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Author:

Sun, Hongchen (Sun, Hongchen.) | Xu, Ran (Xu, Ran.) | Zhu, Qingshan (Zhu, Qingshan.) | Zhao, Shiyu (Zhao, Shiyu.) | Wang, Mengjiao (Wang, Mengjiao.) | Wei, Xiaoyong (Wei, Xiaoyong.) | Feng, Yujun (Feng, Yujun.) | Xu, Zhuo (Xu, Zhuo.) | Yao, Xi (Yao, Xi.)

Indexed by:

SCIE EI Scopus Web of Science

Abstract:

Antiferroelectric (AFE) materials have superior energy storage properties in high power multilayer ceramic capacitors (MLCCs). To adapt to the sintering temperature of inner metal electrodes with less palladium content, in this work, Al2O3 was added to Pb0.95Ta0.02Sr0.02(Zr0.50Sn0.10Ti0.10)O-3 (PLSZST) AFE ceramics, in an attempt to reduce the sintering temperature. Results of this study demonstrate that the optimal composition of PLSZST-0.8 wt% Al2O3 sintered at a lower temperature 1040 degrees C, has a high recoverable energy density (W-re, 3.23 J/cm(3)) and a high efficiency (eta, 90 %) at room temperature. It is also high in pulse discharge energy density (W-dis, 2.45 J/cm(3)), current density (1369 A/cm(2)), and has an extremely short period of discharge (less than 500 ns). In addition, both W-re and eta demonstrate a good stability in temperature within a wide range of 30 degrees C-100 degrees C. In sum, this novel AFE composition has great potentials for energy storage applications such as high energy density MLCCs.

Keyword:

Antiferroelectric ceramics Energy storage Eutectic Low sintering temperature MLCCs

Author Community:

  • [ 1 ] [Wei, Xiaoyong]Xi An Jiao Tong Univ, Elect Mat Res Lab, Key Lab Minist Educ, Sch Elect & Informat Engn, Xian 710049, Peoples R China
  • [ 2 ] [Wei, Xiaoyong]Xi An Jiao Tong Univ, Int Ctr Dielect Res, Sch Elect & Informat Engn, Xian 710049, Peoples R China
  • [ 3 ] [Feng, Yujun]Xi An Jiao Tong Univ, Elect Mat Res Lab, Key Lab Minist Educ, Sch Elect & Informat Engn, Xian 710049, Peoples R China
  • [ 4 ] [Feng, Yujun]Xi An Jiao Tong Univ, Int Ctr Dielect Res, Sch Elect & Informat Engn, Xian 710049, Peoples R China

Reprint Author's Address:

  • X. Wei;;Electronic Materials Research Laboratory, Key Laboratory of the Ministry of Education & International Center for Dielectric Research, School of Electronic and Information Engineering, Xi'an Jiaotong University, Xi'an, 710049, China;;email: wdy@mail.xjtu.edu.cn;;

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Source :

JOURNAL OF THE EUROPEAN CERAMIC SOCIETY

ISSN: 0955-2219

Year: 2022

Issue: 4

Volume: 42

Page: 1380-1387

5 . 3 0 2

JCR@2020

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:7

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 23

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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