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Abstract:
Complex porous structure and properties of a solid oxide fuel cell (SOFC) anode significantly affect the SOFC performance. In this study, the sintering process of the typical NiO-YSZ anode is simulated by a coarse-grained molecular dynamics method. After the sintering process simulation, the porous nanostructure is obtained and the thermophysical properties of the sintered anode are evaluated. It is found that the volume shrinkage occurs along with the self-assembly phenomenon during the sintering process. Sintering at relatively low temperature and high pressure could contribute to the densification of the anode. Compared with the experimental structure, the sintered anode obtained from this study shows a common morphology. Sintering at the nanoscale is beneficial to distribute the functional components equally. Furthermore, the effects of the sintering temperature, sintering pressure and material composition on the volumetric heat capacity and thermal expansion coefficient of the sintered anode are systematically discussed. The predicted thermophysical properties of the anode agree well with the open literature data. Results in this study could provide a guide of the sintering conditions and composition during the experimental studies to obtain the desired properties of the SOFC anode. (C) 2017 Elsevier Ltd. All rights reserved.
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APPLIED THERMAL ENGINEERING
ISSN: 1359-4311
Year: 2017
Volume: 125
Page: 209-219
3 . 7 7 1
JCR@2017
5 . 2 9 5
JCR@2020
ESI Discipline: ENGINEERING;
ESI HC Threshold:121
JCR Journal Grade:2
CAS Journal Grade:1
Cited Count:
WoS CC Cited Count: 2
SCOPUS Cited Count: 11
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 8
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