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学者姓名:娄晓杰

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High energy density hybrid supercapacitors derived from novel Ni3Se2nanowires: In situ constructed on porous nickel foam EI SCIE
期刊论文 | 2021 , 8 (4) , 1093-1101 | Inorganic Chemistry Frontiers
WoS CC Cited Count: 1
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Abstract :

In this work, novel Ni3Se2 nanowires are synthesized in situ on the surface of nickel foam (Ni3Se2 NWs@NF) through a one-step hydrothermal reaction under different reaction times, and they demonstrate excellent energy storage performance for hybrid supercapacitors (HSCs). Owing to their good electron transfer capability and porous and hierarchical architecture, the as-prepared Ni3Se2 NWs@NF shows a high capacity of 2.6 C cm-2 at 5 mA cm-2 in a three-electrode cell. Even if the current density increases up to 250 mA cm-2, its specific capacity still remains at 0.93 C cm-2, exhibiting excellent rate capability. Furthermore, an HSC was assembled with the as-prepared Ni3Se2 NWs@NF as the positive electrode and activated carbon (AC) as the negative electrode, in 2 M KOH aqueous electrolyte. The Ni3Se2 NWs@NF//AC HSC demonstrates a high energy density of 64.4 W h kg-1 at a power density of 446.8 W kg-1 at 0.43 A g-1 with an extended voltage of 1.6 V, along with outstanding long-term cycling stability that retains 93.9% of the initial capacity after 10?000 cycles. To the best of our knowledge, the Ni3Se2 NWs@NF//AC HSC developed in this work demonstrates the best capacity performance among the reported HSCs with nickel selenides as electrode materials in aqueous electrolytes. Our results manifest that the Ni3Se2 NWs@NF is a promising electrode material for high-performance HSCs. This journal is © the Partner Organisations.

Keyword :

Electrodes Electrolytes Electron transport properties Energy storage Nickel compounds Potassium hydroxide Selenium compounds Supercapacitor

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GB/T 7714 Li, Wei , Chen, Tianqi , Li, Ao et al. High energy density hybrid supercapacitors derived from novel Ni3Se2nanowires: In situ constructed on porous nickel foam [J]. | Inorganic Chemistry Frontiers , 2021 , 8 (4) : 1093-1101 .
MLA Li, Wei et al. "High energy density hybrid supercapacitors derived from novel Ni3Se2nanowires: In situ constructed on porous nickel foam" . | Inorganic Chemistry Frontiers 8 . 4 (2021) : 1093-1101 .
APA Li, Wei , Chen, Tianqi , Li, Ao , Shi, Peng , Wu, Ming , Li, Tingting et al. High energy density hybrid supercapacitors derived from novel Ni3Se2nanowires: In situ constructed on porous nickel foam . | Inorganic Chemistry Frontiers , 2021 , 8 (4) , 1093-1101 .
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Colossal Reversible Barocaloric Effects in Layered Hybrid Perovskite (C10H21NH3)(2)MnCl4 under Low Pressure Near Room Temperature EI SCIE
期刊论文 | 2021 , 31 (46) | ADVANCED FUNCTIONAL MATERIALS
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Abstract :

Barocaloric effects in a layered hybrid organic-inorganic compound, (C10H21NH3)(2)MnCl4, that are reversible and colossal under pressure changes below 0.1 GPa are reported. This barocaloric performance originates in a phase transition characterized by different features: A strong disordering of the organic chains, a very large volume change, a very large sensitivity of the transition temperature to pressure and a small hysteresis. The obtained values are unprecedented among solid-state cooling materials at such low pressure changes and demonstrate that colossal effects can be obtained in compounds other than plastic crystals. The temperature-pressure phase diagram displays a triple point indicating enantiotropy at high pressure.

Keyword :

barocaloric effects calorimetry hybrid layered perovskites phase diagrams Raman scattering

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GB/T 7714 Li, Junning , Barrio, Maria , Dunstan, David J. et al. Colossal Reversible Barocaloric Effects in Layered Hybrid Perovskite (C10H21NH3)(2)MnCl4 under Low Pressure Near Room Temperature [J]. | ADVANCED FUNCTIONAL MATERIALS , 2021 , 31 (46) .
MLA Li, Junning et al. "Colossal Reversible Barocaloric Effects in Layered Hybrid Perovskite (C10H21NH3)(2)MnCl4 under Low Pressure Near Room Temperature" . | ADVANCED FUNCTIONAL MATERIALS 31 . 46 (2021) .
APA Li, Junning , Barrio, Maria , Dunstan, David J. , Dixey, Richard , Lou, Xiaojie , Tamarit, Josep-Lluis et al. Colossal Reversible Barocaloric Effects in Layered Hybrid Perovskite (C10H21NH3)(2)MnCl4 under Low Pressure Near Room Temperature . | ADVANCED FUNCTIONAL MATERIALS , 2021 , 31 (46) .
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Doping-induced Polar Defects Improve the Electrocaloric Performance of Ba0(0.9)Sr(0.1)Hf(0.1)Ti(0.9)O(3) EI SCIE
期刊论文 | 2021 , 16 (1) | PHYSICAL REVIEW APPLIED
WoS CC Cited Count: 2
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In materials science, intentional doping has been widely used to improve the properties of a variety of materials. However, such an approach is not yet exploited in the fast-growing field of electrocaloric materials, which represent a serious alternative for next-generation cooling systems. Here we demonstrate with Ba0.9Sr0.1Hf0.1Ti0.9O3, an ecofriendly ferroelectric material, that doping with 2% of Cu introduces defect dipoles into the ferroelectric matrix and results in (i) enhancement of the adiabatic temperature change AT by up to 54% while maintaining performance after a large number (up to 104) of electric field cycles, (ii) suppression of the parasitic irreversibility of AT between on-field and off -field states, and (iii) an alternative design of refrigeration cycle with a prepoled sample, allowing a two-field-step process showing both conventional (AT> 0) and inverse (AT< 0) responses when the field is sequentially varied. We also demonstrate that doping significantly increases the energy storage density (by up to 72%). The defect engineering approach therefore offers a path for designing ferroelectrics with improved electrocaloric performances. Beyond ferroelectrics, this strategy could also be promising in other solid-state caloric materials (magnetocalorics, elastocalorics, etc.).

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GB/T 7714 Li, Junning , Lv, Jing , Zhang, Dawei et al. Doping-induced Polar Defects Improve the Electrocaloric Performance of Ba0(0.9)Sr(0.1)Hf(0.1)Ti(0.9)O(3) [J]. | PHYSICAL REVIEW APPLIED , 2021 , 16 (1) .
MLA Li, Junning et al. "Doping-induced Polar Defects Improve the Electrocaloric Performance of Ba0(0.9)Sr(0.1)Hf(0.1)Ti(0.9)O(3)" . | PHYSICAL REVIEW APPLIED 16 . 1 (2021) .
APA Li, Junning , Lv, Jing , Zhang, Dawei , Zhang, Lixue , Hao, Xihong , Wu, Ming et al. Doping-induced Polar Defects Improve the Electrocaloric Performance of Ba0(0.9)Sr(0.1)Hf(0.1)Ti(0.9)O(3) . | PHYSICAL REVIEW APPLIED , 2021 , 16 (1) .
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Amino-rich surface-modified MXene as anode for hybrid aqueous proton supercapacitors with superior volumetric capacity EI SCIE
期刊论文 | 2021 , 495 | Journal of Power Sources
WoS CC Cited Count: 2
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Supercapacitors (SCs) have attracted considerable attention due to their outstanding power density and cycling performance. In this work, the amino-rich surface functional groups (–NH– and –N+H-) surface modified Ti3C2Tx MXene nanosheets (N–Ti3C2Tx-200) are synthesized via the solvothermal method, which is accompanied by the generation of surface titanium atom defects. Moreover, kinetic analysis confirms that the surface amino-rich functional groups are in favor of the rapid hydrogen ions transmission within electrode, leading to an enhancement of capacitive capacitance. Specifically, the flexible N–Ti3C2Tx-200 electrode exhibits a volumetric capacity of 936.0 C cm−3, which is 1.49 times that of the pristine Ti3C2Tx. Further, the modified electrode even can keep a volumetric capacity of 839.7 C cm−3 at 1 V s−1, which is much higher than that of the pristine Ti3C2Tx (277.7 C cm−3). More importantly, the hybrid aqueous proton supercapacitors (HAPSs), constructed by N–Ti3C2Tx-200 anode and copper hexacyanoferrate (CuHCF) cathode, achieve a 2 V wide voltage window and an ultrahigh volumetric energy density of 104.9 Wh L−1 at 0.38 kW L−1. This work offers a basic understanding of the amino-rich surface-modified flexible Ti3C2Tx film electrodes with high volumetric energy density and high-rate performance, providing a strategy to fabricate HAPSs with superior volumetric capacity. © 2021 Elsevier B.V.

Keyword :

Anodes Capacitance Copper compounds Nanosheets Supercapacitor Surface treatment

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GB/T 7714 Tian, Yapeng , Que, Bowen , Luo, Yangyang et al. Amino-rich surface-modified MXene as anode for hybrid aqueous proton supercapacitors with superior volumetric capacity [J]. | Journal of Power Sources , 2021 , 495 .
MLA Tian, Yapeng et al. "Amino-rich surface-modified MXene as anode for hybrid aqueous proton supercapacitors with superior volumetric capacity" . | Journal of Power Sources 495 (2021) .
APA Tian, Yapeng , Que, Bowen , Luo, Yangyang , Ju, Maomao , Tang, Yi , Lou, Xiaojie et al. Amino-rich surface-modified MXene as anode for hybrid aqueous proton supercapacitors with superior volumetric capacity . | Journal of Power Sources , 2021 , 495 .
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Extraordinary energy storage performance and thermal stability in sodium niobate-based ceramics modified by the ion disorder and stabilized antiferroelectric orthorhombic R phase EI SCIE
期刊论文 | 2021 , 9 (43) , 24387-24396 | JOURNAL OF MATERIALS CHEMISTRY A
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Developing high-performance dielectric capacitors is essential to meet the growing demands of hybrid electric vehicles and high-power applications. The energy storage efficiency and the temperature-variant energy storage properties should be considered besides the energy density. In this work, we prepared (1 - x)(0.8NaNbO(3)-0.2SrTiO(3)) - xBi(Zn0.5Sn0.5)O-3 (abbreviated as (1 - x)(NN-ST) - xBZS) lead-free ceramics, where ion disorder is induced in the A-B sites. The experimental results indicate that the antiferroelectric orthorhombic R phase is stabilized, and the breakdown strength is enhanced due to the decreased grain size after BZS modification, which are conducive to optimizing the energy storage performance. The piezoresponse force microscopy (PFM) observation reveals that the incorporated BZS promotes the reversibility of domains, resulting in enhanced energy storage efficiency. Therefore, an energy density of 5.82 J cm(-3) and an efficiency of 92.3% are simultaneously obtained in the 0.96(NN-ST) - 0.04BZS composition, and the obtained efficiency in this work reaches a record high in NN-based energy storage ceramics. Especially, the sample displays extraordinary temperature stability, that is, high energy storage density (3.6-4.31 J cm(-3)) and efficiency (90-95%) are achieved in a wide temperature range from -60 degrees C to 180 degrees C. Our work would provide a powerful strategy for designing high-performance energy storage capacitors operating in harsh environments.

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GB/T 7714 Kang, Ruirui , Wang, Zepeng , Yang, Weijie et al. Extraordinary energy storage performance and thermal stability in sodium niobate-based ceramics modified by the ion disorder and stabilized antiferroelectric orthorhombic R phase [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2021 , 9 (43) : 24387-24396 .
MLA Kang, Ruirui et al. "Extraordinary energy storage performance and thermal stability in sodium niobate-based ceramics modified by the ion disorder and stabilized antiferroelectric orthorhombic R phase" . | JOURNAL OF MATERIALS CHEMISTRY A 9 . 43 (2021) : 24387-24396 .
APA Kang, Ruirui , Wang, Zepeng , Yang, Weijie , Zhu, Xiaopei , Shi, Peng , Gao, Yangfei et al. Extraordinary energy storage performance and thermal stability in sodium niobate-based ceramics modified by the ion disorder and stabilized antiferroelectric orthorhombic R phase . | JOURNAL OF MATERIALS CHEMISTRY A , 2021 , 9 (43) , 24387-24396 .
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Enhanced energy storage density of Sr0.7BixTiO3 lead-free relaxor ceramics via A-site defect and grain size tuning EI SCIE
期刊论文 | 2021 , 420 | CHEMICAL ENGINEERING JOURNAL
WoS CC Cited Count: 11
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Abstract :

The application of dielectric capacitors with high energy density is very important to solve the increasingly serious energy crisis. However, the further improvement of energy density is seriously confining by their poor breakdown fields. In this work, outstanding energy storage performance is achieved in Sr0.7BixTiO3 (x = 0.1, 0.2, 0.3 and 0.4) ceramics via A-site defect and grain size tuning. It was found that the moderate Bi3+ content is helpful to reduce sintering temperature and refine grain size, which lead to higher activation energy and breakdown field. Besides, moderate Bi3+ doping in A-site enhances polarity owing to the hybridizations between 6p orbital of Bi and 2p orbital of O. Thus, a high recoverable energy density of 4.77 J/cm(3) with prominent efficiency of 85.7% at 570 kV/cm is realized in Sr0.7Bi0.2TiO3 ceramic. Moreover, the Sr0.7Bi0.2TiO3 ceramic also displays superior thermal stability from 20 degrees C to 160 degrees C and excellent fatigue endurance over 10(5) cycles. Our results in this work offer a better understanding and design methodology for developing novel high-performance dielectric capacitors.

Keyword :

Dielectric capacitors Grain size engineering Recoverable energy density Sr0.7BixTiO3 ceramics

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GB/T 7714 Zhu, Xiaopei , Shi, Peng , Kang, Ruirui et al. Enhanced energy storage density of Sr0.7BixTiO3 lead-free relaxor ceramics via A-site defect and grain size tuning [J]. | CHEMICAL ENGINEERING JOURNAL , 2021 , 420 .
MLA Zhu, Xiaopei et al. "Enhanced energy storage density of Sr0.7BixTiO3 lead-free relaxor ceramics via A-site defect and grain size tuning" . | CHEMICAL ENGINEERING JOURNAL 420 (2021) .
APA Zhu, Xiaopei , Shi, Peng , Kang, Ruirui , Li, Siyi , Wang, Zepeng , Qiao, Wenjing et al. Enhanced energy storage density of Sr0.7BixTiO3 lead-free relaxor ceramics via A-site defect and grain size tuning . | CHEMICAL ENGINEERING JOURNAL , 2021 , 420 .
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Large electric-field-induced strain and energy storage properties in Bi0.5Na0.5TiO3-(0.5Ba0.7Ca0.3TiO3-0.5BaTi0.8Zr0.2O3) lead-free relaxor ferroelectric ceramics EI SCIE
期刊论文 | 2021 , 860 | Journal of Alloys and Compounds
WoS CC Cited Count: 9
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Abstract :

Piezoelectric ceramics with high strain can convert electrical energy and mechanical energy into each other for a wide range of applications. (1-x)Bi0.5Na0.5TiO3-x(0.5Ba0.7Ca0.3TiO3-0.5BaTi0.8Zr0.2O3) (BNT-x(BCT-BZT)) lead-free piezoelectric ceramics were prepared through solid-state reaction methods. The structural, dielectric, field-induced strain and energy storage properties of the ceramics were investigated systematically by various characterization techniques. A large field-induced strain of 0.42% with negligible negative strain and large reverse piezoelectric coefficient of 547 pm/V are obtained in BNT-9(BCT-BZT) ceramics. A large recoverable energy storage of 3.49 J/cm3 under 360 kV/cm and high energy storage efficiency of 64.9% are achieved in the BNT-10(BCT-BZT) ceramics. It believes that the large strain with negligible negative strain is mainly due to the crossover of relaxor nonpolar state to ferroelectric polar state. We believe that the BNT-x(BCT-BZT) ceramics are favorable for the practical applications in the mobile electronic devices. © 2020 Elsevier B.V.

Keyword :

Energy storage Ferroelectric ceramics Ferroelectricity Ferroelectric materials Piezoelectric ceramics Piezoelectricity Solid state reactions

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GB/T 7714 Shi, Peng , Li, Tangyuan , Lou, Xiaojie et al. Large electric-field-induced strain and energy storage properties in Bi0.5Na0.5TiO3-(0.5Ba0.7Ca0.3TiO3-0.5BaTi0.8Zr0.2O3) lead-free relaxor ferroelectric ceramics [J]. | Journal of Alloys and Compounds , 2021 , 860 .
MLA Shi, Peng et al. "Large electric-field-induced strain and energy storage properties in Bi0.5Na0.5TiO3-(0.5Ba0.7Ca0.3TiO3-0.5BaTi0.8Zr0.2O3) lead-free relaxor ferroelectric ceramics" . | Journal of Alloys and Compounds 860 (2021) .
APA Shi, Peng , Li, Tangyuan , Lou, Xiaojie , Yu, Zhonghai , Zhu, Xiaopei , Zhou, Chao et al. Large electric-field-induced strain and energy storage properties in Bi0.5Na0.5TiO3-(0.5Ba0.7Ca0.3TiO3-0.5BaTi0.8Zr0.2O3) lead-free relaxor ferroelectric ceramics . | Journal of Alloys and Compounds , 2021 , 860 .
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Atomic-scale fatigue mechanism of ferroelectric tunnel junctions EI SCIE PubMed
期刊论文 | 2021 , 7 (48) | SCIENCE ADVANCES
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Ferroelectric tunnel junctions (FTJs) are promising candidates for next-generation memories due to fast read/write speeds and low-power consumptions. Here, we investigate resistance fatigue of FTJs, which is performed on Pt/BaTiO3/Nb:SrTiO3 devices. By direct observations of the 5-unit cell-thick BaTiO3 barrier with high-angle annular dark-field imaging and electron energy loss spectroscopy, oxygen vacancies are found to aggregate at the Pt/ BaTiO3 interface during repetitive switching, leading to a ferroelectric dead layer preventing domain nucleation and growth. Severe oxygen deficiency also makes BaTiO3 lattices energetically unfavorable and lastly induces a destruction of local perovskite structure of the barrier. Ferroelectric properties are thus degraded, which reduces barrier contrast between ON and OFF states and smears electroresistance characteristics of Pt/BaTiO3/Nb:SrTiO3 FTJs. These results reveal an atomic-scale fatigue mechanism of ultrathin ferroelectric barriers associated with the aggregation of charged defects, facilitating the design of reliable FTJs and ferroelectric nanoelectronic devices for practical applications.

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GB/T 7714 Yang, Yihao , Wu, Ming , Zheng, Xingwen et al. Atomic-scale fatigue mechanism of ferroelectric tunnel junctions [J]. | SCIENCE ADVANCES , 2021 , 7 (48) .
MLA Yang, Yihao et al. "Atomic-scale fatigue mechanism of ferroelectric tunnel junctions" . | SCIENCE ADVANCES 7 . 48 (2021) .
APA Yang, Yihao , Wu, Ming , Zheng, Xingwen , Zheng, Chunyan , Xu, Jibo , Xu, Zhiyu et al. Atomic-scale fatigue mechanism of ferroelectric tunnel junctions . | SCIENCE ADVANCES , 2021 , 7 (48) .
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Bi0.5Na0.5TiO3-based lead-free ceramics with superior energy storage properties at high temperatures EI SCIE
期刊论文 | 2021 , 215 | Composites Part B: Engineering
WoS CC Cited Count: 14
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Dielectric capacitors with high energy storage and dielectric properties at high temperatures have significantly practical application in many fields. Lead-free ceramics of (1-x)(0.65Bi0.5Na0.5TiO3-0.35Bi0.2Sr0.7TiO3)-xBaSnO3 were prepared by a solid-state reaction method. It was found that the 0.8(0.65Bi0.5Na0.5TiO3-0.35Bi0.2Sr0.7TiO3)-0.2BaSnO3 ceramic shows a large recoverable energy storage density (Wr) of 3.75 J/cm3 and efficiency (η) of 84.8% under 380 kV/cm along with outstanding power density of 38.73 MW/cm3 under 130 kV/cm at room temperature. Additionally, a high Wr of 3.21 J/cm3 and η of 77% are achieved under a high electric field of 300 kV/cm at 100 °C. When the temperature reaches 140 °C, it still has a high Wr of 3.1 J/cm3 and η of 72%. The outstanding energy storage performance at high temperatures can be explained by the enhancement of breakdown strength and the constructing of polar phase stability caused by the introduction of BaSnO3. © 2021 Elsevier Ltd

Keyword :

Barium compounds Ceramic materials Dielectric properties Electric fields Energy storage Ferroelectric materials Solid state reactions

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GB/T 7714 Shi, Peng , Zhu, Xiaopei , Lou, Xiaojie et al. Bi0.5Na0.5TiO3-based lead-free ceramics with superior energy storage properties at high temperatures [J]. | Composites Part B: Engineering , 2021 , 215 .
MLA Shi, Peng et al. "Bi0.5Na0.5TiO3-based lead-free ceramics with superior energy storage properties at high temperatures" . | Composites Part B: Engineering 215 (2021) .
APA Shi, Peng , Zhu, Xiaopei , Lou, Xiaojie , Yang, Bian , Guo, Xudong , He, Liqiang et al. Bi0.5Na0.5TiO3-based lead-free ceramics with superior energy storage properties at high temperatures . | Composites Part B: Engineering , 2021 , 215 .
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Sulfate assisted synthesis of alpha-type nickel hydroxide nanowires with 3D reticulation for energy storage in hybrid supercapacitors EI SCIE Scopus
期刊论文 | 2021 , 6 (1) , 94-102 | MATERIALS CHEMISTRY FRONTIERS
SCOPUS Cited Count: 6
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Nickel hydroxide, as a high high-efficiency electroactive material, is a promising electroactive material for advanced hybrid supercapacitors due to its high theoretical capacity, low-cost, and good thermal and chemical stabilities. Although various nanostructures of nickel hydroxide have been widely reported for energy storage devices, such as nanoparticles, nanosheets, nanoflowers, and so on, nickel hydroxide with one-dimensional nanowire morphology has been rarely investigated until now. Meanwhile, previous reports have shown that the energy storage performance of alpha-Ni(OH)(2) is superior to other types of nickel hydroxides. Based on the above points of view, alpha type Ni(OH)(2) nanowires with three-dimensional (3D) reticulation containing SO42- (abbreviated as NSOH NWs) were successfully obtained by a sulfate assisted hydrothermal approach in the present work and further employed as an electroactive material in hybrid supercapacitors (HSCs). The formation mechanism of the NSOH and the effects of SO42- are also discussed. Thanks to its novel 3D porous morphology and alpha-type phase structure, the as-prepared NSOH NW electrode presents a high specific capacity of 246.3 mA h g(-1) at 1 A g(-1), along with a good cycling stability of 91.7% after 4000 cycles. Meanwhile, the as-assembled NSOH NWs//AC HSCs can provide a high energy density of 59.8 W h kg(-1) at a power density of 830.3 W kg(-1). The HSCs also show 91.5% specific capacity retention after 10 000 cycles. All above results manifest that the proposed NSOH NWs with 3D reticulation have significant potential for advanced HSC applications.

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GB/T 7714 Li, Wei , Huang, Zhongzheng , Jia, Yaduo et al. Sulfate assisted synthesis of alpha-type nickel hydroxide nanowires with 3D reticulation for energy storage in hybrid supercapacitors [J]. | MATERIALS CHEMISTRY FRONTIERS , 2021 , 6 (1) : 94-102 .
MLA Li, Wei et al. "Sulfate assisted synthesis of alpha-type nickel hydroxide nanowires with 3D reticulation for energy storage in hybrid supercapacitors" . | MATERIALS CHEMISTRY FRONTIERS 6 . 1 (2021) : 94-102 .
APA Li, Wei , Huang, Zhongzheng , Jia, Yaduo , Cui, Yunlong , Shi, Peng , Li, Tingting et al. Sulfate assisted synthesis of alpha-type nickel hydroxide nanowires with 3D reticulation for energy storage in hybrid supercapacitors . | MATERIALS CHEMISTRY FRONTIERS , 2021 , 6 (1) , 94-102 .
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