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Author:

Li, Xia (Li, Xia.) | Bei, Naifang (Bei, Naifang.) | Hu, Bo (Hu, Bo.) | Wu, Jiarui (Wu, Jiarui.) | Pan, Yuepeng (Pan, Yuepeng.) | Wen, Tianxue (Wen, Tianxue.) | Liu, Zirui (Liu, Zirui.) | Liu, Lang (Liu, Lang.) | Wang, Ruonan (Wang, Ruonan.) | Li, Guohui (Li, Guohui.)

Indexed by:

EI SCIE PubMed Engineering Village

Abstract:

Stringent mitigation measures have reduced wintertime fine particulate matter (PM2.5) concentrations by 42.2% from 2013 to 2018 in the Beijing-Tianjin-Hebei (BTH) region, but severe PM pollution still frequently engulfs the region. The observed nitrate aerosols have not exhibited a significant decreasing trend and constituted a major fraction (about 20%) of the total PM2.5, although the surface-measured NO2 concentration has decreased by over 20%. The contributions of nitrogen oxides (NOX) emissions mitigation to the nitrate and PM2.5 concentrations and how to alleviate nitrate aerosols efficiently under the current situation still remains elusive. The WRF-Chem model simulations of a persistent and heavy PM pollution episode in January 2019 in the BTH reveal that NOX emissions mitigation does not help lower wintertime nitrate and PM2.5 concentrations under current conditions in the BTH. A 50% reduction in NOX emissions only decreases nitrate mass by 10.3% but increases PM2.5 concentrations by 3.2%, because the substantial O3 increase induced by NOX mitigation offsets the HNO3 loss and enhances sulfate and secondary organic aerosols formation. Our results are further consolidated by the occurrence of severe PM pollution in the BTH during the COVID-19 outbreak, with a significant reduction in NO2 concentration. Mitigation of NH3 emissions constitutes the priority measure to effectively lower the nitrate and PM2.5 concentrations in the BTH under current conditions, with 35.5% and 12.7% decrease, respectively, when NH3 emissions are reduced by 50%. © 2021 Elsevier Ltd

Keyword:

Aerosols Ammonia Nitrates Nitrogen oxides Particles (particulate matter) Pollution Sulfur compounds

Author Community:

  • [ 1 ] [Li, Xia]Key Lab of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an; Shaanxi; 710061, China
  • [ 2 ] [Li, Xia]University of the Chinese Academy of Sciences, Beijing; 100049, China
  • [ 3 ] [Bei, Naifang]School of Human Settlements and Civil Engineering, Xi'an Jiaotong University, Xi'an; Shaanxi; 710049, China
  • [ 4 ] [Hu, Bo]State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 5 ] [Wu, Jiarui]Key Lab of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an; Shaanxi; 710061, China
  • [ 6 ] [Pan, Yuepeng]State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 7 ] [Wen, Tianxue]State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 8 ] [Liu, Zirui]State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 9 ] [Liu, Lang]Key Lab of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an; Shaanxi; 710061, China
  • [ 10 ] [Wang, Ruonan]Key Lab of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an; Shaanxi; 710061, China
  • [ 11 ] [Li, Guohui]Key Lab of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an; Shaanxi; 710061, China
  • [ 12 ] [Li, Guohui]CAS Center for Excellence in Quaternary Science and Global Change, Xi'an; Shaanxi; 710061, China

Reprint Author's Address:

  • [Li, Guohui]Key Lab of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an; Shaanxi; 710061, China;;[Li, Guohui]CAS Center for Excellence in Quaternary Science and Global Change, Xi'an; Shaanxi; 710061, China;;

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Source :

Environmental Pollution

ISSN: 0269-7491

Year: 2021

Volume: 279

8 . 0 7 1

JCR@2020

ESI Discipline: ENVIRONMENT/ECOLOGY;

ESI HC Threshold:30

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 9

SCOPUS Cited Count: 30

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 19

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