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Author:

Zhang, Ningning (Zhang, Ningning.) | Cao, Junji (Cao, Junji.) | Liu, Suixin (Liu, Suixin.) | Zhao, ZhuZi (Zhao, ZhuZi.) | Xu, Hongmei (Xu, Hongmei.) | Xiao, Shun (Xiao, Shun.)

Indexed by:

SCIE EI Scopus

Abstract:

PM2.5 and total suspended particulate (TSP) samples were collected from June to September 2010 at Qinghai Lake, northeastern Tibetan Plateau. The concentrations of major water-soluble ions, 10 elements, elemental carbons (ECs) and organic carbons (OCs) were quantified. Mass concentrations of PM2.5 and TSP were 21.27 +/- 10.70 mu g m(-3) and 41.47 +/- 20.25 mu g m(-3), respectively, and the mean ratio of PM2.5/TSP was 0.51. The greatest anion and cation in both PM2.5 and TSP samples were SO42- and Ca2+, respectively. Crustal elements, such as Ca, Fe and K, were the main elements in our aerosol samples, and their enrichment factors (EFs) were lower than 10. EFs for Pb, As, and Zn were greater than 10, indicating that they were influenced by anthropogenic sources. EC concentrations were 0.33 +/- 0.17 mu g m(-3) and 0.47 +/- 0.28 mu g m(-3), whereas OC concentrations were 1.49 +/- 0.63 mu g m(-3) and 2.30 +/- 0.95 mu g m(-3) in PM2.5 and TSP, respectively. Based on the calculated ratios of EC/TC and K+/EC, most of the ECs were found to be related to biomass burning emissions. Because of the pollution from local sources, the ratios of OC/EC were 4.77 +/- 1.32 and 5.23 +/- 1.39 in PM2.5 and TSP, respectively, which were lower than those of other remote sites. Salt particles produced by the salty lake reacted with acid gases and caused most of the nitrates and a small fraction of sulfate to be distributed in coarse mode: Cl deficit was also observed in our aerosol samples. Results of backward trajectories and correlation analysis show that the concentrations of SO42-, OCs, As, Pb, and Zn, were influenced by the long-distance transport from eastern China. (C) 2013 Elsevier B.V. All rights reserved.

Keyword:

Aerosol Carbonaceous components Elemental enrichment Remoter atmosphere Transport

Author Community:

  • [ 1 ] [Zhang, Ningning; Cao, Junji; Liu, Suixin; Zhao, ZhuZi; Xu, Hongmei; Xiao, Shun] Chinese Acad Sci, Inst Earth Environm, SKLLQG, Key Lab Aerosol, Xian, Peoples R China
  • [ 2 ] [Cao, Junji] Xi An Jiao Tong Univ, Inst Global Environm Change, Xian 710049, Peoples R China
  • [ 3 ] [Xiao, Shun] Shaanxi Meteorol Bur, Climate Ctr, Xian, Peoples R China
  • [ 4 ] [Xiao, Shun] Baoji Municipal, Meteorol Bur, Baoji, Peoples R China

Reprint Author's Address:

  • 10 Fenghui South Rd, Xian 710075, Peoples R China.

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Source :

ATMOSPHERIC RESEARCH

ISSN: 0169-8095

Year: 2014

Volume: 138

Page: 213-222

2 . 8 4 4

JCR@2014

5 . 3 6 9

JCR@2020

ESI Discipline: GEOSCIENCES;

ESI HC Threshold:187

JCR Journal Grade:2

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 47

SCOPUS Cited Count: 57

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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