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Author:

Chen, Li (Chen, Li.) (Scholars:陈黎) | Luan, Hui-Bao (Luan, Hui-Bao.) | He, Ya-Ling (He, Ya-Ling.) (Scholars:何雅玲) | Tao, Wen-Quan (Tao, Wen-Quan.) (Scholars:陶文铨)

Indexed by:

SCIE EI Scopus

Abstract:

Lattice Boltzmann method (LBM) is used to investigate liquid water transport and distribution in a porous gas diffusion layer (GDL). The GDL with microscopic porous structures is obtained from three-dimensional reconstruction using the stochastic method, and its macroscopic transport properties including permeability and effective diffusivity are numerically predicted which agree well with the existing experimental results. Simulation results show that liquid water transport mechanism in the GDL is capillary fingering and liquid water pathway is interconnected, which confirms the previous experimental results in literature. Further, effects of GC wettability are explored and it is found out that a hydrophilic GC leads to less liquid water accumulated in the GDL compared with a hydrophobic GC. In addition, effects of GDL wettability on liquid water distribution are explored. Simulation results show that PTFE content itself cannot determine liquid water distribution inside the GDL and detailed distributions of hydrophobic and hydrophilic regions within the GDL also play an import role. Moreover, a hydrophilic GDL is more beneficial for reactant transport than a hydrophobic GDL if liquid water presents as separated droplets or films in the GDL.

Keyword:

gas diffusion layer lattice Boltzmann method liquid water proton exchange membrane fuel cell wettability

Author Community:

  • [ 1 ] [Chen, Li; Luan, Hui-Bao; He, Ya-Ling; Tao, Wen-Quan] Xi An Jiao Tong Univ, Key Lab Thermal Fluid Sci & Engn, MOE Sch Energy & Power Engn, Xian 710049, Shaanxi, Peoples R China

Reprint Author's Address:

  • 陶文铨

    Xi An Jiao Tong Univ, Key Lab Thermal Fluid Sci & Engn, MOE Sch Energy & Power Engn, Xian 710049, Shaanxi, Peoples R China.

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Source :

RUSSIAN JOURNAL OF ELECTROCHEMISTRY

ISSN: 1023-1935

Year: 2012

Issue: 7

Volume: 48

Page: 712-726

0 . 5 0 1

JCR@2012

1 . 0 7 8

JCR@2020

ESI Discipline: CHEMISTRY;

ESI HC Threshold:255

JCR Journal Grade:4

CAS Journal Grade:4

Cited Count:

WoS CC Cited Count: 33

SCOPUS Cited Count: 47

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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