seasonal variations with the highest concentrations in winter and the lowest in Summer, while soot-EC reveals a little different variation, with the highest concentration in spring, indicating different source contributions from other parameters. OC/EC correlations were weaker at Daihai than those from urban areas. Although little differences existed in TSP and PM2.5, average OC/EC ratios varied seasonally and ranged from similar to 9.0 in winter to similar to 5.0 in spring. Char-/soot-EC ratios showed similar pattern, with the highest average ratios (> 3.0) in winter, consistent with the contributions from residential biomass burning and coal combustion. Back trajectories related the highest carbon concentrations with the southeasterly air masses and the lowest carbon levels with northward flows. (c) 2007 Elsevier Ltd. All rights reserved.

Keyword:

black carbon char Char-/soot-EC ratios soot thermal/optical reflectance (TOR) method

Author Community:

  • [ 1 ] [Han, Y. M.; Cao, J. J.; Chow, J. C.; Watson, J. G.; An, Z. S.; Liu, S. X.] Chinese Acad Sci, SKQLLOG, Inst Earth Environm, Xian 710075, Peoples R China
  • [ 2 ] [Han, Z. W.; Zhang, R. J.] Chinese Acad Sci, Inst Atmospher Phys, Beijing 100029, Peoples R China
  • [ 3 ] [Cao, J. J.] Xian Jiaotong Univ, Dept Environm Sci, Xian 710049, Peoples R China
  • [ 4 ] [Chow, J. C.; Watson, J. G.] Desert Res Inst, Reno, NV 89512 USA

Reprint Author's Address:

  • Chinese Acad Sci, SKQLLOG, Inst Earth Environm, Xian 710075, Peoples R China.

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Source :

ATMOSPHERIC ENVIRONMENT

ISSN: 1352-2310

Year: 2008

Issue: 10

Volume: 42

Page: 2405-2414

2 . 8 9

JCR@2008

4 . 7 9 8

JCR@2020

ESI Discipline: GEOSCIENCES;

JCR Journal Grade:2

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 64

SCOPUS Cited Count: 82

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 9

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