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学者姓名:黄佐华

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Experimental Study of Hypergolic Process of Ionic Liquids with BH3(CN)BH2(CN)- Anion EI Scopus CSCD PKU
期刊论文 | 2018 , 26 (7) , 557-564 | Hanneng Cailiao/Chinese Journal of Energetic Materials
SCOPUS Cited Count: 1
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Abstract :

The reactions of 8 newly synthesized ionic liquids containing BH3(CN)BH2(CN)- anion, (I.L.1~ I.L.8), with white fuming nitric acid (WFNA) and red fuming nitric acid (RFNA ) respectively were tested by using the long focus microscope-high speed photography technique and droplet method test device, respectively. Results show that each test achieves stable hypergolic reaction and two different flame development processes were observed. Specifically, after the contact of I.L.8 with WFNA, the microexplosion is occurred and hypergolic ignition is occurred in a short time, while after the contact of I.L.8 with RFNA the aplashing of secondary droplet is occurred. Due to the effect of Leiden Frost effect, the foam like droplets after reaction is rebounded and a short combustion reaction is appeared, the hypergolic ignition is occurred after a long time. For the ionic liquid with same heterocyclic core, the ignition delay time of the ionic liquid containing the allyl group on the side chain is the shortest, followed by the ionic liquid containing ethyl, while the ignition delay time of the ionic liquid containing butyl and WFNA is the longest. For the ionic liquid with the same side chain, the ignition delay time of the ionic liquid containing the pyridine heterocyclic ring is the longest, followed by the imidazole heterocyclic ionic liquid, and the ignition delay time of the ionic liquid containing tetrahydropyrrole reacted with WFNA is the longest.The higher the enthalpy of formation is, the shorter the ignition delay time is. © 2018, Editorial Board of Chinese Journal of Energetic Materials. All right reserved.

Keyword :

Combustion reactions Enthalpy of formation Fuming nitric acids Heterocyclic rings High-speed photography technique Hypergolic ignitions Ignition delay time Ignition delays

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GB/T 7714 Weng, Xin-Yan , Du, Zong-Gang , Yu, Jun et al. Experimental Study of Hypergolic Process of Ionic Liquids with BH3(CN)BH2(CN)- Anion [J]. | Hanneng Cailiao/Chinese Journal of Energetic Materials , 2018 , 26 (7) : 557-564 .
MLA Weng, Xin-Yan et al. "Experimental Study of Hypergolic Process of Ionic Liquids with BH3(CN)BH2(CN)- Anion" . | Hanneng Cailiao/Chinese Journal of Energetic Materials 26 . 7 (2018) : 557-564 .
APA Weng, Xin-Yan , Du, Zong-Gang , Yu, Jun , Tong, Shang-Qing , Li, Jian-Ling , Zhang, Qing-Hua et al. Experimental Study of Hypergolic Process of Ionic Liquids with BH3(CN)BH2(CN)- Anion . | Hanneng Cailiao/Chinese Journal of Energetic Materials , 2018 , 26 (7) , 557-564 .
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可控流场尺度预混湍流燃烧器及其火焰结构分析 CSCD PKU
期刊论文 | 2018 , (2) , 10-17 | 实验流体力学
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Abstract :

为了研究单一湍流场参数对预混湍流火焰结构的影响,以及拓宽湍流场的强度和尺度范围,发展了一套可变结构的预混湍流燃烧器.采用恒温型热线风速仪标定流场,得到了一系列湍流参数.流场标定结果表明:该燃烧器能显著拓宽湍流强度和尺度范围,并能利用不同几何结构产生多种可控流场,实现研究单一湍流参数对湍流燃烧速度和火焰结构影响的目的.选用有代表性的15种湍流孔板组合结构,利用OH-PLIF燃烧激光诊断技术,开展了湍流燃烧实验,结果表明:湍流强度的增大(1<u'/SL.0<10)使得湍流火焰分区扩展到了薄层反应区,火焰面破碎程度明显增强,孤岛结构明显增多.高宏观雷诺数下,积分尺度的增长对湍流燃烧速度起抑制作用,可能存在临界宏观雷诺数Rec,能够表现流体惯性力占主导地位的程度,决定积分尺度对湍流燃烧速度的影响效果.积分尺度能量大,扰动能力强,故积分尺度越大,火焰体积越大;但过高的湍流强度会使火焰面褶皱更加剧烈,小尺度叠加在大尺度上的程度增强,最终也使火焰体积显著增大,掩盖了积分尺度对火焰体积的影响,说明积分尺度(表征大尺度)不如湍流强度(表征叠加小尺度的程度)对火焰放热率影响大.

Keyword :

湍流强度 火焰体积 湍流尺度 预混湍流燃烧 湍流燃烧速度

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GB/T 7714 余芊芊 , 王金华 , 张玮杰 et al. 可控流场尺度预混湍流燃烧器及其火焰结构分析 [J]. | 实验流体力学 , 2018 , (2) : 10-17 .
MLA 余芊芊 et al. "可控流场尺度预混湍流燃烧器及其火焰结构分析" . | 实验流体力学 2 (2018) : 10-17 .
APA 余芊芊 , 王金华 , 张玮杰 , 张猛 , 黄佐华 . 可控流场尺度预混湍流燃烧器及其火焰结构分析 . | 实验流体力学 , 2018 , (2) , 10-17 .
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预混湍流火焰面褶皱结构网络拓扑研究 CSCD PKU
期刊论文 | 2018 , (1) , 19-25,63 | 实验流体力学
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Abstract :

湍流火焰结构是表征湍流与火焰相互作用的组分、速度、温度等标量场信息,理解湍流与火焰相互作用规律,验证和发展湍流燃烧模型的实验基础.针对传统曲率PDF分布反映湍流火焰面褶皱结构失准问题,利用网络拓扑结构方法可以标记系统关键节点和特征结构,构建湍流火焰面的拓扑结构.本文标记了湍流火焰面上的关键褶皱结构,分析了湍流与火焰的作用规律,结果表明:低湍流强度下,湍流火焰面的关键褶皱结构由火焰自身不稳定性引起;当湍流强度增大,湍流火焰面的关键褶皱结构由湍流尺度决定.在本生灯湍流火焰中,火焰自身不稳定性引起的火焰褶皱与火焰发展距离有关.在本生灯火焰底部,火焰自身不稳定性不引起火焰面褶皱,随着火焰向下游发展,其对火焰面影响逐渐增大,火焰褶皱程度增加.

Keyword :

褶皱结构 火焰不稳定 预混湍流火焰 网络拓扑分析 曲率PDF分布

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GB/T 7714 王金华 , 聂要辉 , 常敏 et al. 预混湍流火焰面褶皱结构网络拓扑研究 [J]. | 实验流体力学 , 2018 , (1) : 19-25,63 .
MLA 王金华 et al. "预混湍流火焰面褶皱结构网络拓扑研究" . | 实验流体力学 1 (2018) : 19-25,63 .
APA 王金华 , 聂要辉 , 常敏 , 张猛 , 黄佐华 . 预混湍流火焰面褶皱结构网络拓扑研究 . | 实验流体力学 , 2018 , (1) , 19-25,63 .
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Experimental and kinetic study of pentene isomers and n-pentane in laminar flames EI SCIE Scopus
期刊论文 | 2017 , 36 (1) , 1279-1286 | PROCEEDINGS OF THE COMBUSTION INSTITUTE | IF: 5.336
WoS CC Cited Count: 8 SCOPUS Cited Count: 11
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Abstract :

Laminar flame speeds of three pentene isomers (1-pentene, 2-pentene and 2-methyl-2-butene) and n-pentane are investigated at equivalence ratios of 0.7-1.6, initial pressures of 1-4 atm, and initial temperatures of 353-433 K using a constant volume combustion bomb. Results show that the laminar flame speeds increase in the order of 2-methyl-2-butene, n -pentane, 2-pentene, and 1-pentene. A recently published model on pentane isomers (NUI-PI) has been optimized by refining the submodels of the 1-pentene and 2-methyl-2-butene. This optimized model yields reasonable agreement with the experimental data except over-predictions for 2-pentene. The analysis indicates the discrepancy of laminar flame speeds between 1-pentene and n -pentane is mainly caused by the thermal effect, different from the discrepancy between 1-pentene and 2-methyl-2-butene which mainly results from the chemical kinetic effect. The kinetic effect is further investigated employing the sensitivity and reaction path analyses. The analyses reveal that 1-pentene generates the H-radical precursor ethyl radical, while 2-methyl-2-butene produces large amount of the H-consuming branching intermediates (IC4H8, AC(5)H(9)-C, CC5H9-B and B13DE2MJ) and presents the weaker H regenerating ability. In addition, compared with 1-pentene, 2-methyl-2-butene yields larger amount of methyl radical which would block the whole reaction process. (C) 2016 by The Combustion Institute. Published by Elsevier Inc.

Keyword :

Chemical kinetics Pentene isomers Laminar flame speed n-Pentane

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GB/T 7714 Cheng, Yu , Hu, Erjiang , Lu, Xin et al. Experimental and kinetic study of pentene isomers and n-pentane in laminar flames [J]. | PROCEEDINGS OF THE COMBUSTION INSTITUTE , 2017 , 36 (1) : 1279-1286 .
MLA Cheng, Yu et al. "Experimental and kinetic study of pentene isomers and n-pentane in laminar flames" . | PROCEEDINGS OF THE COMBUSTION INSTITUTE 36 . 1 (2017) : 1279-1286 .
APA Cheng, Yu , Hu, Erjiang , Lu, Xin , Li, Xiaotian , Gong, Jing , Li, Qianqian et al. Experimental and kinetic study of pentene isomers and n-pentane in laminar flames . | PROCEEDINGS OF THE COMBUSTION INSTITUTE , 2017 , 36 (1) , 1279-1286 .
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Ignition delay times of low alkylfurans at high pressures using a rapid compression machine EI SCIE Scopus
期刊论文 | 2017 , 36 (1) , 323-332 | PROCEEDINGS OF THE COMBUSTION INSTITUTE | IF: 5.336
WoS CC Cited Count: 4 SCOPUS Cited Count: 4
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Abstract :

Auto-ignition behavior of 2-ethylfuran (EF) was investigated in the low to intermediate temperature range (766-1013 K) over equivalence ratios of 0.5, 1.0, and 2.0 at 16 and 30 bar using a rapid compression machine. Equivalence ratio was varied by changing the mole fractions of O-2 while fixing the fuel fraction. The fuel did not show "negative temperature coefficient (NTC)" or two stage ignition behavior in the present measuring range. Simulations were conducted on the basis of the alkylfuran mechanism of Somers et al. (2013) [1], in which the EF sub-mechanism is not fully developed. Optimization of the EF sub-mechanism was attempted. Results show that the modified mechanism shows better agreement with our measurements and other data in the literature. Comparison of the reactivity of EF with that of 2-methyl furan (MF) and 2, 5-dimethyl furan (DMF) under various equivalence ratios was conducted and results show that the relative reactivity of the three furanic fuels depends complicatedly on both equivalence ratio and temperature, which was further interpreted by examining the ignition kinetics. As DMF is more branched, H-abstractions contribute most to the fuel consumption. For EF and MF, OH-additions at C2 and C5 positions dominate the reaction pathways. From reaction flux analyses, the reactions involving alkyl side chains of alkylfurans are analogous with those of alkylbenzenes at low to intermediate temperature oxidation conditions. Moreover, large amount of alkylfurans go through OH-addition reactions on the ring, which is not observed in the reaction pathways of alkylbenzenes. (C) 2016 by The Combustion Institute. Published by Elsevier Inc.

Keyword :

Low temperature Ethylfuran Ignition delay times Alkylfurans

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GB/T 7714 Xu, Nan , Wu, Yingtao , Tang, Chenglong et al. Ignition delay times of low alkylfurans at high pressures using a rapid compression machine [J]. | PROCEEDINGS OF THE COMBUSTION INSTITUTE , 2017 , 36 (1) : 323-332 .
MLA Xu, Nan et al. "Ignition delay times of low alkylfurans at high pressures using a rapid compression machine" . | PROCEEDINGS OF THE COMBUSTION INSTITUTE 36 . 1 (2017) : 323-332 .
APA Xu, Nan , Wu, Yingtao , Tang, Chenglong , Zhang, Peng , He, Xin , Wang, Zhi et al. Ignition delay times of low alkylfurans at high pressures using a rapid compression machine . | PROCEEDINGS OF THE COMBUSTION INSTITUTE , 2017 , 36 (1) , 323-332 .
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An ignition delay time and chemical kinetic study of ethane sensitized by nitrogen dioxide EI SCIE Scopus
期刊论文 | 2017 , 207 , 389-401 | FUEL | IF: 4.908
WoS CC Cited Count: 5 SCOPUS Cited Count: 7
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Abstract :

Nitrogen dioxide (NO2) is a dominant component of NOx pollution in combustion of internal combustion engines and gas turbines. Its sensitization on ignition of ethane which is a main component of natural gas has been investigated in this experimental and kinetic study. Ignition delay times of NO2/C2H6/O-2/Ar mixtures, with blending ratios of NO2:C2H6 of 0.3:1 and 1:1, were measured in a shock tube. Experimental conditions cover a range of pressures (1.2-20 atm), temperatures (950-1700 K) and equivalence ratios (0.5-2.0). Similarly to our previous work of CH4/NO2 (Deng et al., 2016) [14], NO2 addition promotes the reactivity of ethane and reduces the global activation energy particularly at higher pressures (p > 5.0 atm) and lower temperatures (T < 1175 K), whereas it only presents a limited effect at low pressure (1.0 atm) and higher temperatures (T > 1175 K). Furthermore, an opposite effect of NO2 addition is observed in both the experiments and the simulations at different temperature regimes. Compared to fuel-rich mixture, NO2 addition exhibits more significantly promoting effect on the ignition of fuel-lean mixture under given NO2 concentration. Four literature kinetic mechanisms and an updated mechanism proposed in this study have been compared to simulate the new ignition delay time data and the literature data. Overall, the proposed model is capable of reproducing the experimental results measured by various facilities over a wide range of conditions. The proposed model is thus used to carry out the sensitivity and flux analyses to clarify the chemistry interaction between NO2 and ethane. Based on the kinetic analyses, the impact of NO2 has been expounded at different conditions. (C) 2017 Elsevier Ltd. All rights reserved.

Keyword :

Chemical sensitization Nitrogen dioxide Ethane Ignition delay times

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GB/T 7714 Deng, Fuquan , Pan, Youshun , Sun, Wuchuan et al. An ignition delay time and chemical kinetic study of ethane sensitized by nitrogen dioxide [J]. | FUEL , 2017 , 207 : 389-401 .
MLA Deng, Fuquan et al. "An ignition delay time and chemical kinetic study of ethane sensitized by nitrogen dioxide" . | FUEL 207 (2017) : 389-401 .
APA Deng, Fuquan , Pan, Youshun , Sun, Wuchuan , Yang, Feiyu , Zhang, Yingjia , Huang, Zuohua . An ignition delay time and chemical kinetic study of ethane sensitized by nitrogen dioxide . | FUEL , 2017 , 207 , 389-401 .
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Ab initio calculation and kinetic modeling study of diethyl ether ignition with application toward a skeletal mechanism for CI engine modeling EI SCIE Scopus
期刊论文 | 2017 , 209 , 509-520 | FUEL | IF: 4.908
WoS CC Cited Count: 3 SCOPUS Cited Count: 4
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Abstract :

Quantum chemistry and rate constants of reactions such as H-abstraction of diethyl ether (DEE) by H, OH, HO2, O and CH3 radicals as well as DEE and DEE radicals decomposition and isomerization were carried out through high-level ab initio and RRKM master equation computations. A comparison was made between some of the calculated rate constants and literature data. A detailed kinetic mechanism for DEE ignition contains 341 species and 1867 reactions was developed mainly based on the theoretical calculation and literature data and it was then further compared with the literature measurements along with three other existing DEE models, the Yasunaga model, the Sakai model and the Tran model. Compared with the other three models, the current model can give reasonable predictions on the validated ignition data over a wider temperature range. Based on the current model, a skeletal mechanism which contains 49 species and 192 reactions was developed by using a Jacobian-aided DRGEP approach, followed with a TSA method. The skeletal mechanism can precisely represent the detailed mechanism under a wide range of compression engine related conditions for DEE ignition. Finally, reaction pathway analysis and sensitivity analysis was conducted using the current model to gain an in-depth comprehension on DEE ignition at different temperatures.

Keyword :

Detailed model Quantum chemistry Diethyl ether Skeletal mechanism Rate constant

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GB/T 7714 Hu, Erjiang , Chen, Yulin , Zhang, Zihang et al. Ab initio calculation and kinetic modeling study of diethyl ether ignition with application toward a skeletal mechanism for CI engine modeling [J]. | FUEL , 2017 , 209 : 509-520 .
MLA Hu, Erjiang et al. "Ab initio calculation and kinetic modeling study of diethyl ether ignition with application toward a skeletal mechanism for CI engine modeling" . | FUEL 209 (2017) : 509-520 .
APA Hu, Erjiang , Chen, Yulin , Zhang, Zihang , Chen, Jyh-Yuan , Huang, Zuohua . Ab initio calculation and kinetic modeling study of diethyl ether ignition with application toward a skeletal mechanism for CI engine modeling . | FUEL , 2017 , 209 , 509-520 .
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The effect of pentanol addition on the particulate emission characteristics of a biodiesel operated diesel engine EI SCIE Scopus
期刊论文 | 2017 , 209 , 132-140 | FUEL | IF: 4.908
WoS CC Cited Count: 8 SCOPUS Cited Count: 10
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Abstract :

In the present study, combustion performance and the physical and chemical characteristics of soot particles from a DI diesel engine were studied. The engine was fueled with n-pentanol mixed with biodiesel at 15% and 30% by volume and operated at 1800 rpm under three engine loads (20%, 50% and 80% load). In comparison with pure biodiesel, the pentanol-biodiesel blends lead to delayed start of combustion and shortened combustion duration. The particle number concentrations of all size groups are reduced for biodiesel-pentanol blends in all the tested conditions, due to longer ignition delay time, lower viscosity and boiling point, and higher oxygen content of pentanol. The brake specific elemental carbon (EC) emissions of biodiesel were found to be lower compared to diesel and after adding pentanol in biodiesel, the EC emissions further decrease. While for organic carbon (OC) emissions, biodiesel and diesel are at similar level under the tested engine loads, and the blends show a higher fraction of OC at low and medium engine loads. The blended fuel with higher proportion of pentanol gives lower total particle-phase PAHs emissions and also a lower benzo[a] pyrene equivalent (BaPeq) compared to pure biodiesel under the tested engine loads.

Keyword :

Pentanol Particulate emissions PAHs Biodiesel OC Diesel engine EC

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GB/T 7714 Yang, Ke , Wei, Long , Cheung, C. S. et al. The effect of pentanol addition on the particulate emission characteristics of a biodiesel operated diesel engine [J]. | FUEL , 2017 , 209 : 132-140 .
MLA Yang, Ke et al. "The effect of pentanol addition on the particulate emission characteristics of a biodiesel operated diesel engine" . | FUEL 209 (2017) : 132-140 .
APA Yang, Ke , Wei, Long , Cheung, C. S. , Tang, Chenglong , Huang, Zuohua . The effect of pentanol addition on the particulate emission characteristics of a biodiesel operated diesel engine . | FUEL , 2017 , 209 , 132-140 .
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Kinetics of H abstraction and addition reactions of 2,4,4-trimethyl-1-pentene by OH radical EI SCIE Scopus
期刊论文 | 2017 , 210 , 646-658 | FUEL | IF: 4.908
WoS CC Cited Count: 3 SCOPUS Cited Count: 4
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Abstract :

The rate coefficients of H abstraction and OH addition reactions of 2,4,4-trimethyl-1-pentene with OH were determined by both canonical variational transition state theory and conventional transition state theory. The potential energy surfaces were calculated at CCSD(T)/6-311++ G(d, p)//BHANDHLYP/6-311(d, p) level and quantum effects were evaluated by the one-dimensional Wigner method and the multidimensional zero-curvature and small-curvature tunneling methods. 2,4,4-Trimethyl-1-pentene contains primary and secondary allylic H abstraction, alkyl, and vinylic H abstraction channels and OH addition into central and terminal carbon atoms channels. The results show that allylic H abstraction channels dominate the overall H abstractions resulting from the lower barriers, in which, primary H abstraction involves indirect channel via a reactant complex and direct channel. Moreover, OH addition reactions into central and terminal carbon atoms all contain Van der Waals reactant complexes, while the latter channel exhibits negative temperature dependence as a result of its submerged barrier. The branching ratio is more than 75% for addition reactions below 500 K and more than 80% above 1100 K for H abstraction reactions. Rate coefficients of all channels were fitted in terms of a quasi-Arrhenius expression.

Keyword :

OH addition Rate coefficient 2,4,4-Trimethyl-1-pentene H abstraction Transition state

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GB/T 7714 Yin, Geyuan , Hu, Erjiang , Yang, Feiyu et al. Kinetics of H abstraction and addition reactions of 2,4,4-trimethyl-1-pentene by OH radical [J]. | FUEL , 2017 , 210 : 646-658 .
MLA Yin, Geyuan et al. "Kinetics of H abstraction and addition reactions of 2,4,4-trimethyl-1-pentene by OH radical" . | FUEL 210 (2017) : 646-658 .
APA Yin, Geyuan , Hu, Erjiang , Yang, Feiyu , Ku, Jinfeng , Huang, Zuohua . Kinetics of H abstraction and addition reactions of 2,4,4-trimethyl-1-pentene by OH radical . | FUEL , 2017 , 210 , 646-658 .
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Experimental and numerical study on the emission characteristics of laminar premixed biogas-hydrogen impinging flame EI SCIE Scopus
期刊论文 | 2017 , 195 , 1-11 | FUEL | IF: 4.908
WoS CC Cited Count: 4 SCOPUS Cited Count: 5
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The total emissions (EICO, EINOx, EINO2 and NO2/NOx ratio) of laminar premixed biogas-hydrogen impinging flame were obtained experimentally while a computational model was developed to calculate the impinging flame. The NO amount produced via different routes (thermal, prompt, NNH and N2O routes) were isolated and calculated in the simulation. The effects of separated distance and equivalence ratio on the emission formation were discussed quantitatively. The results are summarized as follows. The lower values of EICO at small and large H are caused by the weakened fuel oxidization and improved CO oxidization, respectively, and the EICO is increased with phi owing to the increasingly incomplete fuel oxidization. The NO amounts of thermal, prompt, NNH and N2O routes and their contributions on total NO are affected considerably by the separated distance. The decreased prompt NO with H leads to the initial drop of EINOx at fuel-rich condition. The thermal NO and NNH route dominate the NO formation at phi = 0.8 and 1.0, while the contribution of prompt NO is improved significantly at fuel -rich condition. The rising trend of EINOx with phi is primarily predominated by the enhanced prompt NO. As H is enhanced, the rising and dropping trends of EINO2, as well as NO2/NOx ratio, are caused by more intensive air entrainment, promoting the NO2 formation, and the extended high temperature region, accelerating the NO formation and the NO2 destruction, respectively. The enhanced EINO2 with phi is primarily caused by the increased H atom in the air mixing region to promote the HO2 formation. (C) 2017 Elsevier Ltd. All rights reserved.

Keyword :

NO formation Total emissions NO2 production Biogas-hydrogen fuel Flame impingement

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GB/T 7714 Wei, Z. L. , Zhen, H. S. , Leung, C. W. et al. Experimental and numerical study on the emission characteristics of laminar premixed biogas-hydrogen impinging flame [J]. | FUEL , 2017 , 195 : 1-11 .
MLA Wei, Z. L. et al. "Experimental and numerical study on the emission characteristics of laminar premixed biogas-hydrogen impinging flame" . | FUEL 195 (2017) : 1-11 .
APA Wei, Z. L. , Zhen, H. S. , Leung, C. W. , Cheung, C. S. , Huang, Z. H. . Experimental and numerical study on the emission characteristics of laminar premixed biogas-hydrogen impinging flame . | FUEL , 2017 , 195 , 1-11 .
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