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学者姓名：陈黎
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Abstract ：
Electrode morphological features and the electrolyte inflow pattern are important factors in determining the performance of vanadium redox flow batteries. In this study, a 2-D numerical model that couples electrolyte flow, ion diffusion, and electrochemical reaction is proposed to quantitatively investigate the mass transport and electrochemical reactions at various electrode structures, including the effects of porosity, fiber size, and fiber array pattern, as well as the electrode compression and the electrolyte inflow pattern. The influence of stochastic seeds on the reconstructed geometry was considered and assemble average value was conducted. The established model with the reconstructed geometry has been validated by experiment. The specific surface area, flow resistance, and VO2+ consumption rate increase with a decreasing in electrode porosity and fiber diameter. The fiber array pattern with a 'outlet dense and inlet sparse' structure shows the optimum performance of rapid VO2+ consumption rate and high electrode utilization. The mass transport is dominated by convection in a wide flow path within the electrode, and the collective effects of convection and diffusion are found in a narrow flow path. The main advantage of the compressed electrode is the enhanced electrode utilization. A turning point at a stoich (the ratio of input reactant moles versus the consumed moles at a certain applied current) about 1000 was identified, below which the consumption rate of the flow-through pattern is higher than that of the flow field pattern and above which the consumption rate of the former pattern is slower than the latter. A faster fuel feed in the electrode with a narrower flow channel contributes to a faster species consumption rate in the last stage of the discharge process. The present study provides practical guidance for the design and optimization of VRFB electrode. © 2020 Elsevier Ltd
Keyword ：
Channel flow Electric discharges Electrochemical electrodes Electrolytes Fibers Flow batteries Porosity Stochastic systems Structural optimization Vanadium Vanadium dioxide
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| GB/T 7714 | Wang, Q , Qu, Z.G , Jiang, Z.Y et al. The numerical study of vanadium redox flow battery performance with different electrode morphologies and electrolyte inflow patterns [J]. | Journal of Energy Storage , 2021 , 33 . |
| MLA | Wang, Q et al. "The numerical study of vanadium redox flow battery performance with different electrode morphologies and electrolyte inflow patterns" . | Journal of Energy Storage 33 (2021) . |
| APA | Wang, Q , Qu, Z.G , Jiang, Z.Y , Yin, Y , Chen, L . The numerical study of vanadium redox flow battery performance with different electrode morphologies and electrolyte inflow patterns . | Journal of Energy Storage , 2021 , 33 . |
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Abstract ：
Energy consumption continues to rise as society develops worldwide. Meanwhile, a lot of energy is wasted in the form of heat from various devices and systems. Here we report a new power generator, which works based on a difference in H+-ion concentration in a fuel cell structure and produces electricity by harvesting waste heat. The device works via the following three successive processes: H2 is oxidized at anode to H+ ions, the H+ ions then penetrate through a phosphoric acid-treated polybenzimidazole (PBI-PA) membrane and finally the H+ ions get reduced to H2 at cathode with electrons coming through external circuit from the anode. This system generates electricity at a current density of 21 mA cm−2 and a power density of 1.03 mW cm−2 at 170 °C. The cell's thermoelectric conversion efficiency at 170 °C is 13.72%, which is higher than typical values reported for many common thermoelectric materials in low temperature regimes. This innovative approach may allow for efficient generation of electricity from waste heat. © 2018 Elsevier Ltd
Keyword ：
Electrical energy Innovative approaches Ion concentrations Low-temperature regime Renewable energies Thermal conversion Thermoelectric conversion efficiency Thermo-Electric materials
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| GB/T 7714 | Liu, Yan , Chen, Yuanzhen , Ming, Jun et al. Harvesting waste heat energy by promoting H+-ion concentration difference with a fuel cell structure [J]. | Nano Energy , 2019 , 57 : 101-107 . |
| MLA | Liu, Yan et al. "Harvesting waste heat energy by promoting H+-ion concentration difference with a fuel cell structure" . | Nano Energy 57 (2019) : 101-107 . |
| APA | Liu, Yan , Chen, Yuanzhen , Ming, Jun , Chen, Li , Shu, Chengyong , Qu, Ting et al. Harvesting waste heat energy by promoting H+-ion concentration difference with a fuel cell structure . | Nano Energy , 2019 , 57 , 101-107 . |
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Abstract ：
For applications of reactive transport in porous media, optimal porous structures should possess both high surface area for reactive sites loading and low mass transport resistance. Hierarchical porous media with a combination of pores at different scales are designed for this purpose. Using the lattice Boltzmann method, pore-scale numerical studies are conducted to investigate diffusion-reaction processes in 2D hierarchical porous media generated by self-developed reconstruction scheme. Complex interactions between porous structures and reactive transport are revealed under different conditions. Simulation results show that adding macropores can greatly enhance the mass transport, but at the same time reduce the reactive surface, leading to complex change trend of the total reaction rate. Effects of gradient distribution of macropores within the porous medium are also investigated. It is found that a front-loose, back-tight (FLBT) hierarchical structure is desirable for enhancing mass transport, increasing total reaction rate, and improving catalyst utilization. On the whole, from the viewpoint of reducing cost and improving material performance, hierarchical porous structures, especially gradient structures with the size of macropores gradually decreasing along the transport direction, are desirable for catalyst application.
Keyword ：
Catalyst utilization Gradient distribution Hierarchical porous media Lattice Boltzmann method Pore-scale
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| GB/T 7714 | Chen, Li , Zhang, Ruiyuan , Min, Ting et al. Pore-scale study of effects of macroscopic pores and their distributions on reactive transport in hierarchical porous media [J]. | CHEMICAL ENGINEERING JOURNAL , 2018 , 349 : 428-437 . |
| MLA | Chen, Li et al. "Pore-scale study of effects of macroscopic pores and their distributions on reactive transport in hierarchical porous media" . | CHEMICAL ENGINEERING JOURNAL 349 (2018) : 428-437 . |
| APA | Chen, Li , Zhang, Ruiyuan , Min, Ting , Kang, Qinjun , Tao, Wenquan . Pore-scale study of effects of macroscopic pores and their distributions on reactive transport in hierarchical porous media . | CHEMICAL ENGINEERING JOURNAL , 2018 , 349 , 428-437 . |
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Abstract ：
Nucleate boiling heat transfer (NBHT) from enhanced structures is an effective way to dissipate a high heat flux. In the present study, the behavior of cavities with nucleation on roughened surfaces is studied numerically during the entire ebullition cycle based on the phase-change lattice Boltzmann method. The adopted model is firstly validated by the Laplace law and the two-phase coexistence curve and then is applied to investigate the effects of the cavity structure on NBHT. The bubble departure diameter, departure frequency, and the total boiling heat flux of the ebullition cycle are also studied. It is shown that the cavity widths and the cavity grooves exhibit a significant influence on the NBHT features. A cavity with a circular groove in the present research shows the best performance for NBHT in terms of the averaged heat flux and bubble release frequency. When a specific cavity is combined with other different cavities on roughened surfaces, its nucleation process on different roughened surfaces may differ greatly.
Keyword ：
bubble dynamics cavity groove lattice Boltzmann method nucleate boiling
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| GB/T 7714 | Mu, Yu-Tong , Chen, Li , Kang, Qin-Jun et al. EVALUATION OF THE PERFORMANCE OF CAVITIES IN NUCLEATE BOILING AT MICROSCALE LEVEL [C] . 2018 : 1003-1022 . |
| MLA | Mu, Yu-Tong et al. "EVALUATION OF THE PERFORMANCE OF CAVITIES IN NUCLEATE BOILING AT MICROSCALE LEVEL" . (2018) : 1003-1022 . |
| APA | Mu, Yu-Tong , Chen, Li , Kang, Qin-Jun , Tao, Wen-Quan . EVALUATION OF THE PERFORMANCE OF CAVITIES IN NUCLEATE BOILING AT MICROSCALE LEVEL . (2018) : 1003-1022 . |
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Abstract ：
In this paper, the through-plane and in-plane effective transport properties, including permeability, diffusivity and thermal conductivity, of the perforated gas diffusion layer (GDL) are predicted using multiple-relaxation-time (MRT) lattice Boltzmann method (LBM) based on stochastic reconstructed microstructures. When predicting effective thermal conductivities of GDL, the effect of anisotropic conductive property of fibers is considered. The effective transport properties of dry perforated GDL are fitted as a function of perforation diameter and porosity. It is found that the permeability and effective diffusivity of GDL increase with perforation diameter and porosity while the effective thermal conductivity decreases. The two-phase LBM is adopted to simulate water distributions in perforated GDLs, and dependences of effective transport properties on saturation are then obtained. The results show that: the existence of the perforation significantly affects the water transport in hydrophobic perforated GDLs if its diameter is larger than the average pore size of GDL. The effective permeability and diffusivity of GDL decrease while effective thermal conductivity increases with saturation. The effective transport properties of perforated GDLs change less significantly with saturation than those of non-perforated GDL if the water droplet intruding into the perforation is displaced, while change more rapidly with saturation if the water droplet remains inside the perforation. (C) 2018 Published by Elsevier Ltd.
Keyword ：
Effective transport property Gas diffusion layer Lattice Boltzmann method Multiple-relaxation-time Perforation Saturation
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| GB/T 7714 | Fang, Wen-Zhen , Tang, Yu-Qing , Chen, Li et al. Influences of the perforation on effective transport properties of gas diffusion layers [J]. | INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER , 2018 , 126 : 243-255 . |
| MLA | Fang, Wen-Zhen et al. "Influences of the perforation on effective transport properties of gas diffusion layers" . | INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER 126 (2018) : 243-255 . |
| APA | Fang, Wen-Zhen , Tang, Yu-Qing , Chen, Li , Kang, Qin-Jun , Tao, Wen-Quan . Influences of the perforation on effective transport properties of gas diffusion layers . | INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER , 2018 , 126 , 243-255 . |
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Abstract ：
In the present paper, a patching type multi-block lattice Boltzmann method is adopted to predict the thermal contact resistance (TCR) at the interface of two solids. The rough surfaces of contact materials are reconstructed based on the fractal theory and the contact pressure is obtained based on the plastic deformation model. The accuracy of the patching type multi-block lattice Boltzmann method is validated by some benchmarks. After validations, effects of the contact pressure, roughness, thermal conductivity of contact material, thermal conductivity of interstitial medium, temperature and radiation on TCR are investigated. The results show that: the TCR decreases when the contact pressure increases, but increases with the root-mean-square roughness; the TCR of two contact aluminums decreases faster than that of stainless steels when contact pressure increases; a higher thermal conductivity of contact materials leads to a smaller TCR; when the thermal conductivity of interstitial medium is close to zero or the gap is in vacuum, the TCR is much larger than that filled with air, especially at low contact pressure; at the high temperature, the contribution of the radiation to the TCR becomes appreciable if the thermal conductivity of the interstitial medium is low. Especially when the gap is in vacuum, the contribution of radiation on the TCR cannot be neglected.
Keyword ：
Fractal Lattice Boltzmann method Multi-block Thermal contact resistance
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| GB/T 7714 | Fang, Wen-Zhen , Gou, Jian-Jun , Chen, Li et al. A multi-block lattice Boltzmann method for the thermal contact resistance at the interface of two solids [J]. | APPLIED THERMAL ENGINEERING , 2018 , 138 : 122-132 . |
| MLA | Fang, Wen-Zhen et al. "A multi-block lattice Boltzmann method for the thermal contact resistance at the interface of two solids" . | APPLIED THERMAL ENGINEERING 138 (2018) : 122-132 . |
| APA | Fang, Wen-Zhen , Gou, Jian-Jun , Chen, Li , Tao, Wen-Quan . A multi-block lattice Boltzmann method for the thermal contact resistance at the interface of two solids . | APPLIED THERMAL ENGINEERING , 2018 , 138 , 122-132 . |
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Abstract ：
Reducing Platinum amount in proton exchange membrane fuel cell (PEMFC) is one of the main tasks to achieve low cost PEMFC. Recently, significant performance loss has been found under low Pt loading due to local mass transport limitations. In this study, pore-scale simulations are conducted to study oxygen transport within four-constituent microscopic structures of catalyst layer including a carbon particle, ionomer, Pt particles, and primary pores inside the carbon particle. Multiphase physicochemical processes are considered, including oxygen dissolution at the pore/ionomer interface, oxygen diffusion within the ionomer film and inside the primary pores, and reactions at the Pt interface. Local transport resistance is calculated based on the pore-scale concentration field predicted. The simulation results are compared with existing experimental results and 1D models. Simulation results show that dissolution resistance at the secondary pore/ionomer interface is about 10–50 times higher than that inside the ionomoer. Local transport resistance increases as Pt loading decreases, especially under Pt loading of 0.1 mg cm−2. Besides, local transport resistance can be reduced by depositing more Pt outside the carbon particle, alleviating agglomeration and/or decreasing the ionomer thickness. The simulation results indicate that local transport characteristics should be considered when developing 1D agglomeration model of catalyst layer. © 2018 Elsevier B.V.
Keyword ：
Catalyst layers Lattice Boltzmann method Local transport Mass transport limitation Microscopic structures Nano-scale simulations Physicochemical process Pore-scale simulation
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| GB/T 7714 | Chen, Li , Zhang, Ruiyuan , He, Pu et al. Nanoscale simulation of local gas transport in catalyst layers of proton exchange membrane fuel cells [J]. | Journal of Power Sources , 2018 , 400 : 114-125 . |
| MLA | Chen, Li et al. "Nanoscale simulation of local gas transport in catalyst layers of proton exchange membrane fuel cells" . | Journal of Power Sources 400 (2018) : 114-125 . |
| APA | Chen, Li , Zhang, Ruiyuan , He, Pu , Kang, Qinjun , He, Ya-Ling , Tao, Wen-Quan . Nanoscale simulation of local gas transport in catalyst layers of proton exchange membrane fuel cells . | Journal of Power Sources , 2018 , 400 , 114-125 . |
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Abstract ：
Solubility trapping is crucial for permanent CO 2 sequestration in deep saline aquifers. For the first time, a pore-scale numerical method is developed to investigate coupled scCO(2)-water two-phase flow, multicomponent (CO2(aq), H+, HCO3, CO32- and OH ) mass transport, heterogeneous interfacial dissolution reaction, and homogeneous dissociation reactions. Pore-scale details of evolutions of multiphase distributions and concentration fields are presented and discussed. Time evolutions of several variables including averaged CO2(aq) concentration, scCO(2) saturation, and pH value are analyzed. Specific interfacial length, an important variable which cannot be determined but is required by continuum models, is investigated in detail. Mass transport coefficient or efficient dissolution rate is also evaluated. The pore-scale results show strong non-equilibrium characteristics during solubility trapping due to non-uniform distributions of multiphase as well as slow mass transport process. Complicated coupling mechanisms between multiphase flow, mass transport and chemical reactions are also revealed. Finally, effects of wettability are also studied. The pore-scale studies provide deep understanding of non-linear non-equilibrium multiple physicochemical processes during CO2 solubility trapping processes, and also allow to quantitatively predict some important empirical relationships, such as saturation-interfacial surface area, for continuum models.
Keyword ：
CO2 sequestration Lattice Boltzmann method Multiphase flow Porous media Reactive transport Solubility trapping
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| GB/T 7714 | Chen, Li , Wang, Mengyi , Kang, Qinjun et al. Pore scale study of multiphase multicomponent reactive transport during CO2 dissolution trapping [J]. | ADVANCES IN WATER RESOURCES , 2018 , 116 : 208-218 . |
| MLA | Chen, Li et al. "Pore scale study of multiphase multicomponent reactive transport during CO2 dissolution trapping" . | ADVANCES IN WATER RESOURCES 116 (2018) : 208-218 . |
| APA | Chen, Li , Wang, Mengyi , Kang, Qinjun , Tao, Wenquan . Pore scale study of multiphase multicomponent reactive transport during CO2 dissolution trapping . | ADVANCES IN WATER RESOURCES , 2018 , 116 , 208-218 . |
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Abstract ：
Droplet wetting and distortion on flat surfaces with heterogeneous wettability are studied using the 3D Shan Chen pseudopotential multiphase lattice Boltzmann model (LBM). The contact angles are compared with the Cassie mode, which predicts an apparent contact angle for flat surfaces with different wetting properties, where the droplet size is large compared to the size of the heterogeneity. In this study, the surface studied consists in a regular checkboard pattern with two different Young's contact angles (hydrophilic and hydrophobic) and equal surface fraction. The droplet size and patch size of the checkboard are varied beyond the limit where Cassie's equation is valid. A critical ratio of patch size to droplet radius is found below which the apparent contact angle follows the Cassie mode. Above the critical value, the droplet shape changes from a spherical cap to a more distorted form, and no single contact angle can be determined. The local contact angles are found to vary along the contact line between minimum and maximum values. The droplet is found to wet preferentially the hydrophilic region, and the wetted area fraction of the hydrophilic region increases quasi-linearly with the ratio between patch and droplet sizes. We propose a new equation beyond the critical ratio, defining an equivalent contact angle, where the wetted area fractions are used as weighting coefficients for the maximum and minimum local contact angles. This equivalent contact angle is found to equal Cassie's contact angle.
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| GB/T 7714 | Carmeliet, Jan , Chen, Li , Kang, Qinjun et al. Beyond-Cassie Mode of Wetting and Local Contact Angles of Droplets on Checkboard-Patterned Surfaces [J]. | LANGMUIR , 2017 , 33 (24) : 6192-6200 . |
| MLA | Carmeliet, Jan et al. "Beyond-Cassie Mode of Wetting and Local Contact Angles of Droplets on Checkboard-Patterned Surfaces" . | LANGMUIR 33 . 24 (2017) : 6192-6200 . |
| APA | Carmeliet, Jan , Chen, Li , Kang, Qinjun , Derome, Dominique . Beyond-Cassie Mode of Wetting and Local Contact Angles of Droplets on Checkboard-Patterned Surfaces . | LANGMUIR , 2017 , 33 (24) , 6192-6200 . |
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Abstract ：
This article applied the multiple relaxation time multicomponent/multiphase pseudopotential lattice Boltzmann model to simulate two immiscible fluids flow in 2D porous media, and analyzed the effects of capillary number (Ca), viscosity ratio (M) and wettability on the relative permeability curves. Simulation results indicate that the nonwetting phase (NWP) relative permeability increases with increasing Ca; while the effect of Ca on the wetting phase (WP) relative permeability depends on the wettability. When M > 1, the NWP relative permeability increase with increasing M in a strong wetting condition because of the lubricating effect. The amplitude of the NWP relative permeability may even exceed the single phase permeability. However, the exact value of the amplitude and where it occurs depends on M and the structure of the porous media. The WP relative permeability is insensitive to M. When the porous media converts from strong wetting condition to neutral wetting condition, the NWP relative permeability decreases while the WP relative permeability increases.
Keyword ：
Lattice Boltzmann method Relative permeability Two phase flow
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| GB/T 7714 | Zhao, Huawei , Ning, Zhengfu , Kang, Qinjun et al. Relative permeability of two immiscible fluids flowing through porous media determined by lattice Boltzmann method [J]. | INTERNATIONAL COMMUNICATIONS IN HEAT AND MASS TRANSFER , 2017 , 85 : 53-61 . |
| MLA | Zhao, Huawei et al. "Relative permeability of two immiscible fluids flowing through porous media determined by lattice Boltzmann method" . | INTERNATIONAL COMMUNICATIONS IN HEAT AND MASS TRANSFER 85 (2017) : 53-61 . |
| APA | Zhao, Huawei , Ning, Zhengfu , Kang, Qinjun , Chen, Li , Zhao, Tianyi . Relative permeability of two immiscible fluids flowing through porous media determined by lattice Boltzmann method . | INTERNATIONAL COMMUNICATIONS IN HEAT AND MASS TRANSFER , 2017 , 85 , 53-61 . |
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