Ni-based　superalloy　with　ceramic　thermal　barrier　coatings　(TBCs)　is　a　composite　material,　which　can　be　used　in　special　environments　with　high　temperature　and　high　pressure　such　as　aeroengine　blade.　In　order　to　improve　the　cooling　effect　of　the　aeroengine,　it　is　necessary　to　perform　multi-size　and　large-area　holes　processing　on　the　surface　of　blades.　As　a　non-contact　processing　method　with　fast　processing　speed,　good　processing　quality　and　almost　no　deformation,　laser　processing　has　been　one　of　the　important　processing　methods　for　film　cooling　hole　processing　of　aeroengine　blades.　Percussion　drilling　is　presented　using　picosecond　ultrashort　pulse　laser　in　order　to　explore　processing　of　deep　holes　in　Ni-based　superalloy,　ceramic　TBCs,　and　ceramic　TBCs/substrate　multilayer　material.　The　effects　of　pulses,　threshold　and　wavelength　on　hole　diameter　have　been　discussed,　and　the　experiment　on　the　deep　hole　ablation　with　1064　nm　wavelength　has　been　performed.　By　analyzing　the　hole　size　and　morphological　characteristics　of　multiple　processing　parameters,　the　variation　of　hole　cylindricity　is　obtained.　A　high-quality　hole,　without　spatters　around　the　periphery　of　hole　entrance　and　without　recast　layer　on　the　side-wall　surface,　in　Ni-based　superalloy　coated　with　ceramic　TBCs　has　been　drilled.　This　research　has　potential　applications　to　blade　film　cooling　holes.　©　2020　by　the　authors.