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学者姓名:王树众

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< Page ,Total 66 >
Supercritical water oxidation of quinoline with moderate preheat temperature and initial concentration EI Scopus SCIE
期刊论文 | 2019 , 236 , 1408-1414 | Fuel
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Abstract :

This work reports an experimental study on supercritical water oxidation of quinoline. Moderate preheat temperature (420 °C–510 °C) and initial concentration (1 wt%–10 wt%) are selected to address the possibility of utilizing the heat released during the reaction, in order to realize high conversion rate at relatively low preheat temperature. The effects of temperature, residence time, oxidation ratio, pressure and concentration are analyzed. The results show that considerable conversion can happen at relatively low preheat temperature, while increase in temperature will significantly promote the complete conversion. The yield of carbon dioxide increases with the residence time but there is an upper limit due to the stronger dependence on oxidizer concentration, for which an estimated reaction order is 1.90. When the quinoline concentration is larger than 8 wt%, clear exothermic peaks with temperature rise about 100 °C are detected. These exothermic peaks can be interpreted as a sign of ignition interrupted by the heat loss to the surrounding salt bath. An analogy is made between the start temperatures of these exothermic peaks and the ignition temperatures reported in methanol and isopropanol hydrothermal flame research. We conclude that quinoline solutions can be ignited without co-fuels, at comparable ignition temperature as methanol and isopropanol around 450 °C. © 2018 Elsevier Ltd

Keyword :

Heat release Initial concentration Preheat temperature Quinoline Supercritical water oxidation

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GB/T 7714 Ren, Mengmeng , Wang, Shuzhong , Yang, Chuang et al. Supercritical water oxidation of quinoline with moderate preheat temperature and initial concentration [J]. | Fuel , 2019 , 236 : 1408-1414 .
MLA Ren, Mengmeng et al. "Supercritical water oxidation of quinoline with moderate preheat temperature and initial concentration" . | Fuel 236 (2019) : 1408-1414 .
APA Ren, Mengmeng , Wang, Shuzhong , Yang, Chuang , Xu, Haitao , Guo, Yang , Roekaerts, Dirk . Supercritical water oxidation of quinoline with moderate preheat temperature and initial concentration . | Fuel , 2019 , 236 , 1408-1414 .
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Supercritical CO2-water-shale interactions and their effects on element mobilization and shale pore structure during stimulation EI
期刊论文 | 2019 , 202 , 109-127 | International Journal of Coal Geology
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Abstract :

There are many advantages to using supercritical carbon dioxide (ScCO2) fracturing technology to exploit shale gas reservoirs in China, including minimal damage to the environment or formation, and displacing methane (CH4) in the adsorbed state. When ScCO2 enters fractures in the formation, ScCO2-water-shale interactions may affect the physicochemical properties of shale. In this study, a high-pressure reaction system was adopted to simulate ScCO2-water-shale interactions under ScCO2 stimulation conditions. The element mobilization and pore structure before and after the reaction were measured using ICP-MS, XRF. The results show that the major elements, including Ca, Mg, Na, K, and Al, exhibit varying degrees of mobilization after the interactions because of dissolution of carbonate and silicate minerals in shale samples. Compared with the major elements, trace elements have a lower mobility, quantified as <13.97%. The specific surface areas and pore volumes of two shale samples increase at different degrees after the reaction. The interactions have a more significant influence on the micropores. In addition, fractal features of the shale pore structure were analyzed. The fractal dimensions of the shale samples increase after the reaction, indicating that pore surface roughness increases, and pore structure morphology gradually transforms from regular to complex. © 2018 Elsevier B.V.

Keyword :

Element mobilization Fractal feature Major elements Minimal damage Physicochemical property Shale gas reservoirs Supercritical carbon dioxides Supercritical CO2

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GB/T 7714 Luo, Xiangrong , Ren, Xiaojuan , Wang, Shuzhong . Supercritical CO2-water-shale interactions and their effects on element mobilization and shale pore structure during stimulation [J]. | International Journal of Coal Geology , 2019 , 202 : 109-127 .
MLA Luo, Xiangrong et al. "Supercritical CO2-water-shale interactions and their effects on element mobilization and shale pore structure during stimulation" . | International Journal of Coal Geology 202 (2019) : 109-127 .
APA Luo, Xiangrong , Ren, Xiaojuan , Wang, Shuzhong . Supercritical CO2-water-shale interactions and their effects on element mobilization and shale pore structure during stimulation . | International Journal of Coal Geology , 2019 , 202 , 109-127 .
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Effect Mechanism of Auxiliary Fuel in Supercritical Water: A Review SCIE
期刊论文 | 2019 , 58 (4) , 1480-1494 | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
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Abstract :

Supercritical water oxidation is a promising alternative for treatment of wastewater and sludge. The addition of auxiliary fuel can achieve the optimization of the system. Owing to the discrepancy in the fuel parameter and reaction condition, the auxiliary fuel presents two different behavior mechanisms in supercritical water, co-oxidation and hydrothermal combustion. The process mechanism, kinetics analysis, and effect behavior for these two processes were systematically reviewed in this work. The co-oxidation between auxiliary fuel compounds, such as methanol, ethanol, isopropyl alcohol, etc. and ammonia, polychlorinated biphenyls was analyzed, and the mixing kinetics models and mechanism investigation approaches were summerized. Besides, the process analysis, kinetics model, and interaction during the supercritical hydrothermal combustion with higher concentration of auxiliary fuel were discussed. Finally, a supercritical water oxidation system with optimized auxiliary fuel was proposed and evaluated by the mechanism-based kinetics simulation, and further research needs were put forward.

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GB/T 7714 Zhang, Jie , Wang, Shuzhong , Ren, Mengmeng et al. Effect Mechanism of Auxiliary Fuel in Supercritical Water: A Review [J]. | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH , 2019 , 58 (4) : 1480-1494 .
MLA Zhang, Jie et al. "Effect Mechanism of Auxiliary Fuel in Supercritical Water: A Review" . | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 58 . 4 (2019) : 1480-1494 .
APA Zhang, Jie , Wang, Shuzhong , Ren, Mengmeng , Lu, Jinling , Chen, Senlin , Zhang, Huamin . Effect Mechanism of Auxiliary Fuel in Supercritical Water: A Review . | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH , 2019 , 58 (4) , 1480-1494 .
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Catalytic performances of Ni-based catalysts on supercritical water gasification of phenol solution and coal-gasification wastewater SCIE
期刊论文 | 2019 , 44 (7) , 3470-3480 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
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Abstract :

Activity and stability of the supported Ni-based catalysts for the gasification performances of phenol solution and coal-gasification wastewater in supercritical water were studied in a continuous reactor at 480 degrees C, 25 MPa and oxygen ratio of 0.2 for 50 h operation. The in- fluences of the supports (gamma-Al2O3, active carbon (AC) and carbon nanotube (CNT)) on gas yields, gasification efficiencies for phenol solution were investigated, and the loading amount of Ni were optimized. Results showed that the catalytic activity and the stability of the catalysts followed the order of Ni/CNT > Ni/AC > Ni/gamma-Al2O3. The activity of Ni/AC and Ni/gamma-Al(2)O(3 )decreased after 30 h continuous operation, and there occurred significant leaching of Ni2+. For Ni/CNT catalyst, H-2 yield increased obviously when the loading amount of Ni lower than 15 wt%, while increased little at higher loading amount. Then, 15 wt% Ni/CNT with a thickness of 1.5 mm was coated on 316 L stainless steel (SS316L, an economic material usually used as the reactor material), which can act as a "catalytic tube wall" in reactor. The catalytic activity and corrosion resistance of Ni/CNT/SS316L for the gasification of real coal-gasification wastewater were studied. Results showed that Ni/CNT/SS316L gave a great positive effect on H-2 production. H-2 yield increased from 25.36 mmol/g (total organic carbon) without catalyst to 75.12 mmol/g (total organic carbon) with Ni/CNT/ SS316L after operated for 20 h, respectively. However, obvious pealing of the coating was found after 50 h operation. Further study is necessary for the improvement of the coating preparation method. (C) 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

Keyword :

Ni Phenol Supercritical water gasification Catalyst Coal-gasification wastewater

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GB/T 7714 Wang, Yuzhen , Zhu, Yitong , Liu, Zhuan et al. Catalytic performances of Ni-based catalysts on supercritical water gasification of phenol solution and coal-gasification wastewater [J]. | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2019 , 44 (7) : 3470-3480 .
MLA Wang, Yuzhen et al. "Catalytic performances of Ni-based catalysts on supercritical water gasification of phenol solution and coal-gasification wastewater" . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 44 . 7 (2019) : 3470-3480 .
APA Wang, Yuzhen , Zhu, Yitong , Liu, Zhuan , Wang, Laibin , Xu, Donghai , Fang, Changqing et al. Catalytic performances of Ni-based catalysts on supercritical water gasification of phenol solution and coal-gasification wastewater . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2019 , 44 (7) , 3470-3480 .
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Experimental study on convection heat-transfer characteristics of BCG-CO2 fracturing fluid EI SCIE Scopus
期刊论文 | 2018 , 160 , 258-266 | JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING
SCOPUS Cited Count: 1
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Abstract :

A BCG-CO2 fracturing fluid system is especially suitable for shale gas stimulation because it has many advantages, including minimizing water consumption, reducing damage to the formation, and recovering more rapidly and efficiently. A major objective of this experimental study is to ascertain the convection heat-transfer characteristics of a BCG-CO2 fracturing fluid system. A high-parameter foam fracturing fluid test system was adopted in this study. The measurement of convection heat transfer is based on the double-wall heat-transfer theory. Through experimental research, the correlations for BCG-CO2 fracturing fluid convection heat transfer have been obtained under different foam qualities. The average error of the fitting formula for all experimental data is 10.7%. The results indicate that the convection heat-transfer coefficient decreases with increasing temperature, with an average decrease of about 10%. The convection heat-transfer coefficient shows a decreasing trend with increasing foam quality. There is a linear relationship between the convection heat-transfer coefficient and shear rate, and the shear rate has the most pronounced effect on convection heat-transfer characteristics. The results of this study can be used to calculate heat-transfer parameters to determine the temperature field of BCG-CO2 fracturing fluid flow in fracturing design, and they are significant for the engineering application of BCG-CO2 fracturing fluid.

Keyword :

Foam quality Shear rate BCG-CO2 fracturing fluid Heat transfer

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GB/T 7714 Luo, Xiangrong , Ren, Xiaojuan , Wang, Shuzhong et al. Experimental study on convection heat-transfer characteristics of BCG-CO2 fracturing fluid [J]. | JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING , 2018 , 160 : 258-266 .
MLA Luo, Xiangrong et al. "Experimental study on convection heat-transfer characteristics of BCG-CO2 fracturing fluid" . | JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING 160 (2018) : 258-266 .
APA Luo, Xiangrong , Ren, Xiaojuan , Wang, Shuzhong , Li, Xiaoxiao , Ma, Huanhuan , Liu, Yuyan . Experimental study on convection heat-transfer characteristics of BCG-CO2 fracturing fluid . | JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING , 2018 , 160 , 258-266 .
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Review of hydrogen production using chemical-looping technology EI SCIE Scopus
期刊论文 | 2018 , 81 , 3186-3214 | RENEWABLE & SUSTAINABLE ENERGY REVIEWS
WoS CC Cited Count: 22 SCOPUS Cited Count: 31
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Abstract :

Hydrogen is an attractive energy carrier due to its potentially high energy efficiency and low generation of pollutants, which can be used for transportation and stationary power generation. However, hydrogen is not readily available in sufficient quantities and the production cost is still high. Steam methane reforming (SMR) process is now the most widely used technology for H-2 production, but this process is complex and cannot get thorough carbon capture. Hydrogen production using chemical looping technology has received a great deal of attention in recent years because it can produce hydrogen with higher process efficiency and can capture carbon dioxide. Many researchers have carried out intensive research work on the hydrogen production processes using chemical looping technology. Based on the previous studies stated in the literature, the authors try to give an overview on the recent advances of two categories, chemical looping reforming (CLR) and chemical looping hydrogen production (CLH) processes. Besides, the characteristics of the processes are pointed out based on the comparison with the conventional SMR process. The existing technical problems and the aspects of future research of each approach are also summarized.

Keyword :

Chemical-looping Oxygen carrier Hydrogen CO2 capture

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GB/T 7714 Luo, Ming , Yi, Yang , Wang, Shuzhong et al. Review of hydrogen production using chemical-looping technology [J]. | RENEWABLE & SUSTAINABLE ENERGY REVIEWS , 2018 , 81 : 3186-3214 .
MLA Luo, Ming et al. "Review of hydrogen production using chemical-looping technology" . | RENEWABLE & SUSTAINABLE ENERGY REVIEWS 81 (2018) : 3186-3214 .
APA Luo, Ming , Yi, Yang , Wang, Shuzhong , Wang, Zhuliang , Du, Min , Pan, Jianfeng et al. Review of hydrogen production using chemical-looping technology . | RENEWABLE & SUSTAINABLE ENERGY REVIEWS , 2018 , 81 , 3186-3214 .
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Oxidative degradation of landfill leachate by catalysis of CeMnOx/TiO2 in supercritical water: Mechanism and kinetic study EI SCIE Scopus
期刊论文 | 2018 , 331 , 578-586 | CHEMICAL ENGINEERING JOURNAL
WoS CC Cited Count: 1 SCOPUS Cited Count: 7
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Abstract :

Landfill leachate is a typical refractory wastewater that contains high concentration of organic pollutants. In this work, we investigated the treatment of landfill leachate by supercritical water oxidation (SCWO) in a batch reactor. The effects of temperature (T, 450-600 degrees C), oxidation coefficient (OC, 1.2-3.4), reaction time (t, 60-600 s) and pH (4.13-8.05) on total organic carbon (TOC) removal efficiency (TRE,%) and ammonia nitrogen (NH3-N) removal efficiency (NRE,%) were analyzed. TRE and NRE increased remarkably with increasing temperature and OC. At 3.4 OC and 600 degrees C, 92.5% TRE and 50.9% NRE were achieved after 600 s. A modified kinetic model on TRE and NRE considering the induction time was developed and accurately correlated the experimental results. A significant co-oxidation effect of methanol and landfill leachate in SCWO was detected. Furthermore, heterogeneous catalysts were added to SCWO of landfill leachate to improve the removal rate of organic contaminants. A series of composite catalysts (CeMnOx/TiO2) which consisted of the cerium, manganese and titanium oxides were prepared by impregnation method with varying Ce/Mn ratio. Compared with the SCWO of leachate without catalyst, the CeMnOx/TiO2 catalyst with Ce/Mn ratio of 1: 2 exhibited high catalytic activity and stability. Additionally, a catalytic reaction mechanism was proposed. It was assumed that MnOx is the active component and CeO2 is the additive and oxygen supplier. The results obtained from this work suggest the SCWO with high-efficiency and stable catalyst could be a promising technology for landfill leachate treatment.

Keyword :

Co-oxidation Kinetics Supercritical water oxidation Landfill leachate Catalyst

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GB/T 7714 Gong, Yanmeng , Guo, Yang , Sheehan, James D. et al. Oxidative degradation of landfill leachate by catalysis of CeMnOx/TiO2 in supercritical water: Mechanism and kinetic study [J]. | CHEMICAL ENGINEERING JOURNAL , 2018 , 331 : 578-586 .
MLA Gong, Yanmeng et al. "Oxidative degradation of landfill leachate by catalysis of CeMnOx/TiO2 in supercritical water: Mechanism and kinetic study" . | CHEMICAL ENGINEERING JOURNAL 331 (2018) : 578-586 .
APA Gong, Yanmeng , Guo, Yang , Sheehan, James D. , Chen, Zhifeng , Wang, Shuzhong . Oxidative degradation of landfill leachate by catalysis of CeMnOx/TiO2 in supercritical water: Mechanism and kinetic study . | CHEMICAL ENGINEERING JOURNAL , 2018 , 331 , 578-586 .
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Effect of low oxygen concentration on the oxidation behavior of Ni-based alloys 625 and 825 in supercritical water EI SCIE Scopus
期刊论文 | 2018 , 131 , 1-10 | JOURNAL OF SUPERCRITICAL FLUIDS
WoS CC Cited Count: 2 SCOPUS Cited Count: 7
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In this study, the oxidation behavior of Ni-based alloys 625 and 825 in supercritical water containing 5000 ppm of dissolved oxygen at 500 degrees C was investigated by scanning electron microscopy coupled with energy-dispersive spectroscopy, X-ray diffraction, and laser Raman spectroscopy. Alloy 625 and 825 showed a pitting-like phenomenon after 500 h of exposure. The structure and composition of the oxides formed on alloy 625 and 825 were similar, namely, an outer layer of Fe oxides, spinel structures, and Ni(OH)(2); and an inner NiO layer. The mechanism for the formation of the oxide films was proposed, and the factors affecting corrosion of Ni-based alloys were discussed in detail. In addition, the corrosion resistance performance of alloy 625 and 825 was compared.

Keyword :

Supercritical water oxidation XRD Oxygen concentration Ni-based alloys SEM LAS

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GB/T 7714 Yang, Jianqiao , Wang, Shuzhong , Tang, Xingying et al. Effect of low oxygen concentration on the oxidation behavior of Ni-based alloys 625 and 825 in supercritical water [J]. | JOURNAL OF SUPERCRITICAL FLUIDS , 2018 , 131 : 1-10 .
MLA Yang, Jianqiao et al. "Effect of low oxygen concentration on the oxidation behavior of Ni-based alloys 625 and 825 in supercritical water" . | JOURNAL OF SUPERCRITICAL FLUIDS 131 (2018) : 1-10 .
APA Yang, Jianqiao , Wang, Shuzhong , Tang, Xingying , Wang, Yuzhen , Li, Yanhui . Effect of low oxygen concentration on the oxidation behavior of Ni-based alloys 625 and 825 in supercritical water . | JOURNAL OF SUPERCRITICAL FLUIDS , 2018 , 131 , 1-10 .
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Simulation of a Transpiring Wall Reactor for Supercritical Water Oxidation: Characteristics of Water Film EI SCIE Scopus
期刊论文 | 2018 , 57 (4) , 1307-1318 | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
WoS CC Cited Count: 1 SCOPUS Cited Count: 1
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Abstract :

Reactor corrosion and plugging problems severely hinder commercial application of supercritical water oxidation. A transpiring wall reactor can overcome these two problems by forming a protective water film on the inner surface of a porous transpiring wall to isolate corrosive substances and inorganic salt. This work proposed water film coverage rate and inorganic salt concentration in water film as evaluation indexes of water film characteristics. A computational fluid dynamics model of a new transpiring wall reactor was built to explore the characteristics of water film under key operating parameter conditions by numerical simulation together with experiment validations. The results show that water film coverage rate raised either with transpiration intensity and transpiration water temperature increasing or with feedstock flow rate and feedstock preheating temperature decreasing. Inorganic salt concentration in water film declined as transpiration intensity and transpiration length increased. Two equations were proposed to guide the optimization of reactor operating parameters.

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GB/T 7714 Xu, Donghai , Guo, Shuwei , He, Zhen et al. Simulation of a Transpiring Wall Reactor for Supercritical Water Oxidation: Characteristics of Water Film [J]. | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH , 2018 , 57 (4) : 1307-1318 .
MLA Xu, Donghai et al. "Simulation of a Transpiring Wall Reactor for Supercritical Water Oxidation: Characteristics of Water Film" . | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 57 . 4 (2018) : 1307-1318 .
APA Xu, Donghai , Guo, Shuwei , He, Zhen , Huang, Chuanbao , Jing, Zefeng , Wan, Shuzhong . Simulation of a Transpiring Wall Reactor for Supercritical Water Oxidation: Characteristics of Water Film . | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH , 2018 , 57 (4) , 1307-1318 .
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Ni-Ru/CeO2 Catalytic Hydrothermal Upgrading of Water-Insoluble Biocrude from Algae Hydrothermal Liquefaction SCIE PubMed Scopus
期刊论文 | 2018 | BIOMED RESEARCH INTERNATIONAL
SCOPUS Cited Count: 1
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Hydrothermal liquefaction (HTL) of algae is a promising crude bio-oil (biocrude) production technology, which can convert wet algae into water-insoluble biocrude and other coproducts. In this work, algae HTL at 350 degrees C and 20 min was conducted to obtain water-insoluble biocrude (B-1), which was then hydrothermally upgraded at 450 degrees C, 60 min, or with added H-2 and/or homemade catalyst (i.e., Ni-Ru/CeO2 or Ni/CeO2) for the first time. The characteristics (e.g., yield, elemental component, energy recovery, and molecular and functional group compositions) of upgraded water-insoluble biocrude (B-2) as well as light biocrude thereof were analyzed comprehensively. The results show that Ni-Ru/CeO2+H-2 led to the highest yield and HHV (higher heating value), the best elemental compositions quality of B-2, and the largest fraction and the best light of light biocrude in B-2. Ni-Ru/CeO2+H-2 had good catalytic desulfurization effect and could transform high-molecular-weight compounds into low-molecular-weight compounds in B-1 upgrading. At the condition above, 46.2% of chemical energy in the initial algae could be recovered by B-2, while average 54.9% of chemical energy in B-2 was distributed in its light biocrude (hexane-soluble) portion. On the whole, Ni-Ru/CeO2+H-2 can be considered as the optimal additive in all tested cases.

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GB/T 7714 Xu, Donghai , Guo, Shuwei , Liu, Liang et al. Ni-Ru/CeO2 Catalytic Hydrothermal Upgrading of Water-Insoluble Biocrude from Algae Hydrothermal Liquefaction [J]. | BIOMED RESEARCH INTERNATIONAL , 2018 .
MLA Xu, Donghai et al. "Ni-Ru/CeO2 Catalytic Hydrothermal Upgrading of Water-Insoluble Biocrude from Algae Hydrothermal Liquefaction" . | BIOMED RESEARCH INTERNATIONAL (2018) .
APA Xu, Donghai , Guo, Shuwei , Liu, Liang , Hua, Hui , Guo, Yang , Wang, Shuzhong et al. Ni-Ru/CeO2 Catalytic Hydrothermal Upgrading of Water-Insoluble Biocrude from Algae Hydrothermal Liquefaction . | BIOMED RESEARCH INTERNATIONAL , 2018 .
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