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Author:

Zhou, L. (Zhou, L..) | Qu, Z. G. (Qu, Z. G..) (Scholars:屈治国) | Chen, L. (Chen, L..) (Scholars:陈黎) | Tao, W. Q. (Tao, W. Q..) (Scholars:陶文铨)

Indexed by:

SCIE Scopus

Abstract:

A two-dimensional lattice Boltzmann (LB) approach was established to implement kinetic concentration boundary conditions in interfacial mass-transfer processes and to simulate the adsorption process in porous media at pore scale and mesoscopic levels. A general treatment was applied to conduct three types of concentration boundary conditions effectively and accurately. Applicability for adsorption was verified by two benchmark examples, which were representative of the interparticle mass transport and intraparticle mass transport in the adsorption system, respectively. The gas-solid adsorption process in reconstructed porous media at the pore scale level was numerically investigated. Mass-transfer processes of the adsorption reaction were simulated by executing Langmuir adsorption kinetics on surfaces of adsorbent particles. Meanwhile, the homogeneous solid diffusion model (HSDM) was used for mass transport in interior particles. The transient adsorbed amount was obtained in detail, and the impact of flow condition, porosity, and adsorbent particle size on the entire dynamic adsorption performance was investigated. The time needed to approach steady state decreased with increased fluid velocity. Transient adsorption capability and time consumption to equilibrium were nearly independent of porosity, whereas increasing pore size led to a moderating adsorption rate and more time was consumed to approach the saturation adsorption. Benefiting from the advantages of the LB method, both bulk and intraparticle mass transfer performances during adsorption can be obtained using the present pore scale approach. Thus, interparticle mass transfer and intraparticle mass transfer are the two primary segments, and intraparticle diffusion has the dominant role. (C) 2015 Elsevier Inc. All rights reserved.

Keyword:

Adsorption Langmuir kinetics LBM Pore scale Porous media

Author Community:

  • [ 1 ] [Zhou, L.; Qu, Z. G.; Chen, L.; Tao, W. Q.] Xi An Jiao Tong Univ, Sch Energy & Power Engn, MOE Key Lab Thermal Fluid Sci & Engn, Xian 710049, Peoples R China
  • [ 2 ] [Zhou, L.]Xi An Jiao Tong Univ, Sch Energy & Power Engn, MOE Key Lab Thermal Fluid Sci & Engn, Xian 710049, Peoples R China
  • [ 3 ] [Qu, Z. G.]Xi An Jiao Tong Univ, Sch Energy & Power Engn, MOE Key Lab Thermal Fluid Sci & Engn, Xian 710049, Peoples R China
  • [ 4 ] [Chen, L.]Xi An Jiao Tong Univ, Sch Energy & Power Engn, MOE Key Lab Thermal Fluid Sci & Engn, Xian 710049, Peoples R China
  • [ 5 ] [Tao, W. Q.]Xi An Jiao Tong Univ, Sch Energy & Power Engn, MOE Key Lab Thermal Fluid Sci & Engn, Xian 710049, Peoples R China

Reprint Author's Address:

  • 屈治国

    Xi An Jiao Tong Univ, Sch Energy & Power Engn, MOE Key Lab Thermal Fluid Sci & Engn, Xian 710049, Peoples R China.

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Source :

JOURNAL OF COMPUTATIONAL PHYSICS

ISSN: 0021-9991

Year: 2015

Volume: 300

Page: 800-813

2 . 5 5 6

JCR@2015

3 . 5 5 3

JCR@2020

ESI Discipline: PHYSICS;

ESI HC Threshold:157

JCR Journal Grade:2

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 46

SCOPUS Cited Count: 73

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 7

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