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< Page ,Total 88 >
Intelligent identification of steam jet condensation regime in water pipe flow system by wavelet multiresolution analysis of pressure oscillation and artificial neural network EI Scopus SCIE
期刊论文 | 2019 , 147 , 1047-1058 | Applied Thermal Engineering
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Abstract :

© 2018 Elsevier Ltd On-line recognition of condensation regime of vapor jet in pipe flow systems is a promising approach for flow assurance and intellectualization of industrial processes. However, the selection of distinguishable characteristics from pressure signals associated strongly with various condensation regimes is essential and challenging for satisfactory recognition purpose. Accordingly, an artificial neural network technique using wavelet multiresolution analysis of pressure oscillation signals for objective identification of jet condensation regimes is presented in this paper. The recognition procedure was carried out in two major steps. Statistical features of wavelet multiresolution analysis of pressure signals, i.e., mean of absolute and percentage of energy of each wavelet scale, were chose first. And then artificial neural network was adopted to construct classifiers for forecasting the condensation regimes automatically. The recognition results illustrated that the proposed method is feasible and effective for identifying vapor jet condensation regime in pipe flow system. Furthermore, it is suggested that statistical features of mean of absolute and percentage of energy at least four or more particular wavelet scales, and also sample length longer than 1.5 s could guarantee a satisfactory recognition rate above 90%.

Keyword :

Artificial neural network Condensation regime recognition Multiphase flow Pressure oscillation Wavelet multiresolution analysis

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GB/T 7714 Xu, Qiang , Ye, Shuyan , Liu, Weizhi et al. Intelligent identification of steam jet condensation regime in water pipe flow system by wavelet multiresolution analysis of pressure oscillation and artificial neural network [J]. | Applied Thermal Engineering , 2019 , 147 : 1047-1058 .
MLA Xu, Qiang et al. "Intelligent identification of steam jet condensation regime in water pipe flow system by wavelet multiresolution analysis of pressure oscillation and artificial neural network" . | Applied Thermal Engineering 147 (2019) : 1047-1058 .
APA Xu, Qiang , Ye, Shuyan , Liu, Weizhi , Chen, Yanshuang , Chen, Qiyu , Guo, Liejin . Intelligent identification of steam jet condensation regime in water pipe flow system by wavelet multiresolution analysis of pressure oscillation and artificial neural network . | Applied Thermal Engineering , 2019 , 147 , 1047-1058 .
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DFT study of the enhancement on hydrogen production by alkaline catalyzed water gas shift reaction in supercritical water EI CPCI-S SCIE Scopus
会议论文 | 2018 , 43 (30) , 13879-13886 | 8th International Conference on Hydrogen Production (ICH2P)
WoS CC Cited Count: 1 SCOPUS Cited Count: 8
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Abstract :

Supercritical water gasification (SCWG) is hopefully to be an acceptable choice for hydrogen production, the hydroxide ion assisted water gas shift reaction (WGSR) has been regarded as the most important reaction to generate hydrogen during the process. However, the principle of practical OH-catalyzed reaction is not possible to acquire by experiments. Thus, density functional theory (DFT) is utilized to investigate the reaction mechanism theoretically in this work. Through first principle calculations, every species and energy barrier for elementary steps are achieved, and formate ion is determined as the important intermediate. Besides, HCOO- + H2O -> HCO3- + H-2 is the dominant path to generate hydrogen, as well as the rate-determining step with 47.94 kcal/mol energy barrier. Furthermore, the reaction rate constant is calculated to be kcatalytic(S-1) = 2.34 x 10(12)exp(-1.80 x 10(5)/RT) using transition state theory with Wigner transmission coefficient (TST/w). Lastly, supercritical water condition is demonstrated to be a favored media for WGSR, because it may dissociate, dissolve or hydrolyze more hydroxide anion than conventional steam. The results are expected to benefit the control of reaction process and the design of SCWG reactor. (C) 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

Keyword :

Supercritical water Hydroxide ion DFT Water gas shift reaction

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GB/T 7714 Wang, Runyu , Guo, Liejin , Jin, Hui et al. DFT study of the enhancement on hydrogen production by alkaline catalyzed water gas shift reaction in supercritical water [C] . 2018 : 13879-13886 .
MLA Wang, Runyu et al. "DFT study of the enhancement on hydrogen production by alkaline catalyzed water gas shift reaction in supercritical water" . (2018) : 13879-13886 .
APA Wang, Runyu , Guo, Liejin , Jin, Hui , Lu, Libo , Yi, Lei , Zhang, Deming et al. DFT study of the enhancement on hydrogen production by alkaline catalyzed water gas shift reaction in supercritical water . (2018) : 13879-13886 .
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Evaluation of modified Ni/ZrO2 catalysts for hydrogen production by supercritical water gasification of oil-containing wastewater EI CPCI-S SCIE Scopus
会议论文 | 2018 , 43 (30) , 13896-13903 | 8th International Conference on Hydrogen Production (ICH2P)
WoS CC Cited Count: 1 SCOPUS Cited Count: 4
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Abstract :

Supercritical water gasification (SCWG) technology is a clean and cost-effective conversion technology due to its unique chemical and physical properties. However, the unique properties also lead to instability and inactivity for the pure Ni/ZrO2 catalyst in SCWG process. In this work, we investigated the effect of second metal addition on the catalytic performance by modifying Ni/ZrO2 catalysts with different promoters (Co, Ce, La, Y, Mg), which prepared by a single-step sol-gel method. The analysis results of catalysts by XRD, SEM and automatic micropore & chemisorption analyzer showed that Ce, Y, La may be helpful promoters to stabilize the structure of ZrO2. Compared to the non-catalytic experiment, all the catalysts showed significantly higher activities in the SCWG reaction. Among all catalysts, Ni-Co/ZrO2 exhibited excellent activity, which achieved the highest carbon gasification efficiency (CE) and highest hydrogen yield. Additionally, two key factors, concentration and temperature, were also investigated for the optimum conditions, and the maximum carbon gasification efficiency (CE) of 98.8% was achieved at 600 degrees C with the Ni-Co/ZrO2 catalyst. (C) 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

Keyword :

Oil-containing wastewater Modified Ni/ZrO2 catalysts Supercritical water gasification Hydrogen production

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GB/T 7714 Kou, Jiajing , Xu, Jialing , Jin, Hui et al. Evaluation of modified Ni/ZrO2 catalysts for hydrogen production by supercritical water gasification of oil-containing wastewater [C] . 2018 : 13896-13903 .
MLA Kou, Jiajing et al. "Evaluation of modified Ni/ZrO2 catalysts for hydrogen production by supercritical water gasification of oil-containing wastewater" . (2018) : 13896-13903 .
APA Kou, Jiajing , Xu, Jialing , Jin, Hui , Guo, Liejin , Zhang, Deming , Cao, Wen . Evaluation of modified Ni/ZrO2 catalysts for hydrogen production by supercritical water gasification of oil-containing wastewater . (2018) : 13896-13903 .
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One-pot annealing preparation of Na-doped graphitic carbon nitride from melamine and organometallic sodium salt for enhanced photocatalytic H-2 evolution EI CPCI-S SCIE Scopus
会议论文 | 2018 , 43 (30) , 13953-13961 | 8th International Conference on Hydrogen Production (ICH2P)
WoS CC Cited Count: 4 SCOPUS Cited Count: 4
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Abstract :

Na-doped graphitic carbon nitride was successfully developed by a one-pot preparation, that was, by simply annealing the mixture of melamine and organometallic sodium salt (ethylenediamine tetraacetic acid disodium salt). Visible-light-driven photocatalytic H-2 evolution activity of graphitic carbon nitride was effectively enhanced by Na doping (9.2 times). It was found based on comprehensive analysis that, the absorption of visible light was improved due to the structural change of graphitic carbon nitride by Na doping, thereby promoting the generation of more photo-generated carriers. Meanwhile, the separation and transfer of photo-generated carriers were greatly enhanced by coordination of Na into big C-N rings of the triazine units. Moreover, more active sites for photocatalytic H-2-evolution reaction were provided by the increased surface areas. (C) 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

Keyword :

Graphitic carbon nitride Na doping Visible light Photocatalysis One-pot preparation Hydrogen

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GB/T 7714 Zhang, Yazhou , Zong, Shichao , Cheng, Cheng et al. One-pot annealing preparation of Na-doped graphitic carbon nitride from melamine and organometallic sodium salt for enhanced photocatalytic H-2 evolution [C] . 2018 : 13953-13961 .
MLA Zhang, Yazhou et al. "One-pot annealing preparation of Na-doped graphitic carbon nitride from melamine and organometallic sodium salt for enhanced photocatalytic H-2 evolution" . (2018) : 13953-13961 .
APA Zhang, Yazhou , Zong, Shichao , Cheng, Cheng , Shi, Jinwen , Guan, Xiangjiu , Lu, Youjun et al. One-pot annealing preparation of Na-doped graphitic carbon nitride from melamine and organometallic sodium salt for enhanced photocatalytic H-2 evolution . (2018) : 13953-13961 .
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Assessment of sugarcane bagasse gasification in supercritical water for hydrogen production EI CPCI-S SCIE Scopus
会议论文 | 2018 , 43 (30) , 13711-13719 | 8th International Conference on Hydrogen Production (ICH2P)
WoS CC Cited Count: 2
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Abstract :

Sugarcane bagasse is one of the major resources of agricultural biomass waste in the world. In this work, supercritical water gasification characteristics of sugarcane bagasse were investigated. The effect of temperature (600-750 degrees C), concentration (3-12 wt%), residence time (5-20 min) and catalysts (Raney-Ni, K2CO3 and Na2CO3) on bagasse gasification were studied. A kinetic study on the non-catalytic and Na2CO3 catalytic bagasse gasification was conducted to describe the kinetic information of the bagasse gasification reaction. The results showed that a higher reaction temperature, a lower bagasse concentration and a longer residence time could favor the gasification of bagasse, leading to a higher hydrogen yield. Bagasse was nearly completely gasified at 750 degrees C without using any catalyst and the carbon gasification efficiency could reach up to 96.28%. The addition of employed catalysts remarkably promoted the bagasse gasification reactivity. The maximum hydrogen yield (35.3 moVkg) was achieved at 650 degrees C with the Na2CO3 loading of 20 wt%. The experimental data fitted well with a homogeneous model based on a Pseudo first -order reaction hypothesis. The kinetic study showed that Na2CO3 catalyst could lower the activation energy Ea of bagasse gasification from 117.88 kJ/mol to 78.25 kJ/mol. (C) 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

Keyword :

Supercritical water Kinetic study Sugarcane bagasse Hydrogen production catalyst

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GB/T 7714 Cao, Wen , Guo, Liejin , Yan, Xuecheng et al. Assessment of sugarcane bagasse gasification in supercritical water for hydrogen production [C] . 2018 : 13711-13719 .
MLA Cao, Wen et al. "Assessment of sugarcane bagasse gasification in supercritical water for hydrogen production" . (2018) : 13711-13719 .
APA Cao, Wen , Guo, Liejin , Yan, Xuecheng , Zhang, Deming , Yao, Xiangdong . Assessment of sugarcane bagasse gasification in supercritical water for hydrogen production . (2018) : 13711-13719 .
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Different flow fields, operation modes and designs for proton exchange membrane fuel cells with dead-ended anode EI SCIE Scopus
期刊论文 | 2018 , 43 (3) , 1769-1780 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
WoS CC Cited Count: 1 SCOPUS Cited Count: 4
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Abstract :

Water and nitrogen can accumulate in the anode channel in proton exchange membrane fuel cells (PEMFCs) with dead-ended anode (DEA) and can affect cell performance significantly. In this paper, the cell performance characteristics in DEA PEMFCs with three different anode flow fields under two operating modes are studied through measuring the cell voltages and local current densities. The effect of the anode exit reservoir is also studied for the three different anode flow fields. The experimental results show that the interdigitated flow field has the most stable cell performance under both constant pressure and pressure swing supply modes. Parallel and serpentine flow fields lead to very non-uniform local current distributions under constant pressure supply mode and experience severe fluctuations and spikes in local current densities under pressure swing supply mode. The results also show that anode pressure swing supply mode can achieve more stable cell performance than anode constant pressure supply mode for parallel and serpentine anode flow fields. The anode exit reservoir can significantly improve cell performance stability for parallel and serpentine flow fields, but has no significant effect on interdigitated flow fields. Besides, the results further show that PEMFCs with DEA can maintain very stable operation with anode serpentine flow field and an anode exit reservoir under pressure swing operation. (C) 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

Keyword :

Dead-ended anode Reservoir Anode supply mode Flow field PEM fuel cell

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GB/T 7714 Yang, Yupeng , Zhang, Xu , Guo, Liejin et al. Different flow fields, operation modes and designs for proton exchange membrane fuel cells with dead-ended anode [J]. | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2018 , 43 (3) : 1769-1780 .
MLA Yang, Yupeng et al. "Different flow fields, operation modes and designs for proton exchange membrane fuel cells with dead-ended anode" . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 43 . 3 (2018) : 1769-1780 .
APA Yang, Yupeng , Zhang, Xu , Guo, Liejin , Liu, Hongtan . Different flow fields, operation modes and designs for proton exchange membrane fuel cells with dead-ended anode . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2018 , 43 (3) , 1769-1780 .
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Condensation regime diagram for supersonic and subsonic steam jet condensation in water flow in a vertical pipe EI SCIE Scopus
期刊论文 | 2018 , 130 , 62-73 | APPLIED THERMAL ENGINEERING
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Abstract :

An experimental research is performed to investigate the condensation regime diagram of supersonic and subsonic steam jet condensation in water flow in pipes. The original images of the jet plume are recorded using a visualization window and a high-speed camera. The jet condensation regimes are basically categorized into four types, including Chugging, Oscil-I, Oscil-II and Stable regimes, primarily based on the transient evolution of geometrical profile of the jet plume. And the average geometrical shape of the jet plume is found to shrink gradually with increase of ambient pressure. The stand deviation of pressure oscillation is highly correlated to jet condensation regimes, so it can be applied to quantitatively categorize different regimes. The steam mass flux, scaled by critical steam mass flux at different ambient pressure, is found to be irrelevant to the transitional lines among Chugging, Oscil-I, and "Stable or Oscil-II" regimes in the condensation regime diagram. Furthermore, the Oscil-II regime can be simply isolated from the "Stable or Oscil-II" regime via comparison of the standard deviation of pressure oscillation in this two regimes. Therefore, the jet condensation regime diagram obtained from low ambient pressure could be applied to conditions of elevated ambient pressure. (C) 2017 Elsevier Ltd. All rights reserved.

Keyword :

Condensation regime diagram Regime classification Pressure oscillation Supersonic steam jet Multiphase flow

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GB/T 7714 Xu, Qiang , Ye, Shuyan , Chen, Yanshuang et al. Condensation regime diagram for supersonic and subsonic steam jet condensation in water flow in a vertical pipe [J]. | APPLIED THERMAL ENGINEERING , 2018 , 130 : 62-73 .
MLA Xu, Qiang et al. "Condensation regime diagram for supersonic and subsonic steam jet condensation in water flow in a vertical pipe" . | APPLIED THERMAL ENGINEERING 130 (2018) : 62-73 .
APA Xu, Qiang , Ye, Shuyan , Chen, Yanshuang , Chen, Qiyu , Guo, Liejin . Condensation regime diagram for supersonic and subsonic steam jet condensation in water flow in a vertical pipe . | APPLIED THERMAL ENGINEERING , 2018 , 130 , 62-73 .
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Enhanced Photoelectrochemical Water Oxidation on BiVO4 with Mesoporous Cobalt Nitride Sheets as Oxygen-Evolution Cocatalysts SCIE Scopus
期刊论文 | 2018 , (22) , 2557-2563 | EUROPEAN JOURNAL OF INORGANIC CHEMISTRY
WoS CC Cited Count: 2 SCOPUS Cited Count: 3
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Abstract :

A series of cobalt-based oxide and nitride sheet electrocatalysts were developed and then coupled with BiVO4 to investigate the cocatalytic effect and the relationship between electrocatalysis and photoelectrochemical (PEC) water oxidation. The cobalt nitride sheets were synthesized by a hydrothermal method before calcination in ammonia and show superior electrocatalytic activities for oxygen evolution. BiVO4 has been reported to be a desirable candidate among semiconductor materials for photoelectrochemical water splitting except for its sluggish surface oxygen-evolution kinetics. In this work, the PEC performance of BiVO4 was significantly enhanced by efficient oxygen-evolution catalysts serving as cocatalysts. The enhancement of the PEC performance after cocatalyst loading agrees well with the electrocatalytic activities and can be ascribed to the improved surface kinetics. The photocurrent characteristics combined with the results of the electrochemical tests indicate that favourable overpotential and Tafel slope are both important factors in the role of cocatalysts for efficient photoelectrochemical water oxidation. Benefiting from the cocatalytic effect, Co2N0.67-loaded BiVO4 exhibited the highest photocurrent of 2.21 mA/cm(2) at 1.23 V vs. RHE, which is about 80% higher than that of bare BiVO4.

Keyword :

Bismuth Cocatalysts Electrochemistry Cobalt Nitrides Water splitting

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GB/T 7714 Wan, Xiaokang , Su, Jinzhan , Guo, Liejin . Enhanced Photoelectrochemical Water Oxidation on BiVO4 with Mesoporous Cobalt Nitride Sheets as Oxygen-Evolution Cocatalysts [J]. | EUROPEAN JOURNAL OF INORGANIC CHEMISTRY , 2018 , (22) : 2557-2563 .
MLA Wan, Xiaokang et al. "Enhanced Photoelectrochemical Water Oxidation on BiVO4 with Mesoporous Cobalt Nitride Sheets as Oxygen-Evolution Cocatalysts" . | EUROPEAN JOURNAL OF INORGANIC CHEMISTRY 22 (2018) : 2557-2563 .
APA Wan, Xiaokang , Su, Jinzhan , Guo, Liejin . Enhanced Photoelectrochemical Water Oxidation on BiVO4 with Mesoporous Cobalt Nitride Sheets as Oxygen-Evolution Cocatalysts . | EUROPEAN JOURNAL OF INORGANIC CHEMISTRY , 2018 , (22) , 2557-2563 .
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Gasification of unsymmetrical dimethylhydrazine in supercritical water: Reaction pathway and kinetics EI SCIE Scopus
期刊论文 | 2018 , 43 (18) , 8644-8654 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
SCOPUS Cited Count: 2
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Unsymmetrical dimethylhydrazine (UDMH) is a high N-containing (as much as nearly 50%) substance. Traditional treatment methods such as incineration will inevitably cause the formation of nitric oxide and secondary pollution. Supercritical water is a preferred transformation medium due to its unique physicochemical properties. However, at present most of studies are limited to supercritical water oxidation (SCWO) which tends to produce hydrogen nitrate resulting in corrosion to the reactor. To conquer this problem, we propose supercritical water gasification (SCWG) technology which is in a reducing environment, realizing both harmless treatment and resource utilization. In order to promote its industrialization process, the reaction pathways and kinetic parameters should be studied. In this paper, the reaction pathways and kinetics of UDMH in supercritical water were conducted under the conditions of 400 C-degrees-550 C-degrees in quartz reactor, which avoids the catalytic effect on the reaction kinetics. From the resource utilization perspective, the most abundant quantitatively detectable gaseous product is methane, together with less hydrogen, carbon monoxide and ethane orderly. All these gaseous products are combustible. The maximum of carbon efficiency is 90.25% at 550 C-degrees, 10 min. In the point of view of harmless treatment, the organic compounds contained in the residual liquid are detected with H-1 NMR, FTIR and GC/MS. Results show that UDMH could be fully degraded within 3 min and the ultimate organic compounds in the residual liquid are mainly dimethylamino acetonitrile and trimethylamine. In addition, a reaction pathway for UDMH disposed in supercritical water is developed. Finally, the quantitative kinetic model for describing the gaseous products and ammonia-nitrogen in the residual liquid is brought forward. The pyrolysis activation energy for UDMH in supercritical water is 49.98 +/- 7.38 kJ/mol. (C) 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

Keyword :

SCWG Kinetics Harmless treatment UDMH Reaction pathway Resource utilization

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GB/T 7714 Yi, Lei , Guo, Liejin , Jin, Hui et al. Gasification of unsymmetrical dimethylhydrazine in supercritical water: Reaction pathway and kinetics [J]. | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2018 , 43 (18) : 8644-8654 .
MLA Yi, Lei et al. "Gasification of unsymmetrical dimethylhydrazine in supercritical water: Reaction pathway and kinetics" . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 43 . 18 (2018) : 8644-8654 .
APA Yi, Lei , Guo, Liejin , Jin, Hui , Kou, Jiajing , Zhang, Deming , Wang, Runyu . Gasification of unsymmetrical dimethylhydrazine in supercritical water: Reaction pathway and kinetics . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2018 , 43 (18) , 8644-8654 .
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Facet-Selective Growth of Cadmium Sulfide Nanorods on Zinc Oxide Microrods: Intergrowth Effect for Improved Photocatalytic Performance EI SCIE Scopus
期刊论文 | 2018 , 10 (1) , 153-158 | CHEMCATCHEM
WoS CC Cited Count: 2 SCOPUS Cited Count: 3
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Abstract :

Well-designed architectures play an important role in accelerating charge transfer between the different components of hybrid photocatalysts. Herein, we report a simple one-step hydrothermal method to achieve a CdS/ZnO heterostructure with a novel spatial arrangement. The CdS nanorods were found to be attached to the surface of the ZnO microrods with an intimate face-to-face contact, and the heterointerfaces corresponded to {100} facets of CdS and {100} facets of ZnO. It was discovered that Zn(OH)(2) intermediates were formed at first and then grew into hexagonal ZnO microrods through a solid-solid-phase transformation. Simultaneously, CdS nuclei grew to nanorods on the {100} facets of ZnO by oriented attachment during the one-step hydrothermal process. Under visible-light irradiation, obtained CdS/ZnO exhibited enhanced photocatalytic hydrogen generation owing to improved charge separation from the two-phase intergrowth effect. This work provides a facile hydrothermal route to construct intergrown heterostructures with desired spatial arrangements for improved photocatalytic properties.

Keyword :

nanostructures ZnO facet selective CdS photocatalysis heterostructures

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GB/T 7714 Guo, Xu , Chen, Yubin , Qin, Zhixiao et al. Facet-Selective Growth of Cadmium Sulfide Nanorods on Zinc Oxide Microrods: Intergrowth Effect for Improved Photocatalytic Performance [J]. | CHEMCATCHEM , 2018 , 10 (1) : 153-158 .
MLA Guo, Xu et al. "Facet-Selective Growth of Cadmium Sulfide Nanorods on Zinc Oxide Microrods: Intergrowth Effect for Improved Photocatalytic Performance" . | CHEMCATCHEM 10 . 1 (2018) : 153-158 .
APA Guo, Xu , Chen, Yubin , Qin, Zhixiao , Su, Jinzhan , Guo, Liejin . Facet-Selective Growth of Cadmium Sulfide Nanorods on Zinc Oxide Microrods: Intergrowth Effect for Improved Photocatalytic Performance . | CHEMCATCHEM , 2018 , 10 (1) , 153-158 .
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